Publications by authors named "Zhensen Zheng"

Aircraft observations have revealed ubiquitous new particle formation in the tropical upper troposphere over the Amazon and the Atlantic and Pacific oceans. Although the vapours involved remain unknown, recent satellite observations have revealed surprisingly high night-time isoprene mixing ratios of up to 1 part per billion by volume (ppbv) in the tropical upper troposphere. Here, in experiments performed with the CERN CLOUD (Cosmics Leaving Outdoor Droplets) chamber, we report new particle formation initiated by the reaction of hydroxyl radicals with isoprene at upper-tropospheric temperatures of -30 °C and -50 °C.

View Article and Find Full Text PDF

Black carbon (BC) aerosol can lead to adverse health effects and drive climate change; therefore, the characteristic research and identification of BC sources are essential for lowering emissions. In this study, equivalent black carbon (eBC) measurement was performed using a seven-wavelength Aethalometer (AE33) at an urban site in a typical industrial city (Zibo) of Northern China for the first time. The monitoring was performed from February 2021 to January 2022.

View Article and Find Full Text PDF

During summer, ammonia emissions in Southeast Asia influence air pollution and cloud formation. Convective transport by the South Asian monsoon carries these pollutant air masses into the upper troposphere and lower stratosphere (UTLS), where they accumulate under anticyclonic flow conditions. This air mass accumulation is thought to contribute to particle formation and the development of the Asian Tropopause Aerosol Layer (ATAL).

View Article and Find Full Text PDF

Volatile organic compounds (VOCs) are consumed by photochemical reactions during transport, leading to inaccuracies in estimating the local ozone (O) formation mechanism and its subsequent strategy for O attainment. To comprehensively quantify the deviations in O formation mechanism by consumed VOCs (C-VOCs), a 5-month field campaign was conducted in a typical industrial city in Northern China over incorporating a 0-D box model (implemented with MCMv3.3.

View Article and Find Full Text PDF

To explore the formation mechanism of the ozone (O) and emission reduction strategy in a northwestern city, an extensive field campaign was conducted in summertime in 2021 in Yining City, in which the 0-D box model incorporating the latest explicit chemical mechanism (MCMv3.3.1) was applied for the first time to quantify the O-NO-VOCs sensitivity and formulate a precise O control strategy in this city.

View Article and Find Full Text PDF

Black carbon (BC) significantly affects climate, environmental quality, and human health. This study utilised Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), which can compensate for the shortcomings of ground BC monitoring in spatial-temporal distribution to study the pollution characteristics of BC and potential pollution sources in a typical industrial city (Xinxiang) with serious air pollution in northern China. The results showed that average daily ground observation and MERRA-2 concentration of BC of 7.

View Article and Find Full Text PDF

To investigate the characteristics and formation mechanism of ozone (O) pollution in an industrial city, an extensive one-month field campaign focusing on O and its precursors (e.g., volatile organic compounds[VOC] and nitrogen oxides[NO]) was conducted in Zibo City, a highly industrializd city in the North China Plain, in June 2021.

View Article and Find Full Text PDF

Quantifying the impact of carbonyl compounds (carbonyls) on ozone (O) photochemical formation is crucial to formulating targeted O mitigation strategies. To investigate the emission source of ambient carbonyls and their integrated observational constraint on the impact of O formation chemistry, a field campaign was conducted in an industrial city (Zibo) of the North China Plain from August to September 2020. The site-to-site variations of OH reactivity for carbonyls were in accordance with the sequence of Beijiao (BJ, urban, 4.

View Article and Find Full Text PDF

The significant role of traffic emissions mixed from various sources in urban air pollution has been widely recognized. However, the corresponding contributions to the roadside particle distribution are poorly understood due to the mixed impacts of various sources. Particle number concentrations of different sizes at the roadside in Nankai District of Tianjin were continuously monitored using a portable aerosol particle spectrometer during the morning rush hour (07:30-09:20) from Nov.

View Article and Find Full Text PDF