Organic, single crystals have emerged as unique optoelectrical materials due to their highly ordered structure and low defects. In this work, pentacene nanoribbons and nanosheets were selectively fabricated by controlling their growth temperature. The results show that their photoluminescence (PL) activity and electrical properties were strongly dependent on their geometrical morphology and molecular stacking mode such as the degree of π-orbital overlap and intermolecular interaction.
View Article and Find Full Text PDFHybrid systems have recently attracted increasing attention, which combine the special attributes of each constitute and create interesting functionalities through multiple heterointerface interactions. Here, we design a two-dimensional (2D) hybrid phototransistor utilizing Janus-interface engineering, in which the WSe channel combines light-sensitive perovskite and spontaneously polarized ferroelectrics, achieving collective ultrasensitive detection performance. The top perovskite (BA(MA)PbI) layer can absorb the light efficiently and provide generous photoexcited holes to WSe.
View Article and Find Full Text PDFOrganic materials exhibit efficient light absorption and low-temperature, large-scale processability, and have stimulated enormous research efforts for next-generation optoelectronics. While, high-performance organic devices with fast speed and high responsivity still face intractable challenges, due to their intrinsic limitations including finite carrier mobility and high exciton binding energy. Here an ultrafast and highly sensitive broadband phototransistor is demonstrated by integrating high-quality pentacene single crystal with monolayer graphene.
View Article and Find Full Text PDFACS Appl Mater Interfaces
December 2021
Rubrene single crystals have received a lot of attention for their great potential in electronic and wearable nanoelectronics due to their high carrier mobility and excellent flexibility. While they exhibited remarkable electrical performances, their intrinsic potential as photon detectors has not been fully exploited. Here, we fabricate a sensitive and ultrafast organic phototransistor based on rubrene single crystals.
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