Publications by authors named "Zhaoqi Deng"

Ionic liquid (IL) additives proved to have a positive effect on the device efficiency and stability of perovskite solar cells. However, since ILs are small molecules and undergo Coulomb interactions, they can easily aggregate and evaporate over long times, which would cause instabilities during a long-term device operation. To overcome these problems, we polymerize ILs into macromolecules and incorporate them into perovskite films as well as into the corresponding solar cells.

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Article Synopsis
  • Perovskite solar cells (PSCs) are highly efficient, achieving power conversion efficiencies of up to 25.5%, dependent on good contact between electron transport layers (ETLs) and perovskite films.
  • SnO thin films, processed at low temperatures, are commonly used as ETLs in planar PSCs, but creating optimal interfaces with them is challenging.
  • Modifying SnO ETLs with benzylamine hydrochloride (BH) helps align energy levels, reduces trap states, and significantly improves PSC performance in terms of efficiency, stability, and reduced hysteresis.
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We report room-temperature ultraviolet lasing action in large quantities of uniform multilayer ZnO nanosheets grown by a vapor-transport method via thermal evaporation of Zn powder. An excellent multimode lasing emission at a center wavelength of 390 nm with a mode linewidth less than 0.33 nm occurs above an excitation threshold of 8 mJ pulse(-1) cm(-2).

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High efficiency blue, green, and white inverted microcavity top-emitting organic light-emitting devices based on blue emitter p-bis(p-N,N-diphenyl-amino-styryl) benzene-doped 2-methyl-9,10-di(2-naphthyl) anthracene as the emitting layer are demonstrated. The different colors can be well realized by simply changing the thickness of the hole-transporting layer, thus modifying the cavity length to obtain various resonance wavelengths. The comprehensive analysis on the emission mechanism is presented.

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We demonstrate that the amplified spontaneous emission (ASE) in an Ag-backed red-fluorescent-dye-doped polymer film can be controlled by the effect of the film thickness. Optical losses associated with the metallic contacts necessary for charge injection, an obstacle to the development of an electrically pumped organic solid-state laser, may be possible to be reduced by increasing the gain medium layer thickness. The study of ASE characteristics of Ag-backed 4-(Dicyanomethylene)-2-t-butyl-6-(1,1,7,7-tetramethyljulolidyl-9-enyl)-4H-pyran (DCJTB)-doped polystyrene (PS) films with different thicknesses shows that increasing the film thickness can reduce the influence of the Ag layer.

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By introducing an effective electron injection layer (EIL) material, i.e., lead monoxide (PbO), combined with the optical design in device structure, a high efficiency inverted top-emitting organic light-emitting diode (ITOLED) with saturated and quite stable colors for different viewing angles is demonstrated.

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