In this study, we propose novel three-layer composite scintillators designed for the simultaneous detection of different ionizing radiation components. These scintillators are based on epitaxial structures of LuAG and YAG garnets, doped with Ce and Sc ions. Samples of these composite scintillators, containing YAG:Ce and LuAG:Ce single crystalline films with different thicknesses and LuAG:Sc single crystal substrates, were grown using the liquid phase epitaxy method from melt solutions based on PbO-BO fluxes.
View Article and Find Full Text PDFIn this study, Ce-doped LuAlO garnet (LuAG) crystal detectors, with a density of ρ = 6 g/cm and an effective atomic number Z = 62, are proposed as promising materials for radiotherapy applications. This type of detector demonstrates excellent uniformity of structural and optical properties, high thermoluminescence (TL) light yield, optimal position of main TL glow peaks at temperatures around 245-295 °C, and high radiation stability. The set of TL detectors made from LuAG:Ce single crystal was used to evaluate the uniformity of dose and energy spectra of X-ray radiation from a clinical accelerator with 6 MV and 15 MV beams at the Department of Medical Physics, Oncology Center in Bydgoszcz, Poland, and γ-rays from a Co source at the National Institute of Oncology in Warsaw.
View Article and Find Full Text PDFThe papers published in the first and second Special Issues of "Materials for Luminescent Detectors and Transformers of Ionizing Radiation" were selected from the manuscripts related to the respective presentations at the 11th International Conference on Luminescent Detectors and Transformers of Ionizing Radiation (LUMDETR 2021), which was organized by the Institute of Physics of Kazimierz Wielki University of Bydgoszcz and Oncology Center prof [...
View Article and Find Full Text PDFCe doped AlO-YAG eutectics were successfully grown by the horizontal directional crystallization method. The crystallization rate of eutectic growth was changed in the 1-7.5 mm/h range at a growth temperature of 1835 ℃.
View Article and Find Full Text PDFThis research focuses on LPE growth, and the examination of the optical and photovoltaic properties of single crystalline film (SCF) phosphors based on Ce-doped YMgSiAlO garnets with Mg and Si contents in x = 0-0.345 and y = 0-0.31 ranges.
View Article and Find Full Text PDFMaterials (Basel)
December 2022
Single-crystalline films (SCFs) of the LuAG: Ce garnet grown using the liquid-phase epitaxy method onto YAG single-crystal (SC) substrates were investigated for possible applications as composite thermoluminescent (TL) detectors. Such detectors may help to register the different components of ionizing radiation fields with various penetration depths, e.g.
View Article and Find Full Text PDFThis work is dedicated to the development of new types of composite thermoluminescent detectors based on the single crystalline films of Ce-doped GdAlO perovskite and Mn-doped YAlO and (LuY)AlO:Mn perovskites as well as Ce and Pr-doped YAlO single crystal substrates. These detectors were obtained using the Liquid Phase Epitaxy growth method from the melt solution based on the PbO-BO fluxes. Such composite detectors can by applied for the simultaneous registration of different components of mixed ionization fluxes using the differences between the thermoluminescent glow curves, recorded from the film and crystal parts of epitaxial structures.
View Article and Find Full Text PDFIn this study, the infrared optically stimulated luminescence (IRSL) of single crystals of Ce doped yttrium aluminum garnet (YAG) was investigated for the first time. It was found that infrared stimulation of these crystals, following previous exposure to beta radiation, produces a strong luminescence signal. The highest luminescence efficiency was exhibited by the YAG crystal with 0.
View Article and Find Full Text PDFMaterials (Basel)
November 2022
Thermostimulated luminescence (TSL) dosimetry is a versatile tool for the assessment of dose from ionizing radiation. In this work, the Ce doped YAlO garnet (YAG:Ce) with a density ρ = 4.56 g/cm and effective atomic number Z = 35 emerged as a prospective TSL material in radiotherapy applications due to its excellent radiation stability, uniformity of structural and optical properties, high yield of TSL, and good position of main glow peak around 290-300 °C.
View Article and Find Full Text PDFThis work is dedicated to the crystallization and luminescent properties of a prospective CaYMgScSiO:Ce (CYMSSG:Ce) micropowder (MP) phosphor converter (pc) for a white light-emitting LED (WLED). The set of MP samples was obtained by conventional solid-phase synthesis using different amounts of BO flux in the 1-5 mole percentage range. The luminescent properties of the CYMSSG:Ce MPs were investigated at different Ce concentrations in the 1-5 atomic percentage range.
View Article and Find Full Text PDFThis manuscript summarizes recent results on the development of composite luminescent materials based on the single-crystalline films and single crystals of simple and mixed garnet compounds obtained by the liquid-phase epitaxy growth method. Such composite materials can be applied as scintillating and thermoluminescent (TL) detectors for radiation monitoring of mixed ionization fluxes, as well as scintillation screens in the microimaging techniques. The film and crystal parts of composite detectors were fabricated from efficient scintillation/TL materials based on Ce-, Pr-, and Sc-doped LuAlO garnets, as well as Ce-doped GdAAlGaO mixed garnets, where A = Lu or Tb; x = 0-1; y = 2-3 with significantly different scintillation decay or positions of the main peaks in their TL glow curves.
View Article and Find Full Text PDFIn this work, the luminescence properties of undoped, Tm doped, and Tb plus Tm double-doped crystals of the lithium magnesium phosphate (LiMgPO, LMP) compound were investigated. The crystals under study were grown from melt using the micro-pulling-down method. The intrinsic and dopant-related luminescence of these crystals were studied using cathodo-, radio-, photo-, and thermoluminescence methods.
View Article and Find Full Text PDFSpectrochim Acta A Mol Biomol Spectrosc
April 2020
The Raman response of the YAlO (YAP) perovskite is modeled by means of periodic density functional theory. A number of different approximations to the exchange-correlation functional are benchmarked against the structural and spectroscopic data as imposing all-electron Gaussian-type basis sets. The WC1LYP functional was found to be superior, particularly outperforming other tested approaches in the prediction of the local structure of the AlO subunits, which reflects in the observed lattice-dynamics.
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