Despite two-dimensional (2D) Ruddlesden-Popper-phase layered perovskites (RPLPs) exhibiting excellent environmental stability, most solar cells based on 2D RPLP films are fabricated in a controlled inert atmosphere. Meanwhile, the poor charge transport of 2D RPLP films owing to the unfavorable phase arrangement and defects limits the efficiency of 2D RPLP solar cells. Here, we fabricate high-efficiency 2D RPLP solar cells in ambient air assisted by a zwitterion (ZW) additive.
View Article and Find Full Text PDFACS Appl Mater Interfaces
April 2021
The inorganic CsPbI perovskite has attracted tremendous attention in the photovoltaic fields for its chemical stability and suitable band gap. Generally, CsPbI solar cells with decent performances adopted high annealing temperature to form high-quality black-phase perovskite films. The high-temperature process hinders its practical application and further development.
View Article and Find Full Text PDFSteering the crystallization of two-dimensional (2D) perovskite film is an important strategy to improve the power conversion efficiency (PCE) of 2D perovskite solar cells (PVSCs). In this paper, the deionized water (HO) additive is introduced into the perovskite precursor solution to prepare high-quality 2D perovskite films. The 2D perovskite film treated with 3% HO shows a good surface morphology, increased crystal size, enhanced crystallinity, preferred orientation, and low defect density.
View Article and Find Full Text PDFNanoscale Res Lett
September 2019
The trap-state density in perovskite films largely determines the photovoltaic performance of perovskite solar cells (PSCs). Increasing the crystal grain size in perovskite films is an effective method to reduce the trap-state density. Here, we have added NHSCN into perovskite precursor solution to obtain perovskite films with an increased crystal grain size.
View Article and Find Full Text PDFNanoscale Res Lett
August 2019
All inorganic CsPbIBr perovskites have been widely used in photodetectors due to their excellent optoelectronic properties and simple preparation processes. Here, high-performance flexible photodetectors based on inorganic CsPbIBr perovskites are demonstrated, which are achieved by a modified solution-processed method. When biased at a low voltage of 10 mV, the device yielded fast response speeds (90 μs /110 μs for CsPbIBr PDs and 100 μs/140 μs for CsPbIBr PDs), a high on/off ratio of 10, and a high detectivity about 10 Jones.
View Article and Find Full Text PDFNanoscale Res Lett
August 2019
The application potential of wearable electronics in the healthcare field has been of great interest over the past several decades. Flexible and wearable devices based on skin-friendly soft elastic materials can be snugly attached to the surface of human skin, so that a series of vital health information such as wrist pulse, body temperature, and blood glucose can be extracted and analyzed to help the patient maintain physical fitness. Here, we outlined the most common types of wearable electronics for monitoring human health information, including force sensors, temperature sensors, physiological biochemical sensors, and multifunctional sensors.
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