Unambiguous identification of low concentration chemical mixtures can be performed by broadband enhanced infrared absorption (BEIRA). Here we propose and numerically study a corrugated parallel plate waveguide (CPPW) with gradient grooves which is capable of directly converting transmission modes to surface plasmon modes and could hence serve as a powerful chemical sensor. Such a waveguide can be designed to exhibit a wide pass band covering an extended portion of a molecule absorption spectrum.
View Article and Find Full Text PDFHybrid plasmonic metal-graphene systems are emerging as a class of optical metamaterials that facilitate strong light-matter interactions and are of potential importance for hot carrier graphene-based light harvesting and active plasmonic applications. Here we use femtosecond pump-probe measurements to study the near-field interaction between graphene and plasmonic gold nanodisk resonators. By selectively probing the plasmon-induced hot carrier dynamics in samples with tailored graphene-gold interfaces, we show that plasmon-induced hot carrier generation in the graphene is dominated by direct photoexcitation with minimal contribution from charge transfer from the gold.
View Article and Find Full Text PDFThe small size of plasmonic nanostructures compared to the wavelength of light is one of their most distinct and defining characteristics. It results in the strong compression of an incident wave to intense hot spots which have been used most remarkably for molecular sensing and nanoscale lasers. But another important direction for research is to use this ability to design miniaturized interconnects and modulators between fast, loss-less photonic components.
View Article and Find Full Text PDFStrongly anisotropic media, where the principal components of the dielectric tensor have opposite signs, are called hyperbolic. Such materials exhibit unique nanophotonic properties enabled by the highly directional propagation of slow-light modes localized at deeply sub-diffractional length scales. While artificial hyperbolic metamaterials have been demonstrated, they suffer from high plasmonic losses and require complex nanofabrication, which in turn induces size-dependent limitations on optical confinement.
View Article and Find Full Text PDFWave interference is a fundamental physical phenomenon. Traditionally, the coherent effect of two identical point sources only takes place when the optical path is an integer number of wavelengths. In this paper, we show that mu and epsilon near zero (MENZ) metamaterials can be used to realize a perfectly constructive and isotropic interference.
View Article and Find Full Text PDFIt is demonstrated herein both theoretically and experimentally that Young's interference can be observed in plasmonic structures when two or three nanoparticles with separation on the order of the wavelength are illuminated simultaneously by a plane wave. This effect leads to the formation of intermediate-field hybridized modes with a character distinct of those mediated by near-field and/or far-field radiative effects. The physical mechanism for the enhancement of absorption and scattering of light due to plasmonic Young's interference is revealed, which we explain through a redistribution of the Poynting vector field and the formation of near-field subwavelength optical vortices.
View Article and Find Full Text PDFPlasmonics provides great promise for nanophotonic applications. However, the high optical losses inherent in metal-based plasmonic systems have limited progress. Thus, it is critical to identify alternative low-loss materials.
View Article and Find Full Text PDFIn this article, we use optical transmission spectroscopy to measure the changes in the resonance features of a Au plasmonic nanoresonator array consisting of concentric ring/disc cavity elements, when graphene is introduced as an encapsulating medium. We show that by using finite element modelling to best reproduce our experimental results the dielectric response of the graphene film can be determined. We discuss the potential of such structures for chemical sensing applications.
View Article and Find Full Text PDFWe show in detail how a derivation of Fano theory can serve as a new paradigm to study, understand, and control the interaction of nano-objects with light. Examples include a plasmonic crystal, a dolmen-type structure sustaining dark and bright plasmon modes, and a nanoshell heptamer. On the basis of only three coupling factors, a straightforward analytical formula is obtained, only assuming a plasmonic resonance for the continuum, and retaining the nonclassical character of the original formalism.
View Article and Find Full Text PDFThe interaction between plasmonic resonances, sharp modes, and light in nanoscale plasmonic systems often leads to Fano interference effects. This occurs because the plasmonic excitations are usually spectrally broad and the characteristic narrow asymmetric Fano line-shape results upon interaction with spectrally sharper modes. By considering the plasmonic resonance in the Fano model, as opposed to previous flat continuum approaches, here we show that a simple and exact expression for the line-shape can be found.
View Article and Find Full Text PDF