Publications by authors named "Zhaofu Hu"

Black carbon (BC) significantly contributes to atmospheric warming and glacier melting. However, the atmospheric lifetime of BC from different fuel sources remains poorly constrained. By analyzing ΔC of BC in PM and precipitation samples collected for three years at a remote site in the Tibetan Plateau, we found that BC from fossil fuel contribution ( BC) in PM exhibited greater seasonal variation than those from South Asia and emission inventories.

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Elemental carbon (EC), also known as black carbon, plays an important role in climate change. Accurately assessing EC concentration in aerosols remains challenging due to the overestimations caused by carbonates and organic carbon (OC) during thermal-optical measurement in the Tibetan Plateau (TP). This study evaluates the extent of EC overestimated by carbonates and OC at four remote sites (Nyalamu, Lulang, Everest and Ngari) in southern and western of the TP using different treatments.

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Microplastics (MPs) in glaciers of remote areas are a hot topic linking the global transport of atmospheric MPs. The Tibetan Plateau (TP) holds large volume of glaciers, providing an effective way to trace MPs transport. Moreover, MPs in glaciers may have adverse effects on the local ecosystem and human health.

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Article Synopsis
  • Carbonaceous aerosols significantly influence radiative forcing in the Tibetan Plateau, but their sources are not well understood due to limited regional data.
  • The study presents the first detailed analysis of carbon isotopic signatures (δC) of local carbonaceous aerosol sources, revealing differences compared to other global regions.
  • The findings indicate that fossil fuel-derived aerosols in the TP are C-depleted while biomass-derived aerosols are C-enriched, and that topsoil δC values reflect local vegetation types, enhancing understanding for future environmental assessments.
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Rapid retreat and darkening of most glaciers in the Tibetan Plateau (TP) are enhanced by the deposition of light-absorbing particles (LAPs). Here, we provided new knowledge on the estimation of albedo reduction caused by black carbon (BC), water-insoluble organic carbon (WIOC), and mineral dust (MD), based on a comprehensive study of snowpit samples from ten glaciers across the TP collected in the spring of 2020. According to the albedo reductions caused by the three LAPs, the TP was divided into three sub-regions: the eastern and northern margins, Himalayas and southeastern TP, and western to inner TP.

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Carbonaceous matter (CM) (such as water-insoluble organic carbon (WIOC), black carbon (BC), and water-soluble organic carbon (WSOC)) has a significant impact on the carbon cycle and radiative forcing (RF) of glacier. Precipitation samples and glacier's snow/ice samples (snowpit, surface snow, and granular ice) (Xiao dongkemadi Glacier) were collected at the Dongkemadi River Basin (DRB) in the central Tibetan Plateau (TP) between May and October 2016 to investigate the characteristics and roles of CM in the TP River Basin. WIOC, BC, and WSOC concentrations in precipitation were relatively higher than that in snowpit, but lower than that in surface snow/ice, with the wet deposition fluxes of 0.

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Brown carbon (BrC)/water-soluble organic carbon (WSOC) plays a crucial role in glacier melting. A quantitative evaluation of the light absorption characteristics of WSOC on glacier melting is urgently needed, as the WSOC release from glaciers potentially affects the hydrological cycle, downstream ecological balance, and the global carbon cycle. In this work, the optical properties and composition of WSOC in surface snow/ice on four Tibetan Plateau (TP) glaciers were investigated using a three-dimensional fluorescence spectrometer and electrospray ionization Fourier transform ion cyclotron resonance mass spectrometry.

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Micoroplastics (MPs) can be transported through atmospheric circulations, and have caused global attentions due to their potential risk to the environment. In this study, MPs in snowpit samples collected from Demula (DML) glacier in southeast Tibetan Plateau were investigated. The results showed that the average abundance of MPs in snow was 9.

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Dissolved organic carbon (DOC) makes an important contribution to glacier melting in the Himalayas and the Tibetan Plateau (HTP). Photobleaching can effectively reduce the light absorption ability of DOC, further changing its impact on glacier melting, which is not yet well researched in the HTP. Therefore, snowpit samples from the Bayi, Ganglongjiama (GLJM), Jiemayangzong (JMYZ) and Demula (DML) glaciers were collected to study the influence of photobleaching on the light absorption ability of DOC and its impact on glacier melting.

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Carbonates cause large uncertainties in determining the concentrations of organic carbon (OC) and elemental carbon (EC), as well as EC's light absorption characteristics, in arid locations, such as Central Asia. To investigate this influence, a comparison between acid (HCl)-treated and original total suspended particle (TSP) samples was conducted in Dushanbe, Tajikistan. According to the results, the OC and EC concentrations were overestimated by approximately 22.

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Carbonaceous matter, including organic carbon (OC) and black carbon (BC), is an important climate forcing agent and contributes to glacier retreat in the Himalayas and the Tibetan Plateau (HTP). The HTP - the so-called "Third Pole" - contains the most extensive glacial area outside of the polar regions. Considerable research on carbonaceous matter in the HTP has been conducted, although this research has been challenging due to the complex terrain and strong spatiotemporal heterogeneity of carbonaceous matter in the HTP.

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Carbonaceous particles play an important role in climate change, and an increase in their emission and deposition causes glacier melting in the Himalayas and the Tibetan Plateau (HTP). This implies that studying their basic characteristics is crucial for a better understanding of the climate forcing observed in this area. Thus, we investigated characteristics of carbonaceous particles at a typical remote site of southeastern HTP.

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As an important component of organic carbon (OC), brown carbon (BrC) plays a significant role in radiative forcing in the atmosphere. Water-insoluble OC (WIOC) generally has higher light absorption ability than water-soluble OC (WSOC). The mass absorption cross-section (MAC) of WIOC is normally investigated by dissolving OC in methanol.

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Characteristics of carbonaceous aerosol (CA) and its light absorption properties are limited in Karachi, which is one of the most polluted metropolitan cities in South Asia. This study presents a comprehensive measurement of seasonality of CA compositions and mass absorption cross-section (MAC) of elemental carbon (EC) and water-soluble organic carbon (WSOC) in total suspended particles (TSP) collected from February 2015 to March 2017 in the southwest part of Karachi. The average TSP, organic carbon (OC), and EC concentrations were extremely high with values as 391.

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The Himalayan-Tibetan Plateau is a typical remote region with sparse air pollution. However, air pollution in cites of the inner Himalayan-Tibetan Plateau is relatively serious due to emissions from local residents. Carbonaceous aerosols are not only an important component of air pollutants that affect the health of local residents but also an important trigger of climate change.

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We use 84 rainfall samples collected during June to September 2017 from the Dongkemadi basin, source region of the Yangtze River, China, to analyze the characteristics and influencing factors of stable isotopes in groundwater, and further discuss the groundwater recharge sources. The results showed that the range of groundwater O values in this permafrost region varied from -15.3‰ to -12.

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Using 64 precipitation samples collected from June to September 2013 in the Dongkemadi Basin in the source region of the Yangtze River, the pH, conductivity, and main ionic concentration characteristics of precipitation were analyzed. The main ionic sources of precipitation and their relationships with atmospheric circulation were examined using factor analysis, correlation analysis, enrichment factor analysis, and backward trajectory analysis. The results showed that the range of precipitation pH values varied from 5.

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Based on the stable isotopes of 73 precipitation samples continuously collected from May to October 2014 and related meteorological statistics in the Dongkemaldi Basin, the characteristics of D, O, and -excess of precipitation, as well as the correlations between O and the rainfall amount and air temperature were analyzed. The moisture sources were tracked by the HYSPLIT model to further estimate the contribution of different water vapor sources to the rainfall amount. The results showed that the range of O and D values varied from -26.

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At present, the glaciers in the Himalayas and the Tibetan Plateau (HTP) are retreating partly due to albedo reduction caused by deposited light-absorbing impurities such as mineral dust (MD) and black carbon (BC). Because BC also exists widely in MD from surface soil, it is necessary to further evaluate the contribution of BC from MD to the total BC at glacier region. This will help to improve the study of BC sources by considering the relative contributions from MD and direct combustion sources.

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Carbonaceous matter has an important impact on glacial retreat in the Tibetan Plateau, further affecting the water resource supply. However, the related studies on carbonaceous matter are still scarce in Geladaindong (GLDD) region, the source of the Yangtze River. Therefore, the concentration, source and variations of carbonaceous matter at Ganglongjiama (GLJM) glacier in GLDD region were investigated during the melting period in 2017, which could deepen our understanding on carbonaceous matter contribution to glacier melting.

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Black carbon (BC), which consists of the strongest light-absorbing particles (LAP) in snow/ice, has been regarded as a potential factor accelerating the melting of glaciers and snow cover over the Third Pole. During the winter and summer of 2016, snow, ice and topsoil were sampled from the Laohugou basin located on the northeastern Tibetan Plateau. Concentrations of BC in Laohugou Glacier No.

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Dissolved organic carbon (DOC) released from glaciers has an important role in the biogeochemistry of glacial ecosystems. This study focuses on DOC from glaciers of the southeastern Tibetan Plateau, where glaciers are experiencing rapid shrinkage. We found that concentrations of DOC in snowpits (0.

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