The presence of per- and polyfluoroalkyl substances (PFAS) in surface water has been widely reported in recent years. Many techniques, e.g.
View Article and Find Full Text PDFDissolved organic matter (DOM) plays a pivotal role in drinking water treatment, influencing the performance of unit processes and final water quality (e.g. disinfection byproduct risk).
View Article and Find Full Text PDFSignificant progress has been made previously in the research and development of graphene oxide (GO) membranes for water purification, but their biofouling behavior remains poorly understood. In this study, we investigated the biofilm formation and biofouling of GO membranes with different surface microstructures in the context of filtering natural surface water and for an extended operation period (110 days). The results showed that the relatively hydrophilic and smooth Fe(OH)/GO membrane shaped a thin and spatially heterogeneous biofilm with high stable flux.
View Article and Find Full Text PDFIn this research, the interactions of two azo dyes, Methyl Orange (MO) and Eriochrome Black T (EBT), with dissolved organic matter (DOM) in surface water were studied, emphasizing their removal using nano-filtration membranes (NF-270 and NF-90). High-Performance Size Exclusion Chromatography (HPSEC) findings indicated that the dyes' molecular weight in deionized (DI) water ranged from 500 to 15k Dalton (Da), adjusting peak intensities with Jingmi River (JM) water Beijing. Notably, when dyes were diluted in JM water, ultraviolet (UV & , and UV), together with total organic carbon (TOC) parameters, revealed color removal rates of 99.
View Article and Find Full Text PDFInorganic coagulants such as poly aluminum ferric chloride (Al/Fe) are applied conventionally to sewage sludge dewatering and can be retained in the sludge cake, causing its conductivity to increase and generate secondary pollution. To reduce these disadvantages, there is a need to develop alternative, more sustainable chemicals as substitutes for conventional inorganic coagulants. In the present investigation, the application of a polymeric chitosan quaternary ammonium salt (CQAS) is explored as a complete, or partial, replacement for Al/Fe in the context of sludge dewatering processes.
View Article and Find Full Text PDFGravity-driven membrane (GDM) systems have been well developed previously; however, impacts of driving (i.e., transmembrane) pressure on their performance received little attention, which may influence GDM performance.
View Article and Find Full Text PDFWith the advancement of urban rail transit towards intelligence, the demand for urban rail transit communication has increased significantly, but the traditional urban rail transit vehicle-ground communication system has been unable to meet the future vehicle-ground communication requirements. To improve the performance of vehicle-ground communication, the paper proposes a reliable low-latency multipath routing (RLLMR) algorithm for urban rail transit ad hoc networks. First, RLLMR combines the characteristics of urban rail transit ad hoc networks and uses node location information to configure a proactive multipath to reduce route discovery delay.
View Article and Find Full Text PDFRev Sci Instrum
November 2022
Marine self-potential (SP) measurement is commonly conducted for seafloor sulfide detection and hydrothermal vent studies in deep water using instruments towed close to the seafloor. However, this method has the following shortcomings: (1) It relies on ships for deep towing, and the need for a dedicated ship time lowers its efficiency. (2) Owing to complex topography, most towed instruments are located far from the seafloor to ensure safety, resulting in large effective signal attenuation and low signal-to-noise ratio.
View Article and Find Full Text PDFIn most cases, point-of-use tap water quality is not routinely monitored due to widely-dispersed sampling sites and the costly tests. Although previous studies have revealed the variation of drinking water quality during distribution in municipal networks, the influence of aging pipes in buildings on quality is still unknown and this makes it difficult for water utilities to conduct regular maintenance. Herein, we have undertaken a survey of tap water samples across 8 districts in Beijing (China) to evaluate the potential effects of pipe age on point-of-use water quality, including turbidity, organic matter characteristics, and bacterial community.
View Article and Find Full Text PDFIn the last decades, membrane-based nanofiltration (NF) technique has been widely applied for safe and high-quality drinking water production worldwide. NF membrane fouling has become one of the main obstacles in its application due to high operation cost, and thus numerous efforts have been made. However, there is still a large disconnect between academic findings and their applications.
View Article and Find Full Text PDFMembrane filtration in various forms has become an increasingly used treatment method worldwide for the supply of safe drinking water. The fouling of membranes is commonly considered to be the major operational limitation to its wider application since it leads to frequent backwashing and a shortening of membrane life, and increased production costs. The components of natural organic matter (NOM) in surface waters have been reported previously to be important foulants of nanofiltration (NF) membranes, however, the potential beneficial effect of particular components of these 'foulants' has not been investigated or demonstrated to date.
View Article and Find Full Text PDFEnviron Sci Technol
February 2021
The presence of biopolymers in surface waters and their significance for potable water supply have received little attention previously owing to their low concentrations. In this paper, we present the results of an extensive study that has investigated the role and benefits of biopolymers during the purification of surface water with reference to their specific biological and physico-chemical properties. Using samples collected from two representative surface waters in China and the United Kingdom, macromolecular biopolymers were separated and concentrated for subsequent investigation of their role in coagulation, metal ion adsorption, and membrane separation.
View Article and Find Full Text PDFNatural organic matter (NOM) with the size approaching to membrane pore size is commonly considered as the crucial component leading to severe pore blocking and superfluous energy consumption. Aquatic metal ions coexisting with this NOM constituent (target NOM) exert a significant influence on membrane filtration performance; however, little work elucidated their interactions and the impacts on nanofiltration (NF). Therefore, we systematically investigated this issue by titrating three environmentally-relevant metal ions (Al, Fe and Cu) into the target NOM sample obtained by pre-filtering using NF membrane.
View Article and Find Full Text PDFTo alleviate ultrafiltration (UF) membrane fouling, the pre-coagulation of poly-aluminum chloride (PACl) with the aid of chitosan (CTS) was conducted for synthetic humic acid-kaolin water treatment. Pre-coagulation of three molecular weights (MW) CTSs (50-190 kDa (CTS), 190-310 kDa (CTS) and 310-375 kDa (CTS)) was optimized with slow-mixing speeds of 30, 60 and 90 r/min, respectively. The removal efficiency and floc properties as well as membrane fouling were analyzed, and were compared to results obtained by conventional coagulation with PACl.
View Article and Find Full Text PDFAlthough the treatment of natural surface waters by coagulation has been investigated extensively, the detailed interaction between natural organic matter and alum is still not adequately understood or predictable, owing to the complexity of different components of the organic matrix and the conditions during coagulation. In this paper, we present the results of a novel approach to the study of the topic, which involved the progressive separation of organic components according to size, followed by coagulation of the filtrate solution, in order to expose the influence of particular organic fractions. Using two natural water sources, representative of lake and river waters, solutions of different organic content were obtained by progressively filtering the source waters using membranes of decreasing pore size; viz.
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