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Metal halide perovskites have unique luminescent properties that make them an attractive alternative for high quality light-emitting devices. However, the poor stability of perovskites with many defects and the long cycle time for the preparation of perovskite nanocomposites have hindered their production and application. Here, we prepared the perovskite mesostructures by embedding MAPbBr nanocrystals in the mesopores on the surface of silica nanospheres and mixing the nanospheres with silver nanowires and poly(methyl methacrylate) (PMMA), and further explored their optical properties.
View Article and Find Full Text PDFColloidal semiconductor quantum shells for solution-processed laser applications.
Nanoscale
January 2025
The Canter for Photochemical Sciences and Department of Physics, Bowling Green State University, Bowling Green, Ohio 43403, USA.
Laser diodes based on solution-processed semiconductor quantum dots (QDs) present an economical and color-tunable alternative to traditional epitaxial lasers. However, their efficiency is significantly limited by non-radiative Auger recombination, a process that increases lasing thresholds and diminishes device longevity through excessive heat generation. Recent advancements indicate that these limitations can be mitigated by employing spherical quantum wells, or quantum shells (QSs), in place of conventional QDs.
View Article and Find Full Text PDFMultiphoton and Harmonic Imaging of Microarchitected Materials.
ACS Appl Mater Interfaces
January 2025
Laser Thermal Laboratory, Department of Mechanical Engineering, University of California, Berkeley, California 94720, United States.
Article Synopsis
- Microadditive manufacturing enables the creation of intricate nano- and microscale components, leading to advancements in various industries.
- This research explores two-photon and three-photon fluorescence imaging, along with third-harmonic generation microscopy, to analyze complex lattice structures produced by multiphoton lithography.
- The study reveals that multiphoton fluorescence imaging provides better depth penetration and nondestructive identification of internal modifications and defects, improving quality control in microadditively manufactured products.
Radiative corrections: from medium to high energy experiments.
Eur Phys J A Hadron Nucl
April 2024
Institute of Nuclear Physics, Johannes Gutenberg-Universität, 55099 Mainz, Germany.
Radiative corrections are crucial for modern high-precision physics experiments, and are an area of active research in the experimental and theoretical community. Here we provide an overview of the state of the field of radiative corrections with a focus on several topics: lepton-proton scattering, QED corrections in deep-inelastic scattering, and in radiative light-hadron decays. Particular emphasis is placed on the two-photon exchange, believed to be responsible for the proton form-factor discrepancy, and associated Monte-Carlo codes.
View Article and Find Full Text PDFRational Molecular Design for Balanced Locally Excited and Charge- Transfer Nature for Two-Photon Absorption Phenomenon and Highly Efficient TADF-Based OLEDs.
Angew Chem Int Ed Engl
November 2024
Center for Organic Photonics and Electronics Research (OPERA) and Department of Applied Chemistry, Kyushu University, 744 Motooka, Nishi, Fukuoka, 819-0395, Japan.
The pursuit of highly efficient thermally activated delayed fluorescence (TADF) emitters with two-photon absorption (2PA) character is hampered by the concurrent achievement of a small singlet-triplet energy gap (ΔE) and high photoluminescence quantum yield (Φ). Here, by introducing a terephthalonitrile unit into a sterically crowded donor-π-donor structure, inducing a hybrid electronic excitation character, we designed unique TADF emitters possessing 2PA ability. This rational molecular design was achieved through a main π-conjugated donor-acceptor-donor backbone in line with locally excited feature renders a large oscillator strength and transition dipole moment, maintaining a high 2PA cross-section value.
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