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Insights Into the Local Heating Effects in Triple-Cation Mixed-Halide Perovskite Cells: Charge Dynamics, Coherent Phonons, Anion Segregation.
Small
January 2025
Faculty of Physics and Astronomy, Adam Mickiewicz University, Poznan, 61-614, Poland.
The behavior of triple-cation mixed halide perovskite solar cells (PSCs) under ultrashort laser pulse irradiation at varying fluences is investigated, with a focus on local heating effects observed in femtosecond transient absorption (TA) studies. The carrier cooling time constant is found to increase from 230 fs at 2 µJ cm⁻ to 1.3 ps at 2 mJ cm⁻ while the charge population decay accelerates from tens of nanoseconds to the picosecond range within the same fluence range.
View Article and Find Full Text PDFAll-Optical Generation and Detection of Coherent Acoustic Vibrations in Single Gallium Phosphide Nanoantennas Probed near the Anapole Excitation.
Nano Lett
January 2025
Facultad de Ciencias Exactas y Naturales, Departamento de Física, Universidad de Buenos Aires, 1428 Buenos Aires, Argentina.
Nanostructured high-index dielectrics have shown great promise as low-loss photonic platforms for wavefront control and enhancing optical nonlinearities. However, their potential as optomechanical resonators has remained unexplored. In this work, we investigate the generation and detection of coherent acoustic phonons in individual crystalline gallium phosphide nanodisks on silica in a pump-probe configuration.
View Article and Find Full Text PDFPhotoinduced Fröhlich Interaction-Driven Distinct Electron- and Hole-Polaron Behaviors in Hybrid Organic-Inorganic Perovskites by Ultrafast Terahertz Probes.
ACS Nano
January 2025
School of Information Science and Technology and Department of Optical Science and Engineering and Key Laboratory of Micro and Nano Photonic Structures (MOE), Fudan University, Shanghai 200433, China.
The formation of large polarons resulting from the Fröhlich coupling of photogenerated carriers with the polarized crystal lattice is considered crucial in shaping the outstanding optoelectronic properties in hybrid organic-inorganic perovskite crystals. Until now, the initial polaron dynamics after photoexcitation have remained elusive in the hybrid perovskite system. Here, based on the terahertz time-domain spectroscopy and optical-pump terahertz probe, we access the nature of interplay between photoexcited unbound charge carriers and optical phonons in MAPbBr within the initial 5 ps after excitation and have demonstrated the simultaneous existence of both electron- and hole-polarons, together with the photogenerated carrier dynamic process.
View Article and Find Full Text PDFReal-Space Visualization of Canalized Ray Polaritons in a Single Van der Waals Thin Slab.
Nano Lett
January 2025
Department of Physics, University of Oviedo, Oviedo 33006, Spain.
Polaritons are central to the development of nanophotonics, as they provide mechanisms for manipulating light at the nanoscale. A key advancement has been the demonstration of polariton canalization in which the energy flow is directed along a single direction. An intriguing case is the canalization of ray polaritons, characterized by an enhanced density of optical states.
View Article and Find Full Text PDFEnhanced carrier mobility in strain-engineered PdAs monolayer boosted by suppressing interband scattering.
Phys Chem Chem Phys
January 2025
Institute of Applied Physics and Computational Mathematics, Beijing 100088, People's Republic of China.
Strain engineering is an effective method to modulate the electronic properties of two-dimensional materials. In this study, we theoretically studied the carrier mobility of the PdAs monolayer under different biaxial tensile strains based on the state-of-the-art electron-phonon coupling theory. We observe that the carrier mobility is largely enhanced for both n-type and p-type PdAs monolayers.
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