Submerge-emerge alternation promotes sediment per- and polyfluoroalkyl substance (PFAS) release and bioaccumulation.

Understanding the sediment release and plant bioaccumulation of per- and polyfluoroalkyl substances (PFASs) under submerge-emerge alternation (SE) is crucial to predicting their transport and fate in the riparian zones. In the present study, a simulational device was firstly constructed to explore the effects of SE on the transport of PFASs in riparian sediment-plant systems and the underlying mechanisms. The submerge (CS) and emerge (CE) situations were compared.

Responses and mechanisms of perfluoroalkyl acid release to the cumulative effects of propeller jet force over time.

As the discharge of exogenous perfluoroalkyl acids (PFAAs) is gradually controlled, the secondary release of endogenous PFAAs is poised to become a major challenge. However, the effects of complex hydrodynamic conditions, such as disturbance from ship propeller jets, on PFAA release, are still poorly understood. In the present study, a propeller jet disturbance simulation experiment was carried out using an indoor flume to investigate the responses and mechanisms of PFAA release to the cumulative effects of jet force over time.

Multi-compartment levels and distributions of per- and polyfluoroalkyl substances surrounding fluorochemical manufacturing parks in China: A review of the current literature.

Fluorochemical manufacturing parks (FMPs) are important point sources of per- and polyfluoroalkyl substances (PFASs) emissions to the surrounding environment. With legacy PFASs being phased-out and restricted in developed countries, China has emerged as one of the world's leading producers of PFASs. However, the occurrence and distribution patterns of PFASs emitted from FMPs in China remain poorly understood.

Eco-environmental responses of Eichhornia crassipes rhizobacteria community to co-stress of per(poly)fluoroalkyl substances and microplastics.

The stabilization of rhizobacteria communities plays a crucial role in sustaining healthy macrophyte growth. In light of increasing evidence of combined pollution from microplastics (MPs) and per- and polyfluoroalkyl substances (PFASs), Selecting typical floating macrophyte as a case, this study explored their impacts using hydroponic simulations and 16S rRNA high-throughput sequencing. A total of 31 phyla, 77 classes, 172 orders, 237 families, 332 genera, and 125 rhizobacteria species were identified.

Concentration-dependent cellular responses of coontail (Ceratophyllum demersum) during the substitutions to perfluorooctanoic acid by its two alternatives.

The substitutions of alternatives to legacy per- and polyfluoroalkyl substances (PFASs) may lead to unknown and variational joint toxicity on ecosystems. To comprehensively understand the effects of substitutions on aquatic ecosystems, the single and joint effects of perfluorooctanoic acid (PFOA) and its alternatives (perfluorobutanoic acid, PFBA; 2,3,3,3-tetrafluoro-2-(1,1,2,2,3,3,3,heptafluoropropoxy)propanoic acid, GenX) with various concentrations and compositions on a primary producer, coontail (Ceratophyllum demersum), were investigated at cellular level. Results showed that the substitutions of PFBA/GenX could alleviate the inhibition of PFOA on plant length, hydrogen peroxide accumulation, and chlorophyll b, due to the shifts of reactive oxygen species and their less toxicity to antioxidants.

Occurrence, risk assessment and source apportionment of perfluoroalkyl acids in the river of a hill-plain intersection region: The impacts of land use and river network structure.

Studying the impacts of land use and river network structure on perfluoroalkyl acids (PFAAs) footprint in rivers is crucial for predicting the fate of PFAAs in aquatic environments. This study investigated the distribution, ecological risks, sources and influence factors of 17 PFAAs in water and sediments of rivers from hills to plain areas. The results showed that the detection frequencies were higher for short-chain PFAAs than long-chain PFAAs in water, whereas an opposite pattern was found in sediments.

Characteristics of organic matter driven by Eichhornia crassipes during co-contamination with per(poly)fluoroalkyl substances (PFASs) and microplastics (MPs).

Co-contamination with MPs and PFASs has been recorded, particularly in surface-water environments. Floating macrophyte microcosms are an important part of the surface water ecosystem, and dissolved organic matter (DOM) driven by floating macrophytes (FMDDOM) is critical for maintaining material circulation. However, knowledge gaps remain regarding the impact of MPs and PFASs co-pollution on FMDDOM.

Human activities exacerbate river network degrading in the Qinhuai River basin.

Rivers are undergoing significant changes under the pressures of natural processes and human activities. However, characterizing and understanding these changes over the long term and from a spatial perspective have proven challenging. This paper presents a novel framework featuring twelve indicators that combine geometric and spatial structures for evaluating changes in river network patterns.

A novel longitudinal connectivity index to evaluate reticular river networks based on the combination of network maximum flow and resistance distance.

Reticular river networks, essential for ecosystems and hydrology, pose challenges in assessing longitudinal connectivity due to complex multi-path structures and variable flows, exacerbated by human-made infrastructures like sluices. Existing tools inadequately track water flow's spatiotemporal changes, highlighting the need for targeted methods to gauge connectivity within complex river network systems. The Hydraulic Capacity Connectivity Index (HCCI) was developed adopting complex network theory.

Release of perfluoroalkyl acids from sediments under the effects of the discharge ratio and flow flux at a Y-shaped confluence.

The sediments in riverine environments contain notably high concentrations of perfluoroalkyl acids (PFAAs), which may be released into the water body under different hydrodynamic forces, such as those occurring at Y-shaped confluences. The release of PFAAs may pose a significant risk to the surrounding aquatic ecosystems. However, our understanding of the release and transport of PFAAs from sediments at Y-shaped confluences remains unclear.

Intense Turbulent Bursts Promote the Release of Perfluoroalkyl Acids from Sediments at High Flow Velocity.

Despite frequent detection of high levels of perfluoroalkyl acids (PFAAs) in sediments, research on the environmental fate of PFAAs in sediments, particularly under hydrodynamic conditions, is rather limited, challenging effective management of PFAA loadings. Therefore, this study investigated the release and transport of 15 PFAAs in sediments under environmentally relevant flow velocities using recirculating flumes and revealed the underlying release mechanisms by identifying related momentum transfer. An increased velocity enhanced the release magnitude of total PFAAs by a factor of 3.

The bioaccumulation and ecotoxicity of co-exposure of per(poly)fluoroalkyl substances and polystyrene microplastics to Eichhornia crassipes.

Gen X and F-53B have been popularized as alternatives to PFOA and PFOS, respectively. These per(poly)fluoroalkyl substances pervasively coexist with microplastics (MPs) in aquatic environments. However, there are knowledge gaps regarding their potential eco-environmental risks.

Effects of long-chained perfluoroalkyl acids (PFAAs) on the uptake and bioaccumulation of short-chained PFAAs in two free-floating macrophytes: Eichhornia crassipes and Ceratophyllum demersum.

Short-chained perfluoroalkyl acids (PFAAs, CF-R, n ≤ 6) have merged as global concerns due to their extensive application and considerable toxicity. However, long-chained PFAAs (n ≥ 7) featured with high persistence are still ubiquitously observed in aquatic environment. To understand the uptake behavior of short-chained PFAAs in aquatic macrophytes, the uptake kinetics, bioconcentration, and translocation of short-chained PFAAs (3 ≤n ≤ 6) in two typical free-floating macrophytes (Eichhornia crassipes and Ceratophyllum demersum) were investigated in the treatments with and without long-chained PFAAs (7 ≤n ≤ 11).

Dynamics of antibiotic resistance genes in the sediments of a water-diversion lake and its human exposure risk behaviour.

The dynamics and exposure risk behaviours of antibiotic resistance genes (ARGs) in the sediments of water-diversion lakes remain poorly understood. In this study, spatiotemporal investigations of ARG profiles in sediments targeting non-water (NWDP) and water diversion periods (WDP) were conducted in Luoma Lake, a typical water-diversion lake, and an innovative dynamics-based risk assessment framework was constructed to evaluate ARG exposure risks to local residents. ARGs in sediments were significantly more abundant in the WDP than in the NWDP, but there was no significant variation in their spatial distribution in either period.

Field study on endogenous perfluoroalkyl acid release and their spatiotemporal distribution processes induced by inland navigation.

Dense populations and industries in regions with developed inland waterways have caused the significant discharge of perfluoroalkyl acids (PFAAs) into surrounding waterways. Despite being the dominant energy input in the waterways, the impact of ship navigation on endogenous PFAA release is unclear. In this study, a field experiment was carried out in the Wangyu River (Taihu Basin, China) to investigate the spatiotemporal distribution processes of PFAAs in the water column after passage of ships with different tonnages, speeds, and draughts.

Iron-Nitrogen Amendment Reduced Perfluoroalkyl Acids' Phyto-Uptake in the Wheat-Soil Ecosystem: Contributions of Dissolved Organic Matters in Soil Solution and Root Extracellular Polymeric Substances.

Understanding the mechanisms underlying perfluoroalkyl acids (PFAAs) translocation, distribution, and accumulation in wheat-soil ecosystems is essential for agricultural soil pollution control and crop ecological risk assessment. This study systematically investigated the translocation of 13 PFAAs under different iron and nitrogen fertilization conditions in a wheat-soil ecosystem. Short-chain PFAAs including PFBA, PFPeA, PFHxA, and PFBS mostly accumulated in soil solution (10.

Spatio-temporal distribution and dynamics of antibiotic resistance genes in a water-diversion lake, China.

The distribution and dynamics of antibiotic resistance genes (ARGs) in water-diversion lakes are poorly understood. In this study, two comparative in situ investigations of ARG profiles targeting water diversion (DP) and non-diversion periods (NDP) were conducted in Luoma Lake, a vital transfer node for the eastern route of the South-to-North Water Diversion Project in China. The results demonstrated significant spatiotemporal variations in ARG contamination and notable differences in the co-occurrence patterns of ARGs and bacterial communities between DP and NDP.

Global development and future trends of artificial sweetener research based on bibliometrics.

Artificial sweeteners have sparked a heated debate worldwide due to their ambiguous impacts on public and environmental health and food safety and quality. Many studies on artificial sweeteners have been conducted; however, none scientometric studies exist in the field. This study aimed to elaborate on the knowledge creation and development of the field of artificial sweeteners and predict the frontiers of knowledge based on bibliometrics.

Mechanisms of propeller jet-induced migration, release, and distribution of perfluoroalkyl acids in sediment-water systems.

Perfluoroalkyl acids (PFAAs) are continuously accumulated in surface sediments due to extensive and long-term application. However, the mechanisms through which disturbances induced by ship propeller jets at the riverbed cause secondary release of PFAAs from sediments remain unclear. In this study, the effects of different propeller rotational speeds on PFAA migration, release, and distribution in multiphase media were investigated by performing indoor flume experiments combined with particle tracking velocimetry.

The addition of iron-carbon enhances the removal of perfluoroalkyl acids (PFAAs) in constructed wetlands.

Hazardous perfluoroalkyl acids (PFAAs), particularly perfluorooctane sulfonate (PFOS) and perfluorooctanoate (PFOA), have become ubiquitous environmental persistent organic contaminants, posing serious threats to environmental health, which has led to the development of PFAA treatment methods. Wetland construction in combination with iron-carbon (CW-I), a low-maintenance and high-efficiency technology, may be capable of removing PFAAs through physico-biochemical processes. In this study, we aim to investigate the removal efficiency of PFAAs by CW-I as well as the critical functions of all components within the wetlands.

Effects of Escherichia pollution and salinity on nutrient levels in submerged vegetated wetlands: Insights into benthic community stability and metabolisms.

Inner coastal wetland ecosystems are generally eutrophic and are often exposed to both salinity stress and Escherichia coli pollution. However, the effects of these stressors on nutrient-cycling and microbial communities are under-researched. Here, we established a vegetated wetland ecosystem in a saline environment to understand the effects of E.

Nitrogen addition enhanced Per-fluoroalkyl substances' microbial availability in a wheat soil ecosystem.

Per-fluoroalkyl substances (PFASs) have been widely detected in farmland soils and are understood to pose toxicological threats to soil microbiomes and crop safety. Meanwhile, farmland ecosystems have experienced increasing nitrogen loading caused by soil fertilization. Yet it is still unclear how nitrogen additions affect soil's microbial responses to PFASs.

Insights into effects of discharge ratio on flow characteristics and pollutant transport in a Y-shaped open channel confluence with emergent rigid vegetation.

Turbulence generated within the vegetated confluence system is important for water quality and river management. In this study, we conducted a series of experiments to explore the extent to which emergent rigid vegetation in the confluence channel influences hydrodynamic characteristics and contaminant transport. First, a series of tests with increasing discharge ratios (from 0.