Publications by authors named "Yangzhuo He"

Article Synopsis
  • Atom-site catalysts, particularly those based on graphitic carbon nitride, show great promise for water purification but face challenges in understanding their synthesis and properties.
  • This study investigates the effects of metal site coordination and structure on catalytic efficiency using various analytical techniques, revealing that a specific dual-site configuration (OCN Co/Fe) improves activation of peroxymonosulfate.
  • The resulting OCN-Co/Fe/PVDF composite membrane achieves high rejection efficiency for ciprofloxacin and maintains excellent performance over time, providing insights for future catalyst design.
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Article Synopsis
  • - Organic polymers, especially Schiff base networks (SNWs) with high nitrogen content, show promise in photocatalysis due to their affordability and ability to tailor structure for improved electron transfer.
  • - A series of SNWs were created using melamine units and dialdehydes, with tests revealing that SNW-o, made with o-phthalaldehyde, is effective in visible light, achieving significant tetracycline degradation rates.
  • - The research highlights how manipulating the molecular properties of organic photocatalysts can enhance their performance, suggesting a strategic approach for future applications in photocatalysis.
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In recent years, using semiconductor photocatalysts for antibiotic contaminant degradation under visible light has become a hot topic. Herein, a novel and ingenious cadmium-doped graphite phase carbon nitride (Cd-g-CN) photocatalyst was successfully constructed via the thermal polymerization method. Experimental and characterization results revealed that cadmium (Cd) was well doped at the g-CN surface and exhibited high intercontact with g-CN.

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MOF-derived multi-metal nanomaterials are attracting numerous attentions in widespread applications such as catalysis, sensors, energy storage and conversion, and environmental remediation. Compared to the monometallic counterparts, the presence of foreign metal is expected to bring new physicochemical properties, thus exhibiting synergistic effect for enhanced performance. MOFs have been proved as a good platform for the fabrication of polymetallic nanomaterials with requisite features.

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Organic semiconductors have been recognized as a new generation of photocatalysts for pollutants degradation and energy production. Herein, organic heterojunction (TpMa/CN) consisting of carbon nitride and β-ketoenamine-based covalent organic framework is fabricated via a controllable self-assembly approach. The as-prepared TpMa/CN heterojunctions show enlarged visible-light absorption.

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To develop efficient catalysts is one of the major ways to solve the energy and environmental problems. Spinel ferrites, with the general chemical formula of MFeO (where M = Mg, Co, Ni, Zn, Fe, Mn, etc.), have attracted considerable attention in catalytic research.

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Antibiotic residues in soil may cause potential risks to human health and soil ecosystems. To avoid these potential risks, comprehensive study of the adsorption, transport and biodegradation of antibiotics in soil is very imperative. This review provided current views about the most recent studies, which have been conducted toward the adsorption, transport and biodegradation of antibiotics in soil.

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As a widely used antibiotic, tetracycline has a huge hidden danger to human health. Municipal sludge rich in organic substances has the potential to produce biochar. In this work, the municipal sludge biochar from solid waste was modified by the alkali-acid binding method, and tetracycline was efficiently removed from the aqueous solution, the adsorption removal efficiency reached to 86% at initial concentration of 200 mg/L.

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Persulfate is the latest oxidant which is being used increasingly for the remediation of groundwater and soil contaminated with organic compounds. It is of great significant to offer readers a general summary about different methods of activating persulfate, mainly including heat-activated, metal ions-activated, UV-activated, and alkaline-activated. Meanwhile, in addition to persulfate concentration as an influencing factor for persulfate oxidation process, selected information like temperature, anions, cations, pH, and humic acid are presented and discussed.

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In this study, the oxidized multiwalled carbon nanotube (O-MWCNTs) was obtained by a simple method, and investigated by various techniques (SEM, TEM, FT-IR, XPS and zeta potential) for the removal of pefloxacin and Cu(II). The mutual effects of their adsorption onto O-MWCNTs were comprehensively clarified with sole and binary systems with adsorption kinetics, sorption thermodynamic and sorption isotherm models. The results indicated that there are site enhancement and competition of pefloxacin and Cu(II) on O-MWCNTs.

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Selenium (Se) contamination in surface and ground water in numerous river basins has become a critical problem worldwide in recent years. The exposure to Se, either direct consumption of Se or indirectly may be fatal to the human health because of its toxicity. The review begins with an introduction of Se chemistry, distribution and health threats, which are essential to the remediation techniques.

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A significant amount of antimony (Sb) enters into the environment every year because of the wide use of Sb compounds in industry and agriculture. The exposure to Sb, either direct consumption of Sb or indirectly, may be fatal to the human health because both antimony and antimonide are toxic. Firstly, the introduction of Sb chemistry, distribution and health threats are presented in this review, which is essential to the removal techniques.

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