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Doping Tunable CDW Phase Transition in Bulk 1T-ZrSe.
Nano Lett
January 2025
Department of Quantum Matter Physics, University of Geneva, 24, Quai Ernest-Ansermet, 1211 Geneva 4, Switzerland.
Tunable electronic properties in transition metal dichalcogenides (TMDs) are essential to further their use in device applications. Here, we present a comprehensive scanning tunneling microscopy and spectroscopy study of a doping-induced charge density wave (CDW) in semiconducting bulk 1T-ZrSe. We find that atomic impurities that locally shift the Fermi level () into the conduction band trigger a CDW reconstruction concomitantly to the opening of a gap at .
View Article and Find Full Text PDFDirect Evidence of Anomalous Peierls Transition-Induced Charge Density Wave Order at Room Temperature in Metallic NaRu2O4.
Microsc Microanal
January 2025
Stuttgart Center for Electron Microscopy, Max Planck Institute for Solid State Research, Heisenbergstraße 1, Stuttgart 70569, Germany.
In the field of quantum materials, understanding anomalous behavior under charge degrees of freedom through bond formation is of fundamental importance, with two key concepts: Dimerization and charge order at different cation sites. The coexistence of both dimerization and charge ordering is unusually found in NaRu2O4, even in its metallic state at room temperature. Our work unveils the origin of the interplay of these effects within metallic single-crystalline NaRu2O4.
View Article and Find Full Text PDFThe inductive effect does not explain electron density in haloacetates: are our textbooks wrong?
Chem Sci
December 2024
College of Science, Engineering and Environment, University of Newcastle Callaghan NSW 2308 Australia.
The inductive effect is a central concept in chemistry and is often exemplified by the p values of acetic acid derivatives. The reduction in p is canonically attributed to the reduction in the electron density of the carboxylate group through the inductive effect. However, wave functional theory calculations presented herein reveal that the charge density of the carboxylate group is not explained by the inductive effect.
View Article and Find Full Text PDFProgrammable Electromagnetic Wave Absorption via Tailored Metal Single Atom-Support Interactions.
Adv Mater
January 2025
Laboratory of Advanced Materials, Institute of Optoelectronics, Fudan University, Shanghai, 200438, P. R. China.
Metal single atoms (SA)-support interactions inherently exhibit significant electrochemical activity, demonstrating potential in energy catalysis. However, leveraging these interactions to modulate electronic properties and extend application fields is a formidable challenge, demanding in-depth understanding and quantitative control of atomic-scale interactions. Herein, in situ, off-axis electron holography technique is utilized to directly visualize the interactions between SAs and the graphene surface.
View Article and Find Full Text PDFPossible Sliding Regimes in Twisted Bilayer WTe_{2}.
Phys Rev Lett
December 2024
Department of Physics, Stanford University, Stanford, California 94305, USA.
Inspired by the observation of increasingly one-dimensional (1D) behavior with decreasing temperature in small-angle twisted bilayers of WTe_{2} (tWTe_{2}), we theoretically explore the exotic sliding regimes that could be realized in tWTe_{2}. At zero displacement field, while hole-doped tWTe_{2} can be thought of as an array of weakly coupled conventional two-flavor 1D electron gases (1DEGs), the electron-doped regime is equivalent to coupled four-flavor 1DEGs, due to the presence of an additional "valley" degree of freedom. In the decoupled limit, the electron-doped system can thus realize phases with a range of interesting ordering tendencies, including 4k_{F} charge-density-wave and charge-4e superconductivity.
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