The consumption of organophosphorus flame retardants (OPFRs) has surged significantly recent years since global banning of brominated flame retardants (BFRs). Industrial activities are an important source of OPFRs, however there are few studies on OPFRs contamination in the indoor and outdoor atmosphere of industrial areas. A study was conducted to analyze contamination of 15 OPFRs individuals in both indoor and outdoor air and PM of living and industrial sites of the petrochemical industrial area (outdoor and indoor sites of living area was LO and LI, outdoor and indoor sites of industrial area was LO and LI).
View Article and Find Full Text PDFThe airport and its surrounding areas are home to a variety of pollution sources, and air pollution is a recognized health concern for local populated regions. Submicron particulate matter (PM with an aerodynamic diameter of <1 mm) is a typical pollutant at airports, and the enrichment of heavy metals (HMs) in PM poses a great threat to human health. To comprehensively assess the source-specific health effects of PM-bound HMs in an airport community, PM filter samples were collected around the Tianjin Binhai International Airport for 12 h during the daytime and nighttime, both in the spring and summer, and 10 selected HMs (V, Cr, Mn, Co, Ni, Cu, Zn, As, Cd, and Pb) were analyzed.
View Article and Find Full Text PDFOrganophosphate flame retardants (OPFRs) are widely used as alternatives to brominated flame retardants in a variety of consumer products and their consumption has continuously increased in recent years. However, their concentrations and human exposures in indoor microenvironments, particularly in a university environment, have received limited attention. In this study, the concentrations and seasonal variations of 15 OPFRs were assessed in typical microenvironments of two universities, including dormitories, offices, public microenvironments (PMEs: classroom, dining hall, gymnasium and library), and laboratories on the northern coast of China.
View Article and Find Full Text PDFAtmospheric polycyclic aromatic hydrocarbons (PAHs) and their derivatives are a global problem that influences the environment and threatens human health. To investigate the characteristics, sources, and health risk assessment of PM-bound PAHs and their derivatives, PM were collected at an urban site in Zibo from November 5 to December 26, 2020, and the concentrations of 16 conventional PAHs, nine NPAHs, and five OPAHs in PM were analyzed using gas chromatography-mass spectrometry. Source apportionment of PAHs and their derivatives was conducted using diagnostic ratios and a PMF model, and the health risks of PAHs and their derivatives to adult men and women were evaluated using the source-dependent incremental lifetime cancer risk (ILCR) model.
View Article and Find Full Text PDFA systematic study of the movement of PAHs (Polycyclic aromatic hydrocarbons) and their derivatives through air, soil, and water is key to understanding the exchange and transport mechanisms of these pollutants in the environment and for ultimately improving environmental quality. PAHs and their derivatives, such as nitrated PAHs (NPAHs), oxygenated PAHs (OPAHs), brominated PAHs (BrPAHs) and chlorinated PAHs (ClPAHs), were analyzed in air, bulk deposition, soil, and water samples collected from urban, rural, field, and background sites on the eastern coast of China. The goal was to investigate and discuss their spatiotemporal variations, exchange fluxes, and transport potential.
View Article and Find Full Text PDFThis study focuses on the components and levels of polycyclic aromatic hydrocarbons (PAHs) and their derivatives (MPAHs and OPAHs) in plasma samples from 19 oil workers, pre- and post-workshift, and their exposure-response relationship with mitochondrial DNA (mtDNA) methylation. PAH, MPAH, OPAH, and platelet mtDNA methylation levels were determined using a gas chromatograph mass spectrometer (GC-MS) and a pyrosequencing protocol, respectively. The total plasma concentrations of PAHs in mean value were, respectively, 31.
View Article and Find Full Text PDFExposure to polycyclic aromatic hydrocarbons (PAHs) is emerging as a risk factor for obesity, but with conflicting findings. The aim of this systematic review is to investigate and summarize the current evidence towards the associations between PAHs exposure and risk of obesity. We conducted a systematic search of online databases, including PubMed, Embase, Cochrane Library, and Web of Science up to April 28, 2022.
View Article and Find Full Text PDFFor investigating the spatial, temporal variations and assessing ecological risk of 10 antibiotics and 6 antimycotics, influent sewage water and treated effluent were collected during three different seasons in 19 waste water treatment plants of Tianjin. High performance liquid chromatography tandem mass spectrometry was used to analyze 16 substances. The concentration range of influent samples was not detected (nd) -547.
View Article and Find Full Text PDFPolycyclic aromatic hydrocarbons (PAHs), nitrated-PAHs (NPAHs) and oxygenated-PAHs (OPAHs) are environmental pollutants with adverse effects on human health. The correlation between the concentrations of PAHs, NPAHs and OPAHs in human plasma and the methylation level of mitochondrial DNA (mtDNA) was investigated using data from 110 plasma samples collected in Tianjin, China. The median concentrations of PAHs, NPAHs and OPAHs were 16.
View Article and Find Full Text PDFHuan Jing Ke Xue
April 2022
Based on the field research activity level, the emission inventory of agricultural ammonia in Xining City in 2018 was established using the emission factor method. The emission characteristics of agricultural ammonia in Xining City were analyzed, a spatial grid distribution of 3 km×3 km was carried out by ArcGIS, and an uncertainty analysis of the ammonia emission inventory of livestock and poultry breeding and nitrogen fertilizer application was carried out via Monte Carlo simulation. The results showed that the total amount of ammonia emissions from agricultural sources in Xining City in 2018 was 4644.
View Article and Find Full Text PDFTen nitrated polycyclic aromatic hydrocarbons (nPAHs) and 4 oxygenated polycyclic aromatic hydrocarbons (oPAHs) in fine particulate matter (PM) samples from Mount Tai were analyzed during summer (June to August), 2015. During the observation campaign, the mean concentration of total nPAHs and oPAHs was 31.62 pg/m and 0.
View Article and Find Full Text PDFHuan Jing Ke Xue
September 2020
In order to study the characteristics and sources of carbon fractions in PM in road dust in Anshan, road dust samples were collected from nine roads in Anshan in October 2014 and re-suspended on filters using a NK-ZXF sampler to obtain PM samples. A thermal optical carbon analyzer (IMPROVE-TOR) was employed to measure the mass fraction of organic carbon (OC) and elemental carbon (EC) in PM. The results showed that (TC) in PM in road dust was 9.
View Article and Find Full Text PDFThis study was designed to evaluate the occurrence and variation in concentrations, sources and cancer risk of PM-bound PAHs. Airborne PM-bound PAHs were sampled during a one-year campaign (2014-2015) in Anshan city, a typical iron and steel city in northeast China. A total of 374 PM samples were collected.
View Article and Find Full Text PDFIn order to study the characteristics and sources of carbon fractions in PM and PM of road dust in Tianjin, samples of road dust were collected by the quadrat sampling method in April 2015 in Tianjin, and samples were re-suspended on filters by using a NK-ZXF sampler. A Thermal Optical Carbon Analyzer (IMPROVE-TOR) was employed to measure the concentrations of organic carbon (OC) and elemental carbon (EC), and the pollution characteristics and sources were investigated by non-parametric tests and OC/EC ratio, correlation, and cluster analyses. The results showed that (total carbon, TC) in PM of road dust amounted to 4.
View Article and Find Full Text PDFJ Environ Sci Health A Tox Hazard Subst Environ Eng
November 2019
Main purpose of this study was to determine the concentrations of selected heavy elements (As, Cd, Pb, Cu, Co, Cr and Ni) in the street dust samples (n = 49) collected from seven districts located in suburban/urban zone of Tianjin in order to estimate their possible sources and degree of environmental pollution as well as human health risk. Mean concentrations (mg kg) of As (19.3), Cd (0.
View Article and Find Full Text PDFIn order to study the characteristics and source of water-soluble ions in PM in Panjin, PM samples were collected at three sites in January of 2017, and the levels of eight ions (Na, Mg, Ca, K, NH, SO, Cl, and NO) were determined by ICS-900 ion chromatograph. The characteristics of PM, the water-soluble ion concentration, SOR and NOR calculation, and ion balance calculation were investigated, and a principal component analysis was conducted. The results showed that the concentration of PM and water-soluble ions followed a descending sequence of park > development zone > the second middle school.
View Article and Find Full Text PDFIn order to collect comprehensive information regarding the characteristics and sources of the water-soluble inorganic ions in road dust (RD) PM in Tianjin, samples of road dust were collected in April 2015 in Tianjin, and then re-suspended on filters using a NK-ZXF sampler. The concentrations of the major water-soluble inorganic ions were analyzed by ion chromatography. A correlation analysis, ratio method, and principal component analysis were used to analyze the sources of RD PM.
View Article and Find Full Text PDFTo explore the element pollution characteristics and sources of road dust fall, road dust fall samples were collected during spring in Tianjin and suspended to obtain PM and PM, 16 elements were analyzed, and then their characteristics, sources, and similarities were studied by nonparametric tests, the coefficient of divergence, and enrichment factor. The results showed that the mass fraction (1%-20%) in sequential order of the elements in PM and PM in Tianjin road dust fall were Si > Al > Ca > Fe > Mg > K > Na. The coefficient of divergence of elements in PM and PM was 0.
View Article and Find Full Text PDFIn order to collect comprehensive information on the characteristics and sources of water-soluble inorganic ions in road dust (RD) PM in Liaoning Province, samples of road dust were collected in 2014 and 2016 in Anshan and Panjin and then re-suspended on filters using an NK-ZXF sampler. The concentrations of the major water-soluble inorganic ions were analyzed by ion chromatography. A correlation analysis, ratios, and a principal component analysis were used to analyze the sources of RD.
View Article and Find Full Text PDFIn order to study the pollution characteristics and sources of carbon in Panjin City during autumn and winter, PM samples were collected at three monitoring points in October 2016 and January 2017. Pollution characteristics and sources of carbon components in PM were analyzed by the OC/EC ratio method, EC tracer method, and principal component analysis method. The results showed that the PM concentration exceeded the ambient air quality standard (GB 3095-2012) and that the average concentrations of OC and EC were 10.
View Article and Find Full Text PDFEcotoxicol Environ Saf
January 2018
This is the first study reporting the presence of six phthalic acid esters (PAEs) in 45 composite soil and road dust samples collected in the urban zone of Tianjin, China. Three sample types (one soil and two road dust) were collected from the city parks. Soil samples (SI) were obtained from inside the park, road dust samples (RDI) were gathered from inside the park roads and the others (RDA) from roads surrounding parks.
View Article and Find Full Text PDFFood Addit Contam Part B Surveill
December 2017
The aim of this study was to determine levels of 11 mycotoxins, 10 trace elements, and 6 phthalates in rice samples from Serbian and Chinese market. Mycotoxins were not detected in any of the analysed rice samples. Results revealed similar median levels for following elements: Mn, 17.
View Article and Find Full Text PDFThis is the first study reporting the presence of 6 phthalic acid esters (PAEs) in 60 composite soil and street dust samples collected in the urban zone of Novi Sad, the second largest city in Serbia. The results were further used to assess children's and adults' PAEs nondietary daily intakes (DIs) through incidental soil and dust ingestion and/or dermal absorption. The study could be regarded as the important baseline for future monitoring of PAEs in the urban environments, particularly as it contributes to the rare data on PAEs occurence in the street dust.
View Article and Find Full Text PDFDaily PM2.5 samples were collected at a suburban site of Nanjing around 2014 Chinese Spring Festival (SF) and analyzed for 18 kinds of polycyclic aromatic hydrocarbons (PAHs) by GC-MS. Comparison of PAH concentrations during different periods, with different air mass origins and under different pollution situations was done.
View Article and Find Full Text PDFThe study on determining the concentration of coating solution attaching to honeycomb denuder was conducted, from 1 July to 31 August, 2013, at the roof of Lihua building at Nankai University in Tianjin. The results of experiment showed that the optimized concentration of sodium carbonate coated on the honeycomb denuder was 3%, and the optimized concentration of citric acid was 6%. The contrast sampling results of PM2.
View Article and Find Full Text PDF