Coupled multipolar interactions in small-particle metallic clusters.

J Opt Soc Am A Opt Image Sci Vis

Department of Materials Science, University of Uppsala, The Angstrom Laboratory, Sweden,.

Published: March 2002

We propose a new formalism for computing the optical properties of small clusters of particles. It is a generalization of the coupled dipole-dipole particle-interaction model and allows one in principle to take into account all multipolar interactions in the long-wavelength limit. The method is illustrated by computations of the optical properties of N = 6 particle clusters for different multipolar approximations. We examine the effect of separation between particles and compare the optical spectra with the discrete-dipole approximation and the generalized Mie theory.

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http://dx.doi.org/10.1364/josaa.19.000513DOI Listing

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