We report coherent optical control of a biexciton (two electron-hole pairs), confined in a single quantum dot, that shows coherent oscillations similar to the excited-state Rabi flopping in an isolated atom. The pulse control of the biexciton dynamics, combined with previously demonstrated control of the single-exciton Rabi rotation, serves as the physical basis for a two-bit conditional quantum logic gate. The truth table of the gate shows the features of an all-optical quantum gate with interacting yet distinguishable excitons as qubits. Evaluation of the fidelity yields a value of 0.7 for the gate operation. Such experimental capability is essential to a scheme for scalable quantum computation by means of the optical control of spin qubits in dots.
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http://dx.doi.org/10.1126/science.1083800 | DOI Listing |
Nano Lett
January 2025
Materials Science and Technology Division, Oak Ridge National Laboratory, 1 Bethel Valley Rd, Oak Ridge, Tennessee 37831, United States.
Thermally driven transitions between ferromagnetic and paramagnetic phases are characterized by critical behavior with divergent susceptibilities, long-range correlations, and spin dynamics that can span kHz to GHz scales as the material approaches the critical temperature , but it has proven technically challenging to probe the relevant length and time scales with most conventional measurement techniques. In this study, we employ scanning nitrogen-vacancy center based magnetometry and relaxometry to reveal the critical behavior of a high- ferromagnetic oxide near its Curie temperature. Cluster analysis of the measured temperature-dependent nanoscale magnetic textures points to a 3D universality class with a correlation length that diverges near .
View Article and Find Full Text PDFNano Lett
January 2025
Regensburg Center for Ultrafast Nanoscopy (RUN) and Department of Physics, University of Regensburg, 93040 Regensburg, Germany.
Detecting electromagnetic radiation scattered from a tip-sample junction has enabled overcoming the diffraction limit and started the flourishing field of polariton nanoimaging. However, most techniques only resolve amplitude and relative phase of the scattered radiation. Here, we utilize field-resolved detection of ultrashort scattered pulses to map the dynamics of surface polaritons in both space and time.
View Article and Find Full Text PDFPhotoacoustics
February 2025
Dipartimento di Scienze di Base ed Applicate per l'Ingegneria, Sapienza Università di Roma, Rome 00161, Italy.
A compact and robust optical excitation photoacoustic sensor with a self-integrated laser module excitation and an optimized differential resonator was developed to achieve high sensitivity and full linear range detection of carbon dioxide (CO) based on dual modes of wavelength modulated photoacoustic spectroscopy (WMPAS) and resonant frequency tracking (RFT). The integrated laser module equipped with three lasers (a quantum cascade laser (QCL), a distributed feedback laser (DFB) and a He-Ne laser) working in a time-division multiplexing mode was used as an integrated set of spectroscopic sources for detection of the designated concentration levels of CO. With the absorption photoacoustic mode, the WMPAS detection with the QCL and DFB sources was capable of CO detection at concentrations below 20 %, yielding a noise equivalent concentration (NEC) as low as 240 ppt and a normalized noise equivalent absorption coefficient (NNEA) of 4.
View Article and Find Full Text PDFSensors (Basel)
November 2024
Institute of Basic Operations Technology, China Telecom Research Institute, Beijing 102209, China.
In this paper, the theoretical model of spontaneous Raman scattering (SpRS) in few-mode fiber (FMF) is discussed. The influence of SpRS on quantum key distribution (QKD) in FMF is evaluated by combining wavelength division multiplexing (WDM) and space division multiplexing (SDM) techniques. On this basis, an improved ring-assisted FMF is designed and characterized; the transmission distance can be increased by up to 54.
View Article and Find Full Text PDFNanophotonics
November 2024
Universite Claude Bernard Lyon 1, CNRS, Institut Lumière Matière, UMR5306, F-69100, Villeurbanne, France.
In view of the recent increased interest in light-induced manipulation of magnetism in nanometric length scales this work presents metal clusters as promising elementary units for generating all-optical ultrafast magnetization. We perform a theoretical study of the opto-magnetic properties of metal clusters through ab-initio real-time (RT) simulations in real-space using time-dependent density functional theory (TDDFT). Through ab-initio calculations of plasmon excitation with circularly polarized laser pulse in atomically precise clusters of simple and noble metals, we discuss the generation of orbital magnetic moments due to the transfer of angular momentum from light field through optical absorption at resonance energies.
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