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Plasma-Derived Atomic Hydrogen Enables Eley-Rideal-Type CO Methanation at Low Temperatures.
JACS Au
January 2025
Department of Mechanical Engineering, Tokyo Institute of Technology, Tokyo 152-8550, Japan.
Activating H molecules into atomic hydrogen and utilizing their intrinsic chemical reactivity are important processes in catalytic hydrogenation. Here, we have developed a plasma-catalyst combined system that directly provides atomic hydrogen from the gas phase to the catalytic reaction to utilize the high energy and translational freedom of atomic hydrogen. In this system, we show that the temperature of CO methanation over Ni/AlO can be dramatically lower compared to thermal catalysis.
View Article and Find Full Text PDFBiocatalytic Strategies for Nitration Reactions.
JACS Au
January 2025
Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy, Qingdao New Energy Shandong Laboratory, CAS Key Laboratory of Biofuels, Shandong Provincial Key Laboratory of Synthetic Biology, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao 266101, China.
Nitro compounds are key synthetic intermediates used as enabling tools in synthesis and found in a large range of essential compounds, including pharmaceuticals, pesticides, and various organic dyes. Despite recent methodological developments, the industrial preparation of nitro compounds still suffers from harsh reaction conditions, along with poor selectivity and a problematic environmental footprint. Although biological enzymatic methods exist, mild approaches for bionitration are still underexplored.
View Article and Find Full Text PDFInsight into the Synergistic Effect of Binary Nonmetallic Codoped CoO Catalysts for Efficient Ethyl Acetate Degradation under Humid Conditions.
JACS Au
January 2025
School of Environment and Architecture, University of Shanghai for Science and Technology, Shanghai 200093, China.
The synthesis of high-performance catalysts for volatile organic compounds (VOCs) degradation under humid conditions is essential for their practical industrial application. Herein, a codoping strategy was adopted to synthesize the N-CoO-C catalyst with N, C codoping for low-temperature ethyl acetate (EA) degradation under humid conditions. Results showed that N-CoO-C exhibited great catalytic activity ( = 177 °C) and water resistance (5.
View Article and Find Full Text PDFValorization of agro-industrial waste through solid-state fermentation: Mini review.
Biotechnol Rep (Amst)
March 2025
Department of Chemical and Biological Engineering, American University of Sharjah, Sharjah, P.O.Box 2666, United Arab Emirates.
Agriculture and industrial waste are produced in large volumes every year worldwide, causing serious concerns about their disposal. These wastes have high organic content, which microorganisms can easily assimilate into relevant value-added products. Valorization of agro-industrial waste is required for sustainable development.
View Article and Find Full Text PDFA Manta Ray-Inspired Biosyncretic Robot with Stable Controllability by Dynamic Electric Stimulation.
Cyborg Bionic Syst
July 2022
State Key Laboratory of Robotics, Shenyang Institute of Automation, Chinese Academy of Sciences, Shenyang 110016, China.
Biosyncretic robots, which are new nature-based robots in addition to bionic robots, that utilize biological materials to realize their core function, have been supposed to further promote the progress in robotics. Actuation as the main operation mechanism relates to the robotic overall performance. Therefore, biosyncretic robots actuated by living biological actuators have attracted increasing attention.
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