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Autler-Townes splitting and linear dichroism in colloidal CdSe nanoplatelets driven by near-infrared pulses.
Sci Adv
October 2024
State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, Liaoning 116023, China.
Coherent interaction between light fields and matter has led to many exotic physical phenomena, one of which is the Autler-Townes splitting originating from the optical Stark effect of a three-level system. It has been well documented for atoms, molecules, and low-dimensional, epitaxial-grown semiconductors but rarely for solution-processed samples. Here, we report on Autler-Townes splitting observed in CdSe nanoplatelets.
View Article and Find Full Text PDFMid-Infrared Intersubband Cavity Polaritons in Flexible Single Quantum Well.
Nano Lett
April 2023
Department of Electrical Engineering, University at Buffalo, The State University of New York, Buffalo, New York 14260, United States.
Strong and ultrastrong coupling between intersubband transitions in quantum wells and cavity photons have been realized in mid-infrared and terahertz spectral regions. However, most previous works employed a large number of quantum wells on rigid substrates to achieve coupling strengths reaching the strong or ultrastrong coupling regime. In this work, we experimentally demonstrate ultrastrong coupling between the intersubband transition in a single quantum well and the resonant mode of photonic nanocavity at room temperature.
View Article and Find Full Text PDFDetection of Strong Light-Matter Interaction in a Single Nanocavity with a Thermal Transducer.
ACS Nano
December 2022
Centre de Nanosciences et de Nanotechnologies (C2N), CNRS UMR 9001, Université Paris-Saclay, 10 Boulevard Thomas Gobert, 91120Palaiseau, France.
The concept of strong light-matter coupling has been demonstrated in semiconductor structures, and it is poised to revolutionize the design and implementation of components, including solid state lasers and detectors. We demonstrate an original nanospectroscopy technique that permits the study of the light-matter interaction in single subwavelength-sized nanocavities where far-field spectroscopy is not possible using conventional techniques. We inserted a thin (∼150 nm) polymer layer with negligible absorption in the mid-infrared range (5 μm < λ < 12 μm) inside a metal-insulator-metal resonant cavity, where a photonic mode and the intersubband transition of a semiconductor quantum well are strongly coupled.
View Article and Find Full Text PDFAll-dielectric metasurfaces have recently led to a paradigm shift in nonlinear optics as they allow for circumventing the phase matching constraints of bulk crystals and offer high nonlinear conversion efficiencies when normalized by the light-matter interaction volume. Unlike bulk crystals, in all-dielectric metasurfaces nonlinear conversion efficiencies primarily rely on the material nonlinearity, field enhancements, and the modal overlaps, therefore most efforts to date have only focused on utilizing these degrees of freedom. In this work, we demonstrate that for second-harmonic generation in all-dielectric metasurfaces, an additional degree of freedom is the control of the polarity of the nonlinear susceptibility.
View Article and Find Full Text PDFObserving separate spin and charge Fermi seas in a strongly correlated one-dimensional conductor.
Sci Adv
June 2022
Department of Physics, Cavendish Laboratory, University of Cambridge, Cambridge CB3 0HE, UK.
An electron is usually considered to have only one form of kinetic energy, but could it have more, for its spin and charge, by exciting other electrons? In one dimension (1D), the physics of interacting electrons is captured well at low energies by the Tomonaga-Luttinger model, yet little has been observed experimentally beyond this linear regime. Here, we report on measurements of many-body modes in 1D gated wires using tunneling spectroscopy. We observe two parabolic dispersions, indicative of separate Fermi seas at high energies, associated with spin and charge excitations, together with the emergence of two additional 1D "replica" modes that strengthen with decreasing wire length.
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