We present a theory of the electron smectic fixed point of the stripe phases of doped layered Mott insulators. We show that in the presence of a spin gap three phases generally arise: (a) a smectic superconductor, (b) an insulating stripe crystal, and (c) a smectic metal. The latter phase is a stable two-dimensional anisotropic non-Fermi liquid. In the absence of a spin gap there is also a more conventional Fermi-liquid-like phase. The smectic superconductor and smectic metal phases (or glassy versions thereof) may have already been seen in Nd-doped La2-xSrxCuO4.
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http://dx.doi.org/10.1103/PhysRevLett.85.2160 | DOI Listing |
Rep Prog Phys
September 2024
Department of Physics and HK Institute of Quantum Science & Technology, The University of Hong Kong, Pokfulam Road, Hong Kong SAR, People's Republic of China.
Symmetry-breaking orders can not only compete with each other, but also be intertwined, and the intertwined topological and symmetry-breaking orders make the situation more intriguing. This work examines the archetypal correlated flat band model on a checkerboard lattice at fillingν=2/3and we find that the unique interplay between smectic charge order and topological order gives rise to two novel quantum states. As the interaction strength increases, the system first transitions from a Fermi liquid (FL) into FQAH smectic (FQAHS) state, where the topological order coexists cooperatively with smectic charge order with enlarged ground-state degeneracy and interestingly, the Hall conductivity isσxy=ν=2/3, different from the band-folding or doping scenarios.
View Article and Find Full Text PDFDalton Trans
May 2023
Department of Materials and Environmental Chemistry, Stockholm University, Svante Arrhenius väg 16C, SE-10691 Stockholm, Sweden.
Light-emitting materials based on earth-abundant metals, such as manganese hold great promise as emitters for organic lighting devices. In order to apply such emitter materials and, in particular, to overcome the problem of self-quenching due to cross-relaxation, we investigated a series of tetrabromidomanganate ([MnBr]) salts with bulky tetraalkylphosphonium counter cations [P], namely [P][MnBr] ( = 4 (1), 6 (2) and 8 (3)), which can be obtained by a straightforward reaction of the respective phosphonium bromide and MnBr. Variation of the cation size allows control of the properties of the resulting ionic materials.
View Article and Find Full Text PDFEur Phys J E Soft Matter
September 2022
Faculty of Advanced Technologies and Chemistry, Military University of Technology, ul. gen. Sylwestra Kaliskiego 2, 00-908, Warsaw, Poland.
The report shows the temperature behavior of the real part of dielectric permittivity in the static (dielectric constant) and low-frequency (LF) domains in bulk samples of 11CB and its BaTiO-based nanocolloids. The study covers the isotropic liquid (I), nematic (N), smectic A (SmA), and solid crystal (Cr) phases. For each phase, the dominance of pretransitional fluctuations, significantly moderated by nanoparticles, is shown.
View Article and Find Full Text PDFSoft Matter
June 2022
Sorbonne Université, CNRS, Institut des Nano-Sciences de Paris (INSP), F-75005 Paris, France.
New collective optical properties have emerged recently from organized and oriented arrays of closely packed semiconducting and metallic nanoparticles (NPs). However, it is still challenging to obtain NP assemblies which are similar everywhere on a given sample and, most importantly, share a unique common orientation that would guarantee a unique behavior everywhere on the sample. In this context, by combining optical microscopy, fluorescence microscopy and synchrotron-based grazing incidence X-ray scattering (GISAXS) of assemblies of gold nanospheres and of fluorescent nanorods, we study the interactions between NPs and liquid crystal smectic topological defects that can ultimately lead to unique NP orientations.
View Article and Find Full Text PDFChem Asian J
April 2022
State Key Laboratory for Mechanical Behaviour of Materials, Shaanxi International Research Center for Soft Matter, Xi'an Jiaotong University, Xi'an, 710049, P. R. China.
We report the formation of a 3D body-centred self-assembled superlattice of gold nanoparticles whose interparticle gap, and hence its plasmonic properties, are adjustable exclusively in the xy-plane. Thus, even though the particles are spherical, their anisotropic packing generates tailorable plasmonic dichroism. The gold nanoparticles are coated with forked ligands containing two mesogens: either two cholesterols ("twin"), one cholesterol and one azobenzene ("Janus"), or a mixture of the two.
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