Liquid-liquid interfaces hold the potential to serve as versatile platforms for dynamic processes, due to their inherent fluidity and capacity to accommodate surface-active materials. This study explores laser-driven actuation of liquid-liquid interfaces with and without loading of gold nanoparticles and further exploits the laser-actuated interfaces with nanoparticles for tunable photonics. Upon laser exposure, gold nanoparticles were rearranged along the interface, enabling the reconfigurable, small-aperture modulation of light transmission and the tunable lensing effect.
View Article and Find Full Text PDFRational manipulation and assembly of discrete colloidal particles into architected superstructures have enabled several applications in materials science and nanotechnology. Optical manipulation techniques, typically operated in fluid media, facilitate the precise arrangement of colloidal particles into superstructures by using focused laser beams. However, as the optical energy is turned off, the inherent Brownian motion of the particles in fluid media impedes the retention and reconfiguration of such superstructures.
View Article and Find Full Text PDFStudy Objectives: This study aimed to evaluate the safety and short-term effect of contemporaneous surgeries (bariatric surgery plus uvulopalatopharyngoplasty [UPPP]) in the treatment of morbid obesity comorbid with severe obstructive sleep apnea (OSA).
Methods: A retrospective cohort study was performed to identify patients with obesity and severe OSA who underwent laparoscopic sleeve gastrectomy (LSG) with or without UPPP surgeries between December 2019 and December 2021 in our center. Patients were divided into 2 groups according to different surgical methods (contemporaneous group [LSG with UPPP] vs LSG-only group).
Two-dimensional exciton-polaritons in monolayer transition metal dichalcogenides (TMDs) exhibit practical advantages in valley coherence, optical nonlinearities, and even bosonic condensation owing to their light-emission capability. To achieve robust exciton-polariton emission, strong photon-exciton couplings are required at the TMD monolayer, which is challenging due to its atomic thickness. High-quality () factor optical cavities with narrowband resonances are an effective approach but typically limited to a specific excitonic state of a certain TMD material.
View Article and Find Full Text PDFCephalometric analysis is a standard diagnostic tool in orthodontics and craniofacial surgery. Today, as conventional 2D cephalometry is limited and susceptible to analysis bias, a more reliable and user-friendly three-dimensional system that includes hard tissue, soft tissue, and airways is demanded in clinical practice. We launched our study to develop such a system based on CT data and landmarks.
View Article and Find Full Text PDFOptical tweezers have provided tremendous opportunities for fundamental studies and applications in the life sciences, chemistry, and physics by offering contact-free manipulation of small objects. However, it requires sophisticated real-time imaging and feedback systems for conventional optical tweezers to achieve controlled motion of micro/nanoparticles along textured surfaces, which are required for such applications as high-resolution near-field characterizations of cell membranes with nanoparticles as probes. In addition, most optical tweezers systems are limited to single manipulation modes, restricting their broader applications.
View Article and Find Full Text PDFThe aim of the study was to describe an approach where condylar resection with condylar neck preservation was combined with Le Fort I osteotomy and unilateral mandibular sagittal split ramus osteotomy (SSRO). Patients with a unilateral condylar osteochondroma combined with dentofacial deformity and facial asymmetry who underwent surgery between January 2020 and December 2020 were enrolled. The operation included condylar resection, Le Fort I osteotomy and contralateral mandibular sagittal split ramus osteotomy (SSRO).
View Article and Find Full Text PDFChildren with cleft lip/palate are usually faced with upper airway problems after surgical repair. The severity of upper airway obstruction is more likely associated with the age and preoperative diagnosis of obstructive sleep apnea (OSA). This study aimed to investigate the severity of OSA in toddlers before palatoplasty from the perspective of polysomnography.
View Article and Find Full Text PDFDeep learning (DL) has emerged as a promising tool for photonic inverse design. Nevertheless, despite the initial success in retrieving spectra of modest complexity with nearly instantaneous readout, DL-assisted design methods often underperform in accuracy compared with advanced optimization techniques and have not proven competitive in handling spectra of practical usefulness. Here, we introduce a tandem optimization model that combines a mixture density network (MDN) and a fully connected (FC) network to inversely design practical thin-film high reflectors.
View Article and Find Full Text PDFSubwavelength optical resonators with spatiotemporal control of light are essential to the miniaturization of optical devices. In this work, chemically synthesized transition metal dichalcogenide (TMDC) nanowires are exploited as a new type of dielectric nanoresonators to simultaneously support pronounced excitonic and Mie resonances. Strong light-matter couplings and tunable exciton polaritons in individual nanowires are demonstrated.
View Article and Find Full Text PDFMotors that can convert different forms of energy into mechanical work are of profound importance to the development of human societies. The evolution of micromotors has stimulated many advances in drug delivery and microrobotics for futuristic applications in biomedical engineering and nanotechnology. However, further miniaturization of motors toward the nanoscale is still challenging because of the strong Brownian motion of nanomotors in liquid environments.
View Article and Find Full Text PDFThe homogeneous exciton linewidth, which captures the coherent quantum dynamics of an excitonic state, is a vital parameter in exploring light-matter interactions in 2D transition metal dichalcogenides (TMDs). An efficient control of the exciton linewidth is of great significance, and in particular of its intrinsic linewidth, which determines the minimum timescale for the coherent manipulation of excitons. However, such a control is rarely achieved in TMDs at room temperature (RT).
View Article and Find Full Text PDFCircularly polarized light (CPL) carrying spin angular momentum is crucial to many applications, such as quantum computing, optical communication, novel displays, and biosensing. Nonetheless, the emission from chiral molecules contains comparable CPL components with opposite handedness, resulting in low levels of CPL overall with a small dissymmetry factor and fixed handedness consistent with the handedness of the molecules. Nanoantennas have proved to be useful tools for controlling the emission properties of quantum emitters.
View Article and Find Full Text PDFCoupling emitters with nanoresonators is an effective strategy to control light emission at the subwavelength scale with high efficiency. Low-loss dielectric nanoantennas hold particular promise for this purpose, owing to their strong Mie resonances. Herein, a highly miniaturized platform is explored for the control of emission based on individual subwavelength Si nanospheres (SiNSs) to modulate the directional excitation and exciton emission of 2D transition metal dichalcogenides (2D TMDs).
View Article and Find Full Text PDFACS Appl Mater Interfaces
March 2021
Metamaterials, rationally engineered composite materials with exotic properties, have provided unprecedented opportunities to manipulate the propagation of electromagnetic waves and control light-matter interactions in a prescribed manner. At present, most metamaterials are in solid states, and their functions are fixed once fabricated. Applying external electric fields to assemble metallic and metallodielectric particles into distinct configurations is an approach to realize dynamically tunable or reconfigurable metamaterials.
View Article and Find Full Text PDFWe present a theoretical study of directional light emission by dipole emitters near a spherical nanoparticle. Our analysis is extended from an exact electrodynamical approach for solving the coupling between a dipole and a sphere, providing a full picture of the directional emission for a complete set of combinations of variable emitters, particles, and their orientations. In particular, we show that the Mie resonances of a dielectric sphere are strongly influenced by the coupled dipole emitter, leading to the scattering properties that are different from the prediction by the standard Mie theory.
View Article and Find Full Text PDFSubwavelength nanostructures with tunable compositions and geometries show favorable optical functionalities for the implementation of nanophotonic systems. Precise and versatile control of structural configurations on solid substrates is essential for their applications in on-chip devices. Here, we report all-solid-phase reconfigurable chiral nanostructures with silicon nanoparticles and nanowires as the building blocks in which the configuration and chiroptical response can be tailored on-demand by dynamic manipulation of the silicon nanoparticle.
View Article and Find Full Text PDFMachine learning (ML) techniques, such as neural networks, have emerged as powerful tools for the inverse design of nanophotonic structures. However, this innovative approach suffers some limitations. A primary one is the nonuniqueness problem, which can prevent ML algorithms from properly converging because vastly different designs produce nearly identical spectra.
View Article and Find Full Text PDFBackground: Low plasma sodium concentration has been recognized as a prognostic factor in several disorders but never evaluated in sickle cell disease. The present study evaluates its value at admission to predict a complication in adult patients with sickle cell disease hospitalized for an initially uncomplicated acute painful episode.
Methods: The primary outcome of this retrospective study, performed between 2010 and 2015 in a French referral center for sickle cell disease, was a composite criterion including acute chest syndrome, intensive care unit transfer, red blood cell transfusion or inpatient death.
Longitudinal surface plasmon resonance (LSPR)-based optical signals possess unique advantages in biomolecular sensing and detection which can be attributed to their ultrahigh sensitivity and signal-to-noise ratio. However, the lack of effective strategies for morphological control of gold nanorods (GNRs) complicates the precise tuning of their LSPR property. Herein, a "peptide-encoded" strategy was first developed to precisely control the morphologies of GNRs via overgrowth of GNR seeds in the presence of thiol-containing peptides.
View Article and Find Full Text PDFNanophotonics has been an active research field over the past two decades, triggered by the rising interests in exploring new physics and technologies with light at the nanoscale. As the demands of performance and integration level keep increasing, the design and optimization of nanophotonic devices become computationally expensive and time-inefficient. Advanced computational methods and artificial intelligence, especially its subfield of machine learning, have led to revolutionary development in many applications, such as web searches, computer vision, and speech/image recognition.
View Article and Find Full Text PDFOptical manipulation of colloidal nanoparticles and molecules is significant in numerous fields. Opto-thermoelectric nanotweezers exploiting multiple coupling among light, heat, and electric fields enables the low-power optical trapping of nanoparticles on a plasmonic substrate. However, the management of light-to-heat conversion for the versatile and precise manipulation of nanoparticles is still elusive.
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