The wide utilization of lithium-ion batteries (LIBs) prompts extensive research on the anode materials with large capacity and excellent stability. Despite the attractive electrochemical properties of pure Si anodes outperforming other Si-based materials, its unsafety caused by huge volumetric expansion is commonly admitted. Silicon monoxide (SiO) anode is advantageous in mild volume fluctuation, and would be a proper alternative if the low initial columbic efficiency and conductivity can be ameliorated.
View Article and Find Full Text PDFThis study employed multifractal analysis to investigate the changes in surface morphology of SiO anti-reflective coatings prepared on KDP substrates using the sol-gel method, under various conditions of ultraviolet (UV) irradiance. The coatings were successfully fabricated, and the chemical structure of the SiO sol was comprehensively characterized using Solid-State Nuclear Magnetic Resonance (SSNMR) technology. Under low UV irradiance (4 J/cm), repeated experiments revealed a crack-induced mechanism of surface fatigue damage.
View Article and Find Full Text PDFRev Sci Instrum
January 2024
In x-ray imaging, the size of the x-ray tube light source significantly impacts image quality. However, existing methods for characterizing the size of the x-ray tube light source do not meet measurement requirements due to limitations in processing accuracy and mechanical precision. In this study, we introduce a novel method for accurately characterizing the size of the x-ray tube light source using spherical encoded imaging technology.
View Article and Find Full Text PDFNanomaterials (Basel)
June 2023
On-chip polarization control is in high demand for novel integrated photonic applications such as polarization division multiplexing and quantum communications. However, due to the sensitive scaling of the device dimension with wavelength and the visible-light absorption properties, traditional passive silicon photonic devices with asymmetric waveguide structures cannot achieve polarization control at visible wavelengths. In this paper, a new polarization-splitting mechanism based on energy distributions of the fundamental polarized modes in the r-TiO ridge waveguide is investigated.
View Article and Find Full Text PDFAiming to improve the spatial resolution of a neutron imaging system (NIS) for 14 MeV fusion neutrons, an ideal micron resolution capillary detector filled with a high optical index liquid scintillator was simulated. A threshold for each capillary pixel and a threshold for each cluster were applied to suppress the gamma-induced background. In addition, by using a pattern recognition algorithm and an optimized Hough transform, the accuracy of determining the neutron impinging positions and the dynamic range of this detector were enhanced.
View Article and Find Full Text PDFMetamaterials have gained much attention thanks to their extraordinary and intriguing optical properties beyond natural materials. However, universal high-resolution fabrications of 3D micro/nanometastructures with high-resolution remain a challenge. Here, a novel approach to fabricate sophisticated 3D micro/nanostructures with excellent robustness and precise controllability is demonstrated by simultaneously modulating of flexible resist stencils and basal molds.
View Article and Find Full Text PDFGraphene exhibits extraordinary opto-electronic properties due to its unique dynamic conductivity, bringing great value in optical sensing, surface plasmon modulation and photonic devices. Based on the polarization-sensitive absorption of graphene working at near infrared to ultraviolet wavelengths, we theoretically investigate the refractive index sensing and imaging mechanism under oblique and tight focusing incidences of light respectively. We demonstrate that such graphene-based methods can provide ultrahigh refractive index resolution (∼2.
View Article and Find Full Text PDFSimultaneous broadband and high efficiency merits of designer metasurfaces are currently attracting widespread attention in the field of nanophotonics. However, contemporary metasurfaces rarely achieve both advantages simultaneously. For the category of transmissive metadevices, plasmonic or conventional dielectric metasurfaces are viable for either broadband operation with relatively low efficiency or high efficiency at only a selection of wavelengths.
View Article and Find Full Text PDFACS Appl Mater Interfaces
June 2018
The confinement of light into nanometer-sized metallic nanogaps can lead to an extremely high field enhancement, resulting in dramatically enhanced absorption, emission, and surface-enhanced Raman scattering (SERS) of molecules embedded in nanogaps. However, low-cost, high-throughput, and reliable fabrication of ultra-high-dense nanogap arrays with precise control of the gap size still remains a challenge. Here, by combining colloidal lithography and atomic layer deposition technique, a reproducible method for fabricating ultra-high-dense arrays of hexagonal close-packed annular nanogaps over large areas is demonstrated.
View Article and Find Full Text PDFAluminium (Al)-doped zinc oxide (ZnO) nanowires (NWs) with a unique core-shell structure and a Δ-doping profile at the interface were successfully grown using a combination of chemical vapor deposition re-growth and few-layer AlO atomic layer deposition. Unlike the conventional heavy doping which degrades the near-band-edge (NBE) luminescence and increases the electron-phonon coupling (EPC), it was found that there was an over 20-fold enhanced NBE emission and a notably-weakened EPC in this type of interfacially Al-doped ZnO NWs. Further experiments revealed a greatly suppressed nonradiative decay process and a much enhanced radiative recombination rate.
View Article and Find Full Text PDFMetallic nanogap is very important for a verity of applications in plasmonics. Although several fabrication techniques have been proposed in the last decades, it is still a challenge to produce uniform nanogaps with a few nanometers gap distance and high throughput. Here we present a simple, yet robust method based on the atomic layer deposition (ALD) and lift-off technique for patterning ultranarrow nanogaps array.
View Article and Find Full Text PDFUnidirectional reflectionless phenomenon is reported in periodic ternary layered material (PTLM). The unit of the material is composed of two real dielectric layers and a complex medium (loss or gain) layer. The model is analyzed by coupled mode theory.
View Article and Find Full Text PDFMetasurfaces made of subwavelength resonators can modify the wave front of light within the thickness much less than free space wavelength, showing great promises in integrated optics. In this paper, we theoretically show that electric and magnetic resonances supported simultaneously by a subwavelength nanowire with high refractive-index can be utilized to design metasurfaces with near-unity transmittance. Taking silicon nanowire for instance, we design numerically a near-infrared quarter-waveplate with high transmittance using a subwavelength nanowire array.
View Article and Find Full Text PDFAbrupt phase shift introduced by plasmonic resonances has been frequently used to design subwavelength wave plates for optical integration. Here, with the sandwich structure consisting of a top periodic patterned silver nanopatch, an in-between insulator layer and a bottom thick Au film, we realize a broadband half-wave plate which is capable to cover entire visible light spectrum ranging from 400 to 780 nm. Moreover, when the top layer is replaced with a periodic array of composite super unit cell comprised of two nanopatches with different sizes, the operation bandwidth can be further improved to exceed an octave (400-830 nm).
View Article and Find Full Text PDFSurface plasmon modes originated from various metallic nanostructures possess unique features of strong nanoscale light confinement and enhancement with tunable energy, which make them attractive and promising for a variety of applications such as sensing, solar cell, and lasing. Here, we have investigated the interaction between localized and propagating surface plasmons in a structure consisting of a gold nanobar array and a thick gold film, separated by a silica dielectric spacer layer. It is found that the reflection spectrum of the designed plasmonic structure can be readily tailored by changing the gold nanobar size, array period and the spacer layer thickness.
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