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Electron-Rich Heptacyclic S,N Heteroacene Enabling C-Shaped A-D-A-type Electron Acceptors With Photoelectric Response beyond 1000 Nm for Highly Sensitive Near-Infrared Photodetectors.
Adv Sci (Weinh)
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Department of Applied Chemistry, National Yang Ming Chiao Tung University, Hsinchu, 30010, Taiwan.
A highly electron-rich S,N heteroacene building block is developed and condensed with FIC and Cl-IC acceptors to furnish CT-F and CT-Cl, which exhibit near-infrared (NIR) absorption beyond 1000 nm. The C-shaped CT-F and CT-Cl self-assemble into a highly ordered 3D intermolecular packing network via multiple π-π interactions in the single crystal structures. The CT-F-based organic photovoltaic (OPV) achieved an impressive efficiency of 14.
View Article and Find Full Text PDFFormation of water-in-water emulsions and microgels in nonionic surfactant + gelatin aqueous mixtures.
J Colloid Interface Sci
January 2025
Institute of Advanced Chemistry of Catalonia (IQAC), Consejo Superior de Investigaciones Científicas (CSIC), Jordi Girona, 18-26, 08034 Barcelona, Spain; Networking Research Center on Bioengineering, Biomaterials and Nanomedicine (CIBER-BBN, ISCIII), Jordi Girona, 18-26, 08034 Barcelona, Spain. Electronic address:
Article Synopsis
- The study proposes that water-in-water (W/W) emulsions can be created by mixing a polymer and a surfactant, leading to phase segregation when the surfactant's cloud temperature is lowered.
- Experiments involved using an ethoxylated triglyceride surfactant (Kolliphor ELP) with gelatin, where the gelatin reduced the surfactant's cloud temperature, allowing for two distinct aqueous phases to form.
- The findings reveal that this is the first documented case of W/W emulsions formed with a polymer-surfactant mixture, achieving stability through chemically crosslinked microgels and the incorporation of mucin particles.
Temporally dissociable neural representations of pitch height and chroma.
J Neurosci
January 2025
Department of Psychology, Chinese University of Hong Kong, Hong Kong SAR, China
The extraction and analysis of pitch underpin speech and music recognition, sound segregation, and other auditory tasks. Perceptually, pitch can be represented as a helix composed of two factors: height monotonically aligns with frequency, while chroma cyclically repeats at doubled frequencies. Although the early perceptual and neurophysiological mechanisms for extracting pitch from acoustic signals have been extensively investigated, the equally essential subsequent stages that bridge to high-level auditory cognition remain less well understood.
View Article and Find Full Text PDF2D Titanium Carbide MXene-Interfaced Zinc Oxide/Tungstite Architectures Adorned Mixed Matrix Polymer Membranes for Oily Wastewater Treatment.
ACS Appl Mater Interfaces
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Department of Physics, National Institute of Technology Nagaland, Chumukedima, Dimapur 797103, India.
An exceedingly porous and interwoven fibrous structure was achieved in this study by interlocking titanium carbide (TiC) MXenes onto the electrospun mats using poly(vinylidene fluoride) (PVDF) as the base polymer. The fibrous membrane was further modified with the inclusion of zinc oxide (ZnO) and tungstite (WO·HO) nano/microstructures via annealing and hydrothermal approaches. Through these strategic interfaced morphological developments in novel TiC/ZnO/WO·HO heterostructures, our findings reveal enhanced wettability and charge-segregation desirable for promoting oil-water separation and photoreactivity, respectively.
View Article and Find Full Text PDF"Snakeskin" Bioinspired Design for Polymer Composite with Enhanced Positive Temperature-Dependent Thermal Conductivity.
Nano Lett
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Department of Forest Biomaterials, North Carolina State University, Raleigh, North Carolina 27607, United States.
Albeit there is widespread application of thermally conductive polymer composites, one challenge is their typical negative temperature dependence on thermal conductivity (TDTC) due to the mismatch in thermal expansion between the polymer and fillers, creating voids at the interfaces. Inspired by the hierarchical structure of snakeskin, where rigid scales and a soft intergap manage expansion, we designed a segregated structure by coating a high-expansion high impact polystyrene (HIPS)/graphite (Gt) composite with a copper alloy. We hypothesize that the Cu alloy restricts the thermal expansion of HIPS/Gt while forming a pseudoconductive network, enhancing TDTC and thermal conductivity (TC).
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