Electrochemical liquid-cell transmission electron microscopy (e-LCTEM) offers great potential for investigating the structural dynamics of nanomaterials during electrochemical reactions. However, challenges arise from the difficulty in achieving the optimal electrolyte thickness, leading to inconsistent electrochemical responses and limited spatial resolution. In this study, we present advanced e-LCTEM techniques tailored for tracking Pt/C degradation under electrochemical polarization at short intervals with high spatial resolution.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2022
Solid-state supercapacitors have shown extraordinary promise for flexible and wearable electronics. To date, they are still limited by relatively poor energy volumetric performances, which are largely determined by the pore structures and physicochemical properties of electrode materials. Moreover, the poor mechanical properties afforded because of the intrinsic shortcomings of electrode materials need to be resolved.
View Article and Find Full Text PDFIn this study, nano-scale fillers are added to epoxy matrix-based carbon fibers-reinforced composites (CFRPs) to improve the mechanical properties of multi-scale composites. Single-walled carbon nanotubes (SWCNTs) used as nano-scale fillers are treated with atmospheric-pressure plasma to introduce oxygen functional groups on the fillers' surface to increase the surface free energy and polar component, which relates to the mechanical properties of multi-scale composites. In addition, the effect of dispersibility was analyzed through the fracture surfaces of multi-scale composites containing atmospheric-pressure plasma-treated SWCNTs (P-SWCNTs) under high load conditions.
View Article and Find Full Text PDFNovel and effective reduced graphene oxide-nickel (Ni) doped manganese oxide (RGO/Ni-MnO) adsorbents were fabricated a hydrothermal approach. The reduction of graphite to graphene oxide (GO), formation of α-MnO, and decoration of Ni-MnO onto the surface of reduced graphene oxide (RGO) were independently carried out by a hydrothermal technique. The physical and morphological properties of the as-synthesized adsorbents were analyzed.
View Article and Find Full Text PDFPhase-change materials (PCMs) are essential modern materials for storing thermal energy in the form of sensible and latent heat, which play important roles in the efficient use of waste heat and solar energy. In the development of PCM technology, many types of materials have been studied, including inorganic salt and salt hydrates and organic matter such as paraffin and fatty acids. Considerable research has focused on the relationship between the material structure and energy storage properties to understand the heat storage/emission mechanism involved in controlling the energy storage performance of materials.
View Article and Find Full Text PDFCarbon-based materials, including graphene, single walled carbon nanotubes (SWCNTs), and multi walled carbon nanotubes (MWCNTs), are very promising materials for developing future-generation electronic devices. Their efficient physical, chemical, and electrical properties, such as high conductivity, efficient thermal and electrochemical stability, and high specific surface area, enable them to fulfill the requirements of modern electronic industries. In this review article, we discuss the synthetic methods of different functionalized carbon materials based on graphene oxide (GO), SWCNTs, MWCNTs, carbon fibers (CFs), and activated carbon (AC).
View Article and Find Full Text PDFThermoelectric devices have recently attracted considerable interest owing to their unique ability of converting heat to electrical energy in an environmentally efficient manner. These devices are promising as alternative power generators for harvesting electrical energy compared to conventional batteries. Inorganic crystalline semiconductors have dominated the thermoelectric material fields; however, their application has been restricted by their intrinsic high toxicity, fragility, and high cost.
View Article and Find Full Text PDFIn this study, magnesium oxide (MgO)-modified carbon adsorbents were fabricated using a nitrogen-enriched carbon precursor by microwave-assisted irradiation for CO capture. The X-ray diffraction (XRD) patterns showed the characteristic diffraction peaks of MgO at 43° and 62.5°, and no impurities were apparent.
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