Dynamics of Polar Vortex Crystallization.

Vortex crystals are commonly observed in ultrathin ferroelectrics. However, a clear physical picture of origin of this topological state is currently lacking. Here, we show that vortex crystallization in ultrathin Pb(Zr_{0.

Dynamical Control of Topology in Polar Skyrmions via Twisted Light.

Twisted light carries a nonzero orbital angular momentum, that can be transferred from light to electrons and particles ranging from nanometers to micrometers. Up to now, the interplay between twisted light with dipolar systems has scarcely been explored, though the latter bear abundant forms of topologies such as skyrmions and embrace strong light-matter coupling. Here, using first-principles-based simulations, we show that twisted light can excite and drive dynamical polar skyrmions and transfer its nonzero winding number to ferroelectric ultrathin films.

Motion and teleportation of polar bubbles in low-dimensional ferroelectrics.

Electric bubbles are sub-10nm spherical vortices of electric dipoles that can spontaneously form in ultra-thin ferroelectrics. While the static properties of electric bubbles are well established, little to nothing is known about the dynamics of these particle-like structures. Here, we reveal pathways to realizing both the spontaneous and controlled dynamics of electric bubbles in ultra-thin Pb(ZrTi)O films.

Quantum criticality at cryogenic melting of polar bubble lattices.

Quantum fluctuations (QFs) caused by zero-point phonon vibrations (ZPPVs) are known to prevent the occurrence of polar phases in bulk incipient ferroelectrics down to 0 K. On the other hand, little is known about the effects of QFs on the recently discovered topological patterns in ferroelectric nanostructures. Here, by using an atomistic effective Hamiltonian within classical Monte Carlo (CMC) and path integral quantum Monte Carlo (PI-QMC), we unveil how QFs affect the topology of several dipolar phases in ultrathin Pb(ZrTi)O (PZT) films.

Dynamical Multiferroicity and Magnetic Topological Structures Induced by the Orbital Angular Momentum of Light in a Nonmagnetic Material.

Recent studies have revealed that chiral phonons resonantly excited by ultrafast laser pulses carry magnetic moments and can enhance the magnetization of materials. In this work, using first-principles-based simulations, we present a real-space scenario where circular motions of electric dipoles in ultrathin two-dimensional ferroelectric and nonmagnetic films are driven by orbital angular momentum of light via strong coupling between electric dipoles and optical field. Rotations of these dipoles follow the evolving pattern of the optical field and create strong on-site orbital magnetic moments of ions.