We determine the phase diagram of excitons in a symmetric transition-metal dichalcogenide 3-layer heterostructure. First principles calculations reveal interlayer exciton states of a symmetric quadrupole, from which higher energy asymmetric dipole states are composed. We find quantum phase transitions between a repulsive quadrupolar and an attractive staggered dipolar lattice phases, driven by a competition between interactions and single exciton energies.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
September 2019
Strongly interacting bosons display a rich variety of quantum phases, the study of which has so far been focused in the dilute regime, at a fixed number of particles. Here we demonstrate the formation of a dense Bose-Einstein condensate in a long-lived dark spin state of 2D dipolar excitons. A dark condensate of weakly interacting excitons is very fragile, being unstable against a coherent coupling of dark and bright spin states.
View Article and Find Full Text PDFExciton-polaritons are mutually interacting quantum hybridizations of confined photons and electronic excitations. Here, we demonstrate a system of optically guided, electrically polarized exciton-polaritons ("dipolaritons") that displays up to 200-fold enhancement of the polariton-polariton interaction strength compared to unpolarized polaritons. The magnitude of the dipolar interaction enhancement can be turned on and off and can be easily tuned over a very wide range by varying the applied polarizing electric field.
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