The active site is a highly anticipated property of adsorbent in the field of separation, as it enables a concurrent enhancement of both adsorption efficiency and adsorption rate. Herein, employing morphology-oriented regulation, we successfully fabricated heterogeneous MgO adsorbent from a magnesium-based metal-organic framework (MOF) precursor, octahedral MgO-M and laminated sheets MgO-P, for the capture of Congo red (CR). Specifically, the octahedron MgO-M exhibits a greater abundant of moderately and strongly alkaline sites, which facilitate the adsorption of CR.
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