The rapid growth of flexible quasi-solid-state thermocells (TECs) provides a fresh way forward for wearable electronics. However, their insufficient mechanical strength and power output still hinder their further applications. This work demonstrates a one-stone-two-birds strategy to synergistically enhance the mechanical and thermoelectrochemical properties of the [Fe(CN)]-based TECs.
View Article and Find Full Text PDFThe evolution of wearable technology has prompted the need for adaptive, self-healable, and energy-autonomous energy devices. This study innovatively addresses this challenge by introducing an MXene-boosted hydrogel electrolyte, which expedites the assembly process of flexible thermocell (TEC) arrays and thus circumvents the complicated fabrication of typical wearable electronics. Our findings underscore the hydrogel electrolyte's superior thermoelectrochemical performance under substantial deformations and repeated self-healing cycles.
View Article and Find Full Text PDFMeasurements of vertical distribution of volatile organic compounds (VOCs) have attracted wide attentions, which could help to understand atmospheric oxidation mechanism and provide implications for VOC control. This study measured the non-methane hydrocarbons (NMHCs) and oxygenated VOCs (OVOCs) simultaneously for the first time at three different heights, namely ground, 118 m and 488 m, in the Canton Tower located in the urban core of the Pearl River Delta (PRD). The results show that NMHCs decreased while some OVOC species such as formaldehyde and acetaldehyde increased with increasing height.
View Article and Find Full Text PDFThe increase of surface ozone during the Corona Virus Disease 2019 (COVID-19) lockdown in China has aroused great concern. In this study, we combine 1.5 years of measurements for ozone, volatile organic compounds (VOCs), and nitrogen oxide (NO) at four sites to investigate the effect of COVID-19 lockdown on surface ozone in Dongguan, an industrial city in southern China.
View Article and Find Full Text PDFIn recent decade the ambient fine particle (PM) levels have shown a trend of distinct dropping in China, while ground-level ozone concentrations have been increasing in Beijing and many other Chinese mega-cities. The variation pattern in Los Angeles was markedly different, with PM and ozone decreasing together over past decades. In this study, we utilize observation-based methods to establish the parametric relationship between PM concentration and key aerosol physical properties (including aerosol optical depth and aerosol surface concentration), and an observation-based 1-D photochemical model to quantify the response of PM decline in enhancing ground-level ozone pollution over a large PM concentration range (10-120 μg m).
View Article and Find Full Text PDFSolvent use and paint consumption are significant source sectors of volatile organic compounds (VOCs) emissions in China. The occupational painters have high risk of health effect due to exposure to high VOCs concentration. However, the toxic components in coating environment have not been carefully identified, and the health risks of VOCs exposure have not been sufficiently assessed.
View Article and Find Full Text PDFAccurate estimation of speciated emissions of volatile organic compounds (VOCs) is challenging due to the complexity of both species and sources. Evaluation of the bottom-up emission inventory (EI) by atmospheric observation is needed to better understand the VOC emissions and then to control air pollutions caused by VOCs. This study conducts vertical measurements of VOCs between November 3 and 11, 2018 at the Canton Tower in the urban core of Pearl River Delta (PRD), China.
View Article and Find Full Text PDFApart from the aerodynamic performance (efficiency and safety), the wake after an on-road vehicle substantially influences the tailpipe pollutant dispersion (environment). Remote sensing is the most practicable measures for large-scale emission control. Its reliability, however, is largely dictated by how well the complicated vehicular flows and instrumentation constraint are tackled.
View Article and Find Full Text PDFThis study employs a mass balance technique-box model to calculate the biogenic isoprene emissions based on the ground-level measurements between October 2009 and September 2010 in Beijing. The annual magnitude, monthly variations and diurnal patterns of isoprene emissions are estimated. The annual emissions of isoprene were estimated to be 23.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
October 2018
Development and trend of global wind tunnel research from 1991 to 2014 were evaluated by bibliometric analysis. Based on the statistical data from Science Citation Index Expanded from Web of Science, publication performance of wind tunnel research was analyzed from various aspects, including publication output, category distributions, journals, countries, institutions, leading articles, and words analysis. The results show that scientific articles associated with wind tunnel increased dramatically, with Journal of Wind Engineering and Industrial Aerodynamics as the most productive journal.
View Article and Find Full Text PDFEnviron Sci Pollut Res Int
June 2018
Wind tunnels have been widely employed in aerodynamic research. To characterize the high impact research, a bibliometric analysis was conducted on highly cited articles related to wind tunnel based on the Science Citation Index Expanded (SCI-EXPANDED) database from 1900 to 2014. Articles with at least 100 citations from the Web of Science Core Collection were selected and analyzed in terms of publication years, authors, institutions, countries/territories, journals, Web of Science categories, and citation life cycles.
View Article and Find Full Text PDFThis study provides a top-down approach to establish an emission inventory of volatile organic compounds (VOC) based on ambient measurements, by combining the box model and positive matrix factorization (PMF) model. Species-specified VOC emissions, source contributions, and spatial distributions are determined based on regional-scale gridded measurements between September 2008 to December 2009 in the Pearl River Delta (PRD), China. The most prevalent anthropogenic species in the PRD was toluene estimated by the box model to be annual emissions of 167.
View Article and Find Full Text PDFNingbo is a highly industrialized city in the coastal area of the Yangtze River Delta (YRD), China. Large emissions and transport of non-methane hydrocarbons (NMHCs) may contribute to regional ozone (O) and particulate matter (PM) pollution; however, the concentrations and sources of ambient NMHCs have not yet been investigated in Ningbo. In this study, ambient NMHCs were measured at two residential (SZ and CX) and two industrial (ZH and BL) sites and one suburban (XS) site over ten consecutive days in each season (10-20 December 2012 in winter, 14-23 April 2013 in spring, 15-24 July 2013 in summer, 22-31 October 2013, in autumn).
View Article and Find Full Text PDFUnderstanding the volatile organic compounds (VOCs) emission characteristics from solvent usage industry is essential to reduce PM2.5 and O3 in Yangtze River Delta region. In this work, VOCs source characteristics of ship container, shipbuilding, wood, and automobile painting industry were measured using canister-GC-MS/FID analysis system.
View Article and Find Full Text PDFProcess-specific emission characteristics of volatile organic compounds (VOCs) from petrochemical facilities were investigated in the Yangtze River Delta, China. Source samples were collected from various process units in the petrochemical, basic chemical, and chlorinated chemical plants, and were measured using gas chromatography-mass spectrometry/flame ionization detection. The results showed that propane (19.
View Article and Find Full Text PDFIndustrial sector-based VOC source profiles are reported for the Pearl River Delta (PRD) region, China, based source samples (stack emissions and fugitive emissions) analyzed from sources operating under normal conditions. The industrial sectors considered are printing (letterpress, offset and gravure printing processes), wood furniture coating, shoemaking, paint manufacturing and metal surface coating. More than 250 VOC species were detected following US EPA methods TO-14 and TO-15.
View Article and Find Full Text PDFSci Total Environ
December 2011
A 3 km × 3 km gridded mercury emission inventory in the Pearl River Delta (PRD) region for 2008 was compiled from the best available emission factors and official statistical data. The inventory presented a comprehensive estimation of anthropogenic mercury sources and roughly estimated the emissions from natural sources. The total mercury emissions in the PRD region for the year of 2008 are estimated to be 17,244 kg, of which 85% released as Hg(0), 11% as Hg(2+), and 4% as Hg(P).
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