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http://dx.doi.org/10.1103/PhysRevLett.75.2408 | DOI Listing |
Nat Commun
January 2025
Beijing Advanced Innovation Center for Materials Genome Engineering, Department of Physical Chemistry, University of Science and Technology Beijing, Beijing, China.
Electric field induced antiferroelectric-ferroelectric phase transition is a double-edged sword for energy storage properties, which not only offers a congenital superiority with substantial energy storage density but also poses significant challenges such as large polarization hysteresis and poor efficiency, deteriorating the operation and service life of capacitors. Here, entropy increase effect is utilized to simultaneously break the long-range antiferroelectric order and locally adjust the fourfold commensurate modulated polarization configuration, leading to a breakthrough in the trade-off between recoverable energy storge density (14.8 J cm) and efficiency (90.
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January 2025
Department of Physics and Astronomy, University of California, Riverside, CA, USA.
The floating phase, a critical incommensurate phase, has been theoretically predicted as a potential intermediate phase between crystalline ordered and disordered phases. In this study, we investigate the different quantum phases that arise in ladder arrays comprising up to 92 neutral-atom qubits and experimentally observe the emergence of the quantum floating phase. We analyze the site-resolved Rydberg state densities and the distribution of state occurrences.
View Article and Find Full Text PDFPhys Rev Lett
December 2024
School of Physics, Georgia Institute of Technology, Atlanta, Georgia 30332-0430, USA.
For moiré bilayer TMD superlattices, full-configuration-interaction (FCI) calculations are presented that take into account both the intra-moiré-quantum-dot (MQD) charge-carrier Coulombic interactions, as well as the crystal-field effect from the surrounding moiré pockets (inter-moiré-QD interactions). The effective computational embedding strategy introduced here allows for an FCI methodogy that enables the complete interpretation of the counterintuitive experimental observations reported recently in the context of moiré TMD superlattices at integer fillings ν=2 and 4. Two novel states of matter are reported: (i) a genuinely quantum-mechanical supercrystal of sliding Wigner molecules (WMs) for unstrained moiré TMD materials (when the crystal field is commensurate with the trilobal symmetry of the confining potential in each embedded MQD) and (ii) a supercrystal of pinned Wigner molecules when the crystal field is incommensurate with the trilobal symmetry or straining of the whole material is involved.
View Article and Find Full Text PDFNatl Sci Rev
December 2024
School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074, China.
Because of the lack of translational symmetry, calculating the energy spectrum of an incommensurate system has always been a theoretical challenge. Here, we propose a natural approach to generalize energy band theory to incommensurate systems without reliance on the commensurate approximation, thus providing a comprehensive energy spectrum theory of incommensurate systems. Except for a truncation-dependent weighting factor, the formulae of this theory are formally almost identical to that of Bloch electrons, making it particularly suitable for complex incommensurate structures.
View Article and Find Full Text PDFPhys Rev E
November 2024
Departamento de Química, Universidad Autónoma de Madrid, Cantoblanco, 28049 Madrid, Spain.
We study dynamical localization in an ultracold atom confined in an optical lattice that is simultaneously shaken by two competing pulsatile modulations with different amplitudes, periods, and waveforms. The effects of finite-width time pulses, modulation waveforms, and commensurable and incommensurable driving periods are investigated. We describe a particularly complex scenario and conclude that dynamical localization can survive, or even increase, when a periodic modulation is replaced by a quasiperiodic one of equal amplitude.
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