Observation of spin-glass-like characteristics in ferrimagnetic TbCo through energy-level-selective approach.

Rare earth (RE)-transition metal (TM) ferrimagnetic alloys are gaining increasing attention because of their potential use in the field of antiferromagnetic spintronics. The moment from RE sub-lattice primarily originates from the 4f-electrons located far below the Fermi level (E), and the moment from TM sub-lattice arises from the 3d-electrons across the E. Therefore, the individual magnetic moment configurations at different energy levels must be explored to clarify the microscopic mechanism of antiferromagnetic spin dynamics.

Temperature dependence of intrinsic and extrinsic contributions to anisotropic magnetoresistance.

Electrical conduction in magnetic materials depends on their magnetization configuration, resulting in various magnetoresistances (MRs). The microscopic mechanisms of MR have so far been attributed to either an intrinsic or extrinsic origin, yet the contribution and temperature dependence of either origin has remained elusive due to experimental limitations. In this study, we independently probed the intrinsic and extrinsic contributions to the anisotropic MR (AMR) of a permalloy film at varying temperatures using temperature-variable terahertz time-domain spectroscopy.

A scalable molecule-based magnetic thin film for spin-thermoelectric energy conversion.

Spin thermoelectrics, an emerging thermoelectric technology, offers energy harvesting from waste heat with potential advantages of scalability and energy conversion efficiency, thanks to orthogonal paths for heat and charge flow. However, magnetic insulators previously used for spin thermoelectrics pose challenges for scale-up due to high temperature processing and difficulty in large-area deposition. Here, we introduce a molecule-based magnetic film for spin thermoelectric applications because it entails versatile synthetic routes in addition to weak spin-lattice interaction and low thermal conductivity.

A multicaloric material as a link between electrocaloric and magnetocaloric refrigeration.

The existence and feasibility of the multicaloric, polycrystalline material 0.8Pb(Fe1/2Nb1/2)O3-0.2Pb(Mg1/2W1/2)O3, exhibiting magnetocaloric and electrocaloric properties, are demonstrated.

Large spin Hall magnetoresistance and its correlation to the spin-orbit torque in W/CoFeB/MgO structures.

The phenomena based on spin-orbit interaction in heavy metal/ferromagnet/oxide structures have been investigated extensively due to their applicability to the manipulation of the magnetization direction via the in-plane current. This implies the existence of an inverse effect, in which the conductivity in such structures should depend on the magnetization orientation. In this work, we report a systematic study of the magnetoresistance (MR) of W/CoFeB/MgO structures and its correlation with the current-induced torque to the magnetization.

Thermal spin injection and accumulation in CoFe/MgO/n-type Ge contacts.

Understanding the interplay between spin and heat is a fundamental and intriguing subject. Here we report thermal spin injection and accumulation in CoFe/MgO/n-type Ge contacts with an asymmetry of tunnel spin polarization. Using local heating of electrodes by laser beam or electrical current, the thermally-induced spin accumulation is observed for both polarities of the temperature gradient across the tunnel contact.

Single crystalline β-Ag2Te nanowire as a new topological insulator.

A recent theoretical study suggested that Ag(2)Te is a topological insulator with a highly anisotropic Dirac cone. Novel physics in the topological insulators with an anisotropic Dirac cone is anticipated due to the violation of rotational invariance. From magnetoresistance (MR) measurements of Ag(2)Te nanowires (NWs), we have observed Aharanov-Bohm (AB) oscillation, which is attributed to the quantum interference of electron phase around the perimeter of the NW.

New crystal structure: synthesis and characterization of hexagonal wurtzite MnO.

Most transition metal oxides have a cubic rocksalt crystal structure, but ZnO and CoO are the only stable transition metal oxides known to possess a hexagonal structure. Unprecedented hexagonal wurtzite MnO has been prepared by thermal decomposition of Mn(acac)(2) on a carbon template. Structural characterization has been carried out by TEM, SAED, and a Rietveld analysis using XRD.

Interface effect of magnetic properties in Ni nanoparticles with a hcp core and fcc shell structure.

We have fabricated hexagonal close-packed (hcp) Ni nanoparticles covered by a face-centered cubic (fcc) Ni surface layer by polyol method. The magnetic properties have been investigated as a function of temperature and applied magnetic field. The magnetic behavior reveals that the system should be divided magnetically into three distinct phases with different origins.

Structure-induced ferromagnetic stabilization in free-standing hexagonal Fe(1.3)Ge nanowires.

Single-crystalline free-standing hexagonal Fe(1.3)Ge nanowires (NWs) are synthesized for the first time using a chemical vapor transport process without using any catalyst. Interestingly, Fe(1.

Diffusion-driven crystal structure transformation: synthesis of Heusler alloy Fe3Si nanowires.

We report fabrication of Heusler alloy Fe(3)Si nanowires by a diffusion-driven crystal structure transformation method from paramagnetic FeSi nanowires. Magnetic measurements of the Fe(3)Si nanowire ensemble show high-temperature ferromagnetic properties with T(c) >> 370 K. This methodology is also successfully applied to Co(2)Si nanowires in order to obtain metal-rich nanowires (Co) as another evidence of the structural transformation process.

Itinerant helimagnetic single-crystalline MnSi nanowires.

We report the synthesis of free-standing MnSi nanowires via a vapor transport method with no catalyst and measurements of their electrical and magnetic properties for the first time. The single-crystalline MnSi nanowire ensemble with a simple cubic (B20) crystal structure shows itinerant helimagnetic properties with a T(c) of about 30 K. A single MnSi nanowire device was fabricated by a new method using photolithography and a nanomanipulator that produces good ohmic contacts.

Composition-tuned Co(n)Si nanowires: location-selective simultaneous growth along temperature gradient.

We report the simultaneous and selective synthesis of single-crystalline Co(n)Si NWs (n = 1-3) and their corresponding crystal structures--simple cubic (CoSi), orthorhombic (Co(2)Si), and face-centered cubic (Co(3)Si)--following a composition change. Co(n)Si NWs were synthesized by placing the sapphire substrates along a temperature gradient. The synthetic process is a successful demonstration of tuning the chemical composition in Co(n)Si NWs.

Ferromagnetic signal in nanosized Ag particles.

A new technique using an inductively coupled plasma reactor equipped with a liquid-nitrogen cooling system was developed to prepare Ag nanoparticles. The magnetic signal from these Ag particles with diameters of 4 nm showed, surprisingly, a signal with combined ferromagnetic and diamagnetic components, in contrast to the signal with only one diamagnetic component from bulk Ag. The same technique was used to prepare the Ag/Cu nanoparticles, which are Ag nanoparticles coated with a Cu layer.

Kinetics of monodisperse iron oxide nanocrystal formation by "heating-up" process.

We studied the kinetics of the formation of iron oxide nanocrystals obtained from the solution-phase thermal decomposition of iron-oleate complex via the "heating-up" process. To obtain detailed information on the thermal decomposition process and the formation of iron oxide nanocrystals in the solution, we performed a thermogravimetric-mass spectrometric analysis (TG-MS) and in-situ magnetic measurements using SQUID. The TG-MS results showed that iron-oleate complex was decomposed at around 320 degrees C.

Analysis of H(c2)(θ,T) for Mg(B(1-x)C(x))(2) single crystals by using the dirty two-gap model.

To understand the effect of carbon doping on the superconductivity in MgB(2), we obtained the angle- and temperature-dependent upper critical fields [H(c2)(θ) and H(c2)(T)] for Mg(B(1-x)C(x))(2) single crystals (x = 0.06 and 0.1) from resistivity measurements while varying the temperature, the field, and the direction of the field.

Magnetic properties of single-crystalline CoSi nanowires.

We have observed unusual ferromagnetic properties in single-crystalline CoSi nanowire ensemble, in marked contrast to the diamagnetic CoSi in bulk. High-density freestanding CoSi nanowires with B20 crystal structure are synthesized by a vapor-transport-based method. The reaction of cobalt chloride precursor with a Si substrate produces high-aspect-ratio CoSi nanowires.

Synthesis and Photoluminescence of Cd-doped alpha-MnS Nanowires.

Cd-doped alpha-MnS nanowires (av diam = 70 nm) were synthesized by the chemical vapor deposition of MnCl(2)/CdS powders. They all consisted of single-crystalline rock-salt MnS structures with the [111] growth direction. The X-ray diffraction pattern analysis indicates that 10% Cd doping would expand the lattice constants by 0.

Ferrimagnetic Mn2SnO4 nanowires.

Single-crystalline Mn2SnO4 nanowires were first synthesized by chemical vapor deposition; they consist of inverse spinel structure grown with the [111] direction; the nanowires have a ferrimagnetic phase below 46 K (T(C)) with large hysteresis; this ferrimagnetic transition is probably due to the presence of Mn3+ ions at octahedral sites.