Pelletization of biomass fuels has been promoted as an effective alternative to mitigate particulate matter (PM) emissions from the residential burning of raw biomass materials; however, environmentally persistent free radicals (EPFRs), a class of harmful components in PM, from the biomass pellet burning have been rarely studied yet. Here, laboratory-based combustion experiments were conducted to characterize EPFRs for different pellets burned in cooking and heating stoves and compared with those for the corresponding uncompressed biofuels. Emission factors (EFs) of EPFRs for biomass pellets ranged from 2.
View Article and Find Full Text PDFEnviron Sci Ecotechnol
January 2025
Extensive use of traditional solid fuels necessitates a clean transition to modern energy, yet rising costs hinder equitable progress, presenting a challenge that remains underexplored. Here we quantify household energy inequities in China and evaluate shifts during the cooking and heating transition by compiling data from nationwide questionnaire surveys and statistic datasets. We find that by meeting 42.
View Article and Find Full Text PDFSevere indoor air pollution from solid-fuel combustion is a global health concern. Although stove chimneys can expel most of the smoke to outside, unignorable amounts can remain indoors, known as indoor fugitive emissions. Quantitative analyses of indoor emission rates (IER) and indoor fugitive fractions (IFF) are limited, particularly in field settings.
View Article and Find Full Text PDFRising environmental concerns associated with the domestic use of solid biofuels have driven the search for clean energy alternatives. This study investigated the toxicological characteristics of PM emissions from residential biomass pellet burning using the A549 epithelial cell line. The potential of modern pellet applications to reduce PM emissions was evaluated by considering both mass reduction and toxicity modification.
View Article and Find Full Text PDFUniversal access to clean fuels in household use is one explicit indicator of sustainable development while currently still billions of people rely on solid fuels for daily cooking. Despite of the recognized clean transition trend in general, disparities in household energy mix in different activities (e.g.
View Article and Find Full Text PDFStyphnolobium japonicum (L.) Schott (family Fabaceae Juss.) also called pagoda tree, is widely planted in northern China in landscape plantings, for erosion control and forestry.
View Article and Find Full Text PDFEnviron Geochem Health
November 2023
Polycyclic aromatic hydrocarbons (PAHs) are widespread environmental contaminants associated with various health risks including lung cancer. Indoor exposure to PAHs, particularly from the indoor burning of fuels, is significant; however, long-term large-scale assessments of indoor PAHs are hampered by high costs and time-consuming in field sampling and laboratory experiments. A simple fuel-based approach and statistical regression models were developed as a trial to predict indoor BaP, as a typical PAH, in China, and consequently spatiotemporal variations in indoor BaP and indoor exposure contributions were discussed.
View Article and Find Full Text PDFThe Qinghai-Tibetan Plateau (QTP) and its surrounding areas are undergoing rapid changes in socioeconomic conditions, activity sectors, and emission levels. These changes underscore the significance of conducting local environmental assessments in the future and generating air pollutant emission forecasts necessary for effective evaluation. Current pollutants emissions pathways exhibit regional limitation since their based historical inventory could not accurately reflect the emission characteristics in QTP.
View Article and Find Full Text PDFEnvironmental persistent free radicals (EPFRs) are receiving growing concerns owing to their potentially adverse impacts on human health. Road dust is one important source of air pollution in most cities and may pose significant health risks. Characteristics of EPFRs in urban road dusts and its formation mechanism(s) are still rarely studied.
View Article and Find Full Text PDFSolid fuel use (SFU) is common in most developing countries and would release many hazardous air pollutants posing high risks on human health. The Global Burden of Disease (GBD) study highlighted risks associated with household SFU in Pakistan, however, high uncertainties prevail because of scanty data on SFU and unaccounted energy stacking. This study conducted a field campaign aiming at collecting first-hand data on household energy mix in Pakistan.
View Article and Find Full Text PDFResidential emissions significantly contribute to air pollution. To address this issue, a clean heating campaign was implemented to replace coal with electricity or natural gas among 13.9 million rural households in northern China.
View Article and Find Full Text PDFEnviron Sci Technol
November 2023
Household air pollution associated with solid fuel use is a long-standing public concern. The global population mainly using solid fuels for cooking remains large. Besides cooking, large amounts of coal and biomass fuels are burned for space heating during cold seasons in many regions.
View Article and Find Full Text PDFThe society has high concerns on the inequality that people are disproportionately exposed to ambient air pollution, but with more time spent indoors, the disparity in the total exposure considering both indoor and outdoor exposure has not been explored; and with the socioeconomical development and efforts in fighting against air pollution, it is unknown how the exposure inequality changed over time. Based on the city-level panel data, this study revealed the Concentration Index (C) in ambient PM exposure inequality was positive, indicating the low-income group exposed to lower ambient PM; however, the total PM exposure was negatively correlated with the income, showing a negative C value. The low-income population exposed to high PM associated with larger contributions of indoor exposure from the residential emissions.
View Article and Find Full Text PDFNitroaromatic compounds (NACs) not only are strongly absorbing chromophores but also adversely affect human health. NACs can be emitted from incomplete combustions and can derive secondarily through photochemical reactions. Here, emission experiments were conducted for 31 fuel-stove combinations to elucidate variations in, and influencing factors of, NAC emission factors (EF) and to explore potential tracers for different combustion sources.
View Article and Find Full Text PDFThe household energy mix has significant impacts on human health and climate, as it contributes greatly to many health- and climate-relevant air pollutants. Compared to the well-established urban energy statistical system, the rural household energy statistical system is incomplete and is often associated with high biases. Via a nationwide investigation, this study revealed high contributions to energy supply from coal and biomass fuels in the rural household energy sector, while electricity comprised ∼20%.
View Article and Find Full Text PDFAmbient PM (fine particulate matter with aerodynamic diameters ≤ 2.5 μm) is thought to be associated with the development of diabetes, but few studies traced the effects of PM components and pollution sources on the change in the fasting blood glucose (FBG). In the present study, we assessed the associations of PM constituents and their sources with the FBG in a general Chinese population aged over 40 years.
View Article and Find Full Text PDFInt J Environ Res Public Health
April 2022
Ultrafine particles (UFPs) significantly affect human health and climate. UFPs can be produced largely from the incomplete burning of solid fuels in stoves; however, indoor UFPs are less studied compared to outdoor UFPs, especially in coal-combustion homes. In this study, indoor and outdoor UFP concentrations were measured simultaneously by using a portable instrument, and internal and outdoor source contributions to indoor UFPs were estimated using a statistical approach based on highly temporally resolved data.
View Article and Find Full Text PDFEnergy is vital to human society but significantly contributes to the deterioration of environmental quality and the global issue of climate change. Biomass and fossil fuels are important energy sources but have distinct pollutant emission characteristics during the burning process. This study aimed at attributing radiative forcing of climate forcers, including greenhouse gases but also short-lived climate pollutants, from the burning of fossil and biomass fuels, and the spatiotemporal characteristics.
View Article and Find Full Text PDFExposure to household air pollution (HAP) from solid fuel use (SFU) causes millions of premature deaths globally. Direct leakage from stoves into indoor air is believed to be the main cause of severe HAP. However, previous laboratory-based measurements reported leakage of minimal fractions from wood fuel combustion.
View Article and Find Full Text PDFA large population does not have access to modern household energy and relies on solid fuels such as coal and biomass fuels. Burning of these solid fuels in low-efficiency home stoves produces high amounts of multiple air pollutants, causing severe air pollution and adverse health outcomes. In evaluating impacts on human health and climate, it is critical to understand the formation and emission processes of air pollutants from these combustion sources.
View Article and Find Full Text PDFBlack carbon (BC) emissions, derived primarily from incomplete fuel combustion, significantly affect the global and regional climate. Mass absorption efficiency (MAE) is one important parameter in evaluating the climate impacts of BC. Here, values and variabilities in the MAE of BC (MAE) from real-world residential emissions were investigated from a field campaign covering 163 burning events for different fuel-stove combinations.
View Article and Find Full Text PDFIndoor air quality is critically important to the human as people spend most time indoors. Indoor PM is related to the outdoor levels, but more directly influenced by internal sources. Severe household air pollution from solid fuel use has been recognized as one major risk for human health especailly in rural area, however, the issue is significantly overlooked in most national air quality controls and intervention policies.
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