Development and performance of a low-background gamma-ray spectrometer are described. The spectrometer consists of a 131% efficient Ge detector in U-type configuration. The passive shielding consists of ultrapure lead of 6" thickness. A top muon guard is used as an active shielding. The spectrometer and shielding are positioned inside a steel room made of 6"-thick pre-World War II iron. The steel room is located underground with 33 m of water-equivalent overburden. The total integrated background rate in the energy range 50-2,700 keV was measured at 0.068 counts per second per 100 cm3 Ge volume. The spectrometer serves as a reference instrument for low-level and highly accurate environmental radioactivity measurements. One specific application of 228Ra determination in drinking water is described. With a 1 l water sample, 1-step chemical procedure, and 1,000 min counting time, a detection limit Ld = 20 mBq/l (0.55 pCi/l) was reached, which meets the EPA mandated limit of 1 pCi/l. Methods of upgrading the spectrometer as well as the predicted improvements in 228Ra detection, including direct counting of water without chemical processing, are discussed.
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http://dx.doi.org/10.1016/s0969-8043(02)00085-4 | DOI Listing |
Isotopes Environ Health Stud
January 2025
Research Institute of Biology, Yerevan State University, Yerevan, Republic of Armenia.
Plant test systems are a sensitive way to detect the genetic effects of various contaminants in environmental compartments: water, soil and sediments. Biotesting of the genotoxicity of soil samples with various activity concentrations of naturally occurring (Ra, Th, K) and artificial (Cs) radionuclides in soil, from the territory of the Aragats Massif (Armenia) was carried out with the application of the micronucleus (Trad-MСN) and stamen hair mutation (Trad-SHM) bioassays of (clone 02) model test-object in the soil - plant system. Undisturbed soil sampling was performed in the southern slopes of the Aragats Massif, from different altitudes (from 1000 to 3200 m above sea level).
View Article and Find Full Text PDFAnal Methods
January 2025
National Key Laboratory of Uranium Resources Exploration-Mining and Nuclear Remote Sensing, Beijing, 100029, China.
With the increasing demand for energy, nuclear energy has been developing rapidly. The quantitative detection and qualitative identification of uranium (U) are of great significance for the comprehensive and efficient use of U resources and the control of nuclear and radioactive substances. In this study, the detection of U is divided into liquid sample detection, solid sample detection, gas sample detection, and industrial detection from the perspectives of the sample state and detection environment.
View Article and Find Full Text PDFSci Total Environ
January 2025
Key Laboratory of Coastal Environment and Resources of Zhejiang Province, School of Engineering, Westlake University, Hangzhou 310024, China. Electronic address:
Saltmarshes serve as repositories for various metal species, primarily due to vegetation removal and mineralization processes. However, the significance of potassium (K), one of the three major nutrients (nitrogen, phosphorus, and K) essential for plant growth, has often been overlooked, particularly in the context of saltmarshes where the mechanisms of K transport via porewater exchange remain poorly understood. To address this knowledge gap, we conducted field observations and laboratory analysis, and developed a Rn mass balance model to quantify K fluxes via porewater exchange under physical, biological, and anthropogenic drivers.
View Article and Find Full Text PDFJ Environ Manage
January 2025
Research Group Environmental Economics, Centre of Environmental Sciences, Hasselt University, 3590, Diepenbeek, Belgium.
The use of industrial by-products as substitutes for raw materials in cement production not only reduces raw material use, thereby contributing to the circular economy, but also offers an avenue for reducing greenhouse gas emissions. This study investigates the perceptions of industry representatives and end-users across Belgium, Czechia and Slovenia regarding alternative cement made with industrial by-products categorised as naturally occurring radioactive materials. Based on 66 interviews, three main concerns were discerned: health, performance, and economic.
View Article and Find Full Text PDFSci Total Environ
January 2025
Biological and Environmental Sciences, Faculty of Natural Sciences, University of Stirling, Stirling FK9 4LA, United Kingdom.
Radioactive particles are physically discrete sources of radioactivity that have been released into the environment as result of past accidents, incidents, and practices, and can present a hazard to members of the public. The historical use of radium in the luminising of aircraft components, and the subsequent decommissioning of those aircraft and associated waste disposal practices, has left a legacy of contamination, such as the radioactive particles containing Ra-226 at Dalgety Bay, Scotland. The aim of this research was to physically, chemically, and radiologically characterise Ra-226 particles from Dalgety Bay and consider the implications for radiological protection of the public.
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