The discovery of superconductivity with a critical temperature of about 80 K in LaNiO single crystals under pressure has received enormous attention. LaNiO is not superconducting under ambient pressure but exhibits a transition at T ≃ 115 K. Understanding the electronic correlations and charge dynamics is an important step towards the origin of superconductivity and other instabilities.
View Article and Find Full Text PDFNaturally existing in-plane hyperbolic polaritons and the associated optical topological transitions, which avoid the nano-structuring to achieve hyperbolicity, can outperform their counterparts in artificial metasurfaces. Such plasmon polaritons are rare, but experimentally revealed recently in WTe van der Waals thin films. Different from phonon polaritons, hyperbolic plasmon polaritons originate from the interplay of free carrier Drude response and interband transitions, which promise good intrinsic tunability.
View Article and Find Full Text PDFJ Phys Condens Matter
May 2023
The kagome lattice provides a fertile platform to explore novel symmetry-breaking states. Charge-density wave (CDW) instabilities have been recently discovered in a new kagome metal family, commonly considered to arise from Fermi-surface instabilities. Here we report the observation of Raman-active CDW amplitude modes in CsVSb, which are collective excitations typically thought to emerge out of frozen soft phonons, although phonon softening is elusive experimentally.
View Article and Find Full Text PDFThe discovery of magnetic Weyl semimetal (magnetic WSM) in Co_{3}Sn_{2}S_{2} has triggered great interest for abundant fascinating phenomena induced by band topology conspiring with the magnetism. Understanding how the magnetization affects the band structure can give us a deeper comprehension of the magnetic WSMs and guide us for the innovation in applications. Here, we systematically study the temperature-dependent optical spectra of ferromagnetic WSM Co_{3}Sn_{2}S_{2} experimentally and simulated by first-principles calculations.
View Article and Find Full Text PDFRoom-temperature magnetoelectric (ME) coupling is developed in artificial multilayers and nanocomposites composed of magnetostrictive and electrostrictive materials. While the coupling mechanisms and strengths in multilayers are widely studied, they are largely unexplored in vertically aligned nanocomposites (VANs), even though theory has predicted that VANs exhibit much larger ME coupling coefficients than multilayer structures. Here, strong transverse and longitudinal ME coupling in epitaxial BaTiO:CoFeO VANs measured by both optical second harmonic generation and piezoresponse force microscopy under magnetic fields is reported.
View Article and Find Full Text PDFNanoscale metamaterials exhibit extraordinary optical properties and are proposed for various technological applications. Here, a new class of novel nanoscale two-phase hybrid metamaterials is achieved by combining two major classes of traditional plasmonic materials, metals (e.g.
View Article and Find Full Text PDFBlack TiO2 nanoparticles with a crystalline core and amorphous-shell structure exhibit superior optoelectronic properties in comparison with pristine TiO2. The fundamental mechanisms underlying these enhancements, however, remain unclear, largely due to the inherent complexities and limitations of powder materials. Here, we fabricate TiO2 homojunction films consisting of an oxygen-deficient amorphous layer on top of a highly crystalline layer, to simulate the structural/functional configuration of black TiO2 nanoparticles.
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