Objective: This study aims to evaluate the relationship between the pericoronary fat attenuation index (FAI), derived from coronary artery computed tomography angiography, and post-lipid management levels of low-density lipoprotein cholesterol in patients with coronary artery disease (CAD). Additionally, the study investigates coronary inflammation across different lipid management strategies.
Methods: We selected a cohort comprising 521 CAD patients who met the inclusion criteria.
Hypoxic pulmonary hypertension (HPH) is one of the important pathophysiological changes in chronic pulmonary heart disease. Hypoxia promotes the phenotypic transformation of pulmonary artery smooth muscle cells (PASMCs). Extracellular exosomes regulate vascular smooth muscle cell (VSMC) phenotypic switch.
View Article and Find Full Text PDFBackground: In many clinical situations, it is critical to exclude or identify abnormally lymph nodes (LNs). The nature of superficial abnormally LNs is closely related to the stage, treatment, and prognosis of the disease. Ultrasound (US) is an important method for examining superficial LNs due to its cheap and safe characteristics.
View Article and Find Full Text PDFIEEE Trans Neural Netw Learn Syst
May 2024
With the rapid advances in digital imaging and communication technologies, recently image set classification has attracted significant attention and has been widely used in many real-world scenarios. As an effective technology, the class-specific representation theory-based methods have demonstrated their superior performances. However, this type of methods either only uses one gallery set to measure the gallery-to-probe set distance or ignores the inner connection between different metrics, leading to the learned distance metric lacking robustness, and is sensitive to the size of image sets.
View Article and Find Full Text PDFDevelopment of highly porous carbons with abundant surface functionalities and well-defined nanostructure is of significance for many important electrochemical energy storage systems. However, porous carbons suffer from a compromise between porosity, doped functionality, and nanostructure that have thus far restricted their performances. Here, we report the design of highly porous, nitrogen-enriched hollow carbon nanospheres (PN-HCNs) by an interfacial copolymerization strategy followed by NH-assisted carbonization, and further demonstrate their significance and effectiveness in enhancing the electrochemical performances.
View Article and Find Full Text PDFACS Appl Mater Interfaces
August 2019
Lithium metal is considered to be a holy grail of the battery anode chemistry due to its large specific capacity. Nevertheless, the uncontrollable formation of lithium dendrites resulting from uneven lithium nucleation/growth and the associated safety risk and short cyclability severely impede the practical use of lithium metal anodes. Herein, we demonstrate a highly lithiophilic cobalt nitride nanobrush on a Ni foam (CoN/NF) current collector as a stable three-dimensional (3D) framework to inhibit the dendrite formation of lithium.
View Article and Find Full Text PDFGiven their low cost and eco-friendliness, rechargeable Zn-ion batteries (ZIBs) have received increasing attention as a device with great potential for large-scale energy storage. However, the development of ZIBs with high capacities and long lifespans is challenging because of the dendritic growth of Zn and the absence of suitable cathode materials. Herein, we report a novel rechargeable aqueous Zn-ion battery (AZIB) that consist of Zn coated with reduced graphene oxide as the anode and VO·HO/rGO composite as the cathode.
View Article and Find Full Text PDFTwo-dimensional (2D) SnS materials represent a class of high-capacity candidates as anodes of Li-ion batteries (LIBs); however, they are limited by inferior rate and cycling performance. Herein, we demonstrate unique triaxial nanocables of conducting polypyrrole@SnS@carbon nanofiber (PPy@SnS@CNF) prepared via a facile combination of hydrothermal method and vapor-phase polymerization. The PPy@SnS@CNF manifests a strong synergistic effect from its hierarchical nanoarchitecture, which provides enlarged electrode/electrolyte contact interfaces, highly electrical conductive pathways, sufficient electrolyte ingress/transport channels, and an intimate mechanical/electrochemical safeguard for fast electrode kinetics and good structural stability.
View Article and Find Full Text PDFHierarchically porous carbon nanomaterials with well-defined architecture can afford a promising platform for effectively addressing energy and environmental concerns. Herein, a totally green and straightforward synthesis strategy for the fabrication of hierarchically porous carbon nanotubes (HPCNTs) by a simple carbonization treatment without any assistance of soft/hard templates and activation procedures is demonstrated. A high specific surface area of 1419 m g and hierarchical micro-/meso-/macroporosity can be achieved for the HPCNTs.
View Article and Find Full Text PDFAu-decorated TiO hollow spheres (Au-THS) have been successfully synthesized via a facile one-pot solvothermal method. The Au-THS hybrid features unique hollow structure with a large specific surface area of 120 m g and homogeneous decoration of Au nanoparticles, giving rise to enhanced light harvesting and charge generation/separation efficiency. When incorporated into the active layer of dye-sensitized solar cells (DSSCs), an improved power conversion efficiency of 7.
View Article and Find Full Text PDFA low-cost bio-mass-derived carbon substrate has been employed to synthesize MoS₂@carbon composites through a hydrothermal method. Carbon fibers derived from natural cotton provide a three-dimensional and open framework for the uniform growth of MoS₂ nanosheets, thus hierarchically constructing coaxial architecture. The unique structure could synergistically benefit fast Li-ion and electron transport from the conductive carbon scaffold and porous MoS₂ nanostructures.
View Article and Find Full Text PDFACS Appl Mater Interfaces
February 2017
As a promising Li-metal battery, Li-S battery has an ultrahigh theoretical energy density of 2600 Wh kg. However, most of the previous work has mainly focused on tackling the "polysulfide shuttle" originating from the S cathode, while the dendrite problem coming from the Li-metal anode has often been overlooked. Herein, to solve the issues arising from both the cathode and anode simultaneously, we propose a novel cell configuration for the first time by inserting CNT films on both sides of the separator in Li-S batteries, in which the cathode-side CNT film works as a shield to suppress the "polysulfide shuttle" and the anode-side CNT film acts as a powerful shield to prevent the Li dendrite growth.
View Article and Find Full Text PDFACS Appl Mater Interfaces
October 2016
Owing to its ultrahigh specific capacity and low electrochemical potential, lithium (Li) metal is regarded as one of the most attractive anode materials for next-generation lithium batteries. Nevertheless, the commercialization of Li-metal-based rechargeable batteries (LiMBs) has been retarded by the uncontrollable growth of Li dendrites, as well as the resulting poor cycle stability and safety hazards. In this work, a 3D graphene@Ni scaffold has been proposed to accomplish dendrite-free Li deposition via structural and interfacial synergistic effects.
View Article and Find Full Text PDFAdvanced electrode design is crucial in the rapid development of flexible energy storage devices for emerging flexible electronics. Herein, we report a rational synthesis of graphene/Mn3O4 nanocomposite membranes with excellent mechanical flexibility and Li-ion storage properties. The strong interaction between the large-area graphene nanosheets and long Mn3O4 nanowires not only enables the membrane to endure various mechanical deformations but also produces a strong synergistic effect of enhanced reaction kinetics by providing enlarged electrode/electrolyte contact area and reduced electron/ion transport resistance.
View Article and Find Full Text PDFSeries of catalysts made of Pt nanoparticles supported on reduced graphene oxides (Pt/RGO) were synthesized and tested in methanol oxidation reaction, aiming for optimizing the mass-specific activity of prepared Pt/RGO composites. The loading amount of Pt is controlled through setting different reaction time and determined precisely by atomic absorption spectrophotometer. The structure of Pt/RGO composites is characterized by X-ray diffraction, transmission electron microscopy and Raman spectroscopy.
View Article and Find Full Text PDFDepression is a multicausal disorder and has been associated with metabolism regulation and immuno-inflammatory reaction. The anorectic molecule nesfatin-1 has recently been characterized as a potential mood regulator, but its precise effect on depression and the possible mechanisms remain unknown, especially when given peripherally. In the present study, nesfatin-1 was intraperitoneally injected to the rats and the depression-like behavior and activity of the hypothalamic-pituitary-adrenal (HPA) axis were evaluated.
View Article and Find Full Text PDFNesfatin-1, a newly discovered satiety peptide, has recently been reported to be involved in the stress response. Stress-induced expression of nesfatin-1 has been reported and few studies focus on its expression in the hypothalamus, which is the center of the stress response. To test our hypothesis that peripheral and hypothalamic nesfatin-1 overexpression should play an important role in the stress response and the associated hyperactivity of hypothalamic-pituitary-adrenal (HPA) axis, acute stress (AS) was induced using water avoidance stress (WAS), and chronic unpredictable mild stress (CUMS) was also induced using 3 consecutive weeks of 7 different stressors.
View Article and Find Full Text PDFHigh lithium salt concentration strategy has been recently reported to be an effective method to enable various organic solvents as electrolyte of Li-ion batteries. Here, we utilize in situ atomic force microscopy (AFM) to investigate the interfacial morphology on the graphite electrode in dimethyl sulfoxide (DMSO)-based electrolyte of various concentrations. The significant differences in interfacial features of the graphite in electrolytes of different concentrations are revealed.
View Article and Find Full Text PDFSilicon nanowires (SiNWs) have attracted great attention as promising anode materials for lithium ion batteries (LIBs) on account of their high capacity and improved cyclability compared with bulk silicon. The interface behavior, especially the solid electrolyte interphase (SEI), plays a significant role in the performance and stability of the electrodes. We report herein an in situ single nanowire atomic force microscopy (AFM) method to investigate the interface electrochemistry of silicon nanowire (SiNW) electrode.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
December 2014
The construction of a spatially defined assembly of molecular building blocks, especially in the vertical direction, presents a great challenge for surface molecular engineering. Herein, we demonstrate that an electric field applied between an STM tip and a substrate triggered the formation of a bilayer structure at the solid-liquid interface. In contrast to the typical high electric-field strength (10(9) V m(-1) ) used to induce structural transitions in supramolecular assemblies, a mild electric field (10(5) V m(-1) ) triggered the formation of a bilayer structure of a polar molecule on top of a nanoporous network of trimesic acid on graphite.
View Article and Find Full Text PDFA facile protocol is developed for the direct observation and characterization of a single particle electrode during the lithium ion battery operation by using in situ AFM. The SEI formation on the LiNi0.5Mn1.
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