Electronic waste (e-waste) and diabetes are global challenges to modern societies. However, solving these two challenges together has been challenging until now. Herein, we propose a laser-induced transfer method to fabricate portable glucose sensors by recycling copper from e-waste.
View Article and Find Full Text PDFAdv Sci (Weinh)
September 2024
Due to its outstanding physical and chemical properties, graphene synthesized by laser scribing on polyimide (PI) offers excellent opportunities for photothermal applications, antiviral and antibacterial surfaces, and electrochemical storage and sensing. However, the utilization of such graphene for imaging is yet to be explored. Herein, using chemically durable and electrically conductive laser-induced graphene (LIG) for tomography imaging in aqueous suspensions is proposed.
View Article and Find Full Text PDFFaced with the increasing prevalence of chronic kidney disease (CKD), portable monitoring of CKD-related biomarkers such as potassium ion (K), creatinine (Cre), and lactic acid (Lac) levels in sweat has shown tremendous potential for early diagnosis. However, a rapidly manufacturable portable device integrating multiple CKD-related biomarker sensors for ease of sweat testing use has yet to be reported. Here, a portable electrochemical sensor integrated with multifunctional laser-induced graphene (LIG) circuits and laser-printed nanomaterials based working electrodes fabricated by fully automatic laser manufacturing is proposed for non-invasive human kidney function monitoring.
View Article and Find Full Text PDFThe global water crisis demands immediate attention, and atmospheric water harvesting (AWH) provides a viable alternative. However, studying the real-time subtle relationship between water absorption, diffusion, and internal structure for hygroscopic materials is challenging. Herein, a dynamic visualization technique is proposed that utilizes an in situ electrical impedance tomography (EIT) system and a precise reconstruction algorithm to achieve real-time monitoring of the water sorption process within aerogels from an internal microstructural perspective.
View Article and Find Full Text PDFA portable sweat urea sensing system is a promising solution to satisfy the booming requirement of kidney function tele-monitoring. However, the complicated manufacturing route and the cumbersome electrochemical testing system still need to be improved to develop the urea point-of-care testing (POCT) and tele-monitoring devices. Here, a universal technical route based on a high-throughput automatic laser printing strategy for fabricating the portable integrated urea monitoring system is proposed.
View Article and Find Full Text PDFSi nanoparticles (NPs) are considered as a promising high-capacity anode material owing to their ability to prevent mechanical failure from drastic volume change during (de)lithiation. However, upon cycling, a quick capacity fading is still observed for Si NPs, and the underlying mechanism remains elusive. In this contribution, it is demonstrated that the quick capacity fading is mainly caused by the generation of dead (electrochemically inert) Si with blocked electron conductivity in a densely composited Si/SEI (solid electrolyte interface) hybrid.
View Article and Find Full Text PDFPatterning is crucial for the large-scale application of functional materials. Laser-induced transfer is an emerging patterning method for additively depositing functional materials to the target acceptor. With the rapid development of laser technologies, this laser printing method emerges as a versatile method to deposit functional materials in either liquid or solid format.
View Article and Find Full Text PDFComput Intell Neurosci
March 2023
Object detection and recognition is a very important topic with significant research value. This research develops an optimised model of moving target identification based on CNN to address the issues of insufficient positioning information and low target detection accuracy (convolutional neural network). In this article, the target classification information and semantic location information are obtained through the fusion of the target detection model and the depth semantic segmentation model.
View Article and Find Full Text PDFThis work reports the synthesis of CuSn alloy aerogels for electrochemical CO reduction catalysts. An in situ reduction and the subsequent freeze-drying process can successfully give CnxSny aerogels with tuneable Sn contents, and such aerogels are composed of three-dimensional architectures made from inter-connected fine nanoparticles with pores as the channels. Density functional theory (DFT) calculations show that the introduction of Sn in Cu aerogels inhibits H evolution reaction (HER) activity, while the accelerated CO desorption on the catalyst surface is found at the same time.
View Article and Find Full Text PDFTiO has been considered as a promising intercalation lithium-ion-battery (LIB) anode material owing to its robust cyclability. However, it suffers from low capacity. Herein, we construct a sub 10 nm scale interfused TiO/SiO hybrid with a bicontinuous structure, in which bridged TiO nanoparticles (over 80 wt %) are densely packed within a wormlike SiO network, through the simple oxidation of MAX TiSiC ceramic.
View Article and Find Full Text PDFThis paper reports a general electrospinning method to prepare various metal phosphide/carbon nanofibers composite for electrochemical hydrogen evolution reaction (HER) catalysts. An earth-abundant organic acid-phytic acid is successfully incorporated into a conventional electrospinning precursor as the phosphorus source, and continuous nanofibers can be obtained through spinning. After heat treatment, metal phosphide/carbon composite nanofibers can be obtained, with fine phosphide nanoparticles well dispersed on the surface of an interconnected carbon backbone network.
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