Publications by authors named "Zhipeng Xuan"

Understanding the nature of photogenerated carriers and their subsequent dynamics in semiconducting perovskites is important for the development of solar cell materials and devices. However, most ultrafast dynamic measurements on perovskite materials were conducted under high carrier densities, which likely obscures the genuine dynamics under low carrier densities in solar illumination conditions. In this study, we presented a detailed experimental study of the carrier density-dependent dynamics in hybrid lead iodide perovskites from femtosecond to microsecond using a highly sensitive transient absorption (TA) spectrometer.

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In recent years, perovskite solar cells (PSCs) have experienced rapid development and have presented an excellent commercial prospect as the PSCs are made from raw materials that are readily and cheaply available depending on simple manufacturing techniques. However, the commercial production and utilization of PSCs remain immature, leading to substantial efforts needed to boost the development of scalable fabrication of PSCs, pilot scale tests, and the establishment of industrial production lines. In this way, the PSCs are expected to be successfully popularized from the laboratory to the photovoltaic market.

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Perovskite solar cells have exhibited astonishing photoelectric conversion efficiency and have shown a promising future owing to the tunable content and outstanding optoelectrical property of hybrid perovskite. However, the devices with planar architecture still suffer from huge loss and severe hysteresis effect. In this research, Guanidine hydrobromide (GABr) post-treatment is carried out to enhance the performance of MAPbI n-i-p planar perovskite solar cells.

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Article Synopsis
  • Interface engineering is crucial for improving the efficiency of perovskite solar cells (PSCs), specifically by enhancing the electron mobility and charge transfer in the tin oxide (SnO) electron transport layer (ETL) using a two-dimensional material called MXene.
  • The incorporation of MXene not only improves the performance of the SnO ETL but also creates a better growth environment for perovskite films, leading to lower trap density and reduced charge transport losses.
  • This innovative approach results in PSCs that achieve an efficiency of 20.65%, with significantly reduced non-radiative recombination and minimal hysteresis, demonstrating the potential for more efficient solar energy solutions.
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