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Sub-picosecond biphasic ultrafast all-optical switching in ultraviolet band.
Nanophotonics
November 2024
College of Physical Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, Xiamen University, Xiamen 361005, China.
Ultrafast all-optical control has been a subject of wide-spread attention as a method of manipulating optical fields using light excitation on extremely short time scales. As a fundamental form of ultrafast all-optical control, all-optical switching has achieved sub-picosecond switch speeds in the visible, infrared, and terahertz spectral regions. However, due to the lack of suitable materials, ultrafast all-optical control in the ultraviolet range remains in its early stages.
View Article and Find Full Text PDFSelf-hybridisation between interband transitions and Mie modes in dielectric nanoparticles.
Nanophotonics
June 2024
POLIMA-Center for Polariton-driven Light-Matter Interactions, University of Southern Denmark, Odense M, Denmark.
We discuss the possibility of self-hybridisation in high-index dielectric nanoparticles, where Mie modes of electric or magnetic type can couple to the interband transitions of the material, leading to spectral anticrossings. Starting with an idealised system described by moderately high constant permittivity with a narrow Lorentzian, in which self-hybridisation is visible for both plane-wave and electron-beam excitation, we embark on a quest for realistic systems where this effect should be visible. We explore a variety of spherical particles made of traditional semiconductors such as Si, GaAs, and GaP.
View Article and Find Full Text PDFMagnetic Field Tunable Polaritons in the Ultrastrong Coupling Regime in CrSBr.
ACS Nano
December 2024
Department of Physics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States.
Collective excitations of bound electron-hole pairs, i.e., excitons, are ubiquitous in condensed matter systems, and it has been shown that they can strongly couple to other degrees of freedom, such as spin, orbital, and lattice.
View Article and Find Full Text PDFInterferometric Near-field Fano Spectroscopy of Single Halide Perovskite Nanoparticles.
Nano Lett
December 2024
Institut für Physik, Carl von Ossietzky Universität, 26129 Oldenburg, Germany.
Semiconducting halide perovskite nanoparticles support Mie-type resonances that confine light on the nanoscale in localized modes with well-defined spatial field profiles yet unknown near-field dynamics. We introduce an interferometric scattering-type near-field microscopy technique to probe the local electric field dynamics at the surface of a single MAPbI nanoparticle. The amplitude and phase of the coherent light scattering from such modes are probed in a broad spectral range and with high spatial resolution.
View Article and Find Full Text PDFLight-dependent electron transfer mechanism on a Z-scheme MIL-100(Fe)/AgCl/Ag heterostructure for photocatalytic degradation.
J Colloid Interface Sci
February 2025
State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, Changchun 130012, PR China. Electronic address:
Article Synopsis
- The study investigates how different light sources affect the material properties and photocatalytic mechanisms, focusing on a new composite catalyst, MIL-100(Fe)/AgCl/Ag, for breaking down organic pollutants.
- Techniques like UV-visible spectroscopy and surface-enhanced Raman spectroscopy (SERS) were used to observe the degradation process in real-time, revealing that the catalyst works significantly better under visible light than under UV light.
- The enhanced efficiency under visible light (about 2.5 times higher) is linked to improved electron and hole separation via a mechanism called surface plasmon resonance (SPR), providing insights for developing better light-responsive catalysts in the future.
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