Adv Sci (Weinh)
December 2024
Understanding and manipulating magnetic damping, particularly in magnetic heterostructures, is crucial for fundamental research, versatile engineering, and optimization. Although magnetic damping can be enhanced by the band hybridization between ferromagnetic and nonmagnetic materials at the interface, the contribution of individual subbands on the hybridized bands to magnetic damping is fully unexplored. Here, it is found that magnetic damping α is modified by the Fermi level in Fe/GeTe heterostructures via Bi doping.
View Article and Find Full Text PDFLow-dimensional magnetic structures coupled with superconductors are promising platforms for realizing Majorana zero modes, which have potential applications in topological quantum computing. Here, we report a two-dimensional (2D) magnetic-superconducting heterostructure consisting of single-layer chromium diiodide (CrI) on a niobium diselenide (NbSe) superconductor. Single-layer CrI nanosheets, which hold antiferromagnetic (AFM) ground states by our first-principles calculations, were epitaxially grown on the layered NbSe substrate.
View Article and Find Full Text PDFMagnetic skyrmions, topologically nontrivial whirling spin textures at nanometer scales, have emerged as potential information carriers for spintronic devices. The ability to efficiently create and erase magnetic skyrmions is vital yet challenging for such applications. Based on first-principles studies, we find that switching between intrinsic magnetic skyrmion and high-temperature ferromagnetic states can be achieved in the two-dimensional van der Waals (vdW) multiferroic heterostructure CrSeI/InTe by reversing the ferroelectric polarization of InTe.
View Article and Find Full Text PDFArising from the extreme/saddle point in electronic bands, Van Hove singularity (VHS) manifests divergent density of states (DOS) and induces various new states of matter such as unconventional superconductivity. VHS is believed to exist in one and two dimensions, but rarely found in three dimension (3D). Here, we report the discovery of 3D VHS in a topological magnet EuCdAs by magneto-infrared spectroscopy.
View Article and Find Full Text PDFThe quantum anomalous Hall effect (QAHE) has unique advantages in topotronic applications, but it is still challenging to realize the QAHE with tunable magnetic and topological properties for building functional devices. Through systematic first-principles calculations, we predict that the in-plane magnetization induced QAHE with Chern numbers = ±1 and the out-of-plane magnetization induced QAHE with high Chern numbers = ±3 can be realized in a single material candidate, which is composed of van der Waals (vdW) coupled Bi and MnBiTe monolayers. The switching between different phases of QAHE can be controlled in multiple ways, such as applying strain or (weak) magnetic field or twisting the vdW materials.
View Article and Find Full Text PDFThe understanding and manipulation of anisotropic Gilbert damping is crucial for both fundamental research and versatile engineering and optimization. Although several works on anisotropic damping have been reported, no direct relationship between the band structure and anisotropic damping was established. Here, we observed an anisotropic damping in Fe/GeTe manipulated by the symmetric band structures of GeTe via angle-resolved photoemission spectroscopy.
View Article and Find Full Text PDFThe van der Waals materials down to the monolayer (ML) limit provide a fertile platform for exploring low-dimensional magnetism and developing the novel applications of spintronics. Among them, due to the absence of the net magnetic moment, antiferromagnetic (AFM) materials have received much less attention than ferromagnetic ones. Here, by combining scanning tunneling microscopy and state-of-the-art first-principles calculations, we investigate the preparation, and electronic and magnetic properties of a vanadium(II) iodide (VI) ML.
View Article and Find Full Text PDFElectrical control of magnetic order in van der Waals (vdW) two-dimensional (2D) systems is appealing for high-efficiency and low-dissipation nanospintronic devices. For realistic applications, a vdW 2D material with ferromagnetic (FM) and ferroelectric (FE) orders coexisting and strongly coupling at room temperature is urgently needed. Here we present a potential candidate for nonvolatile electric-field control of magnetic orders at room temperature.
View Article and Find Full Text PDFBackground: Hierarchical diagnosis and treatment has been gradually implemented throughout the China. Primary physicians are the main force in primary-level medical and health services, which means that standardized training of primary-level doctors is indispensable.
Objectives: Evaluation of the effect of primary physician training on standardized management of diabetes, and comparison of the effects of different training models.
Detection and manipulation of spin current lie in the core of spintronics. Here we report an active control of a net spin Hall angle, θ(net), in Pt at an interface with a ferroelectric material PZT (PbZrTiO), using its ferroelectric polarization. The spin Hall angle in the ultra-thin Pt layer is measured using the inverse spin Hall effect with a pulsed tunneling current from a ferromagnetic LaSrMnO electrode.
View Article and Find Full Text PDFSeveral layered transition metal borides can now be realized by a simple and general fabrication method (Fokwa et al 2018 Adv. Mater. 30 1704181), inspiring our interest to transition metal borides monolayer.
View Article and Find Full Text PDFThe distribution of charge density in materials dictates their chemical bonding, electronic transport, and optical and mechanical properties. Indirectly measuring the charge density of bulk materials is possible through X-ray or electron diffraction techniques by fitting their structure factors, but only if the sample is perfectly homogeneous within the area illuminated by the beam. Meanwhile, scanning tunnelling microscopy and atomic force microscopy enable us to see chemical bonds, but only on the surface.
View Article and Find Full Text PDFTo magnetize surfaces of topological insulators without damaging their topological feature is a crucial step for the realization of the quantum anomalous Hall effect (QAHE) and remains as a challenging task. Through density functional calculations, we found that adsorption of a semiconducting two-dimensional van der Waals (2D-vdW) ferromagnetic CrI monolayer can create a sizable spin splitting at the Dirac point of the topological surface states of BiSe films. Furthermore, general rules that connect different quantum and topological parameters are established through model analyses.
View Article and Find Full Text PDFIn a very recent experimental work (Gao et al 2018 Adv. Mater. 30 1707055), a graphene-like CuSe monolayer (ML) was realized.
View Article and Find Full Text PDFWe propose the use of ferromagnetic insulator MnBiSe/BiSe/antiferromagnetic insulator MnBiSe heterostructures for the realization of the axion insulator state. Importantly, the axion insulator state in such heterostructures only depends on the magnetization of the ferromagnetic insulator and, hence, can be observed in a wide range of external magnetic fields. Using density functional calculations and model Hamiltonian simulations, we find that the top and bottom surfaces have opposite half-quantum Hall conductances, [Formula: see text] and [Formula: see text], with a sizable global spin gap of 5.
View Article and Find Full Text PDFTwo-dimensional ferromagnet CrGeTe (CGT) is so resistive below its Curie temperature that probing its magnetism by electrical transport becomes extremely difficult. By forming heterostructures with Pt, however, we observe clear anomalous Hall effect (AHE) in 5 nm thick Pt deposited on thin (<50 nm) exfoliated flakes of CGT. The AHE hysteresis loops persist to ∼60 K, which matches well to the Curie temperature of CGT obtained from the bulk magnetization measurements.
View Article and Find Full Text PDFJ Phys Condens Matter
February 2019
Two-dimensional (2D) metal-diboride ZrB monolayers was predicted theoretically as a stable new electronic material (Lopez-Bezanilla 2018 Phys. Rev. Mater.
View Article and Find Full Text PDFSynthesizing concave-structured nanoparticles (NP) with high-index surfaces offers a viable method to significantly enhance the catalytic activity of NPs. Current approaches for fabricating concave NPs, however, are limited. Exploring novel synthesis methods requires a thorough understanding of the competing mechanisms that contribute to the evolution of surface structures during NP growth.
View Article and Find Full Text PDFPhys Chem Chem Phys
August 2018
We study the electronic transport properties of two-dimensional (2D) fully-hydrogenated borophene (namely, borophane), using density functional theory and non-equilibrium Green's function approaches. Borophane shows a perfect electrical transport anisotropy and is promising for applications. Along the peak- or equivalently the valley-parallel direction, 2D borophane exhibits a metallic characteristic and its current-voltage (I-V) curve shows a linear behavior, corresponding to the ON state in borophane-based nano-switches.
View Article and Find Full Text PDFSince catalytic performance of platinum-metal (Pt-M) nanoparticles is primarily determined by the chemical and structural configurations of the outermost atomic layers, detailed knowledge of the distribution of Pt and M surface atoms is crucial for the design of Pt-M electrocatalysts with optimum activity. Further, an understanding of how the surface composition and structure of electrocatalysts may be controlled by external means is useful for their efficient production. Here, we report our study of surface composition and the dynamics involved in facet-dependent oxidation of equilibrium-shaped PtCo nanoparticles in an initially disordered state via in situ transmission electron microscopy and density functional calculations.
View Article and Find Full Text PDFRecent experiments showed that some perovskite oxyhydrides have surprisingly high magnetic-transition temperature. In order to unveil the origin of this interesting phenomenon, we investigate the magnetism in SrCrO2H and SrVO2H on the basis of first-principles calculations and Monte Carlo simulations. Our work indicates that the Cr-O-Cr superexchange interaction in SrCrO2H is unexpectedly strong.
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