Enhanced continuous atmospheric water harvesting with scalable hygroscopic gel driven by natural sunlight and wind.

Sorption-based atmospheric water harvesting (SAWH) has received unprecedented attention as a future water and energy platform. However, the water productivity of SAWH systems is still constrained by the slow sorption kinetics at material and component levels and inefficient condensation. Here, we report a facile method to prepare hygroscopic interconnected porous gel (HIPG) with fast sorption-desorption kinetics, high scalability and stability, and strong adhesion property for highly efficient SAWH.

Curriculum learning for ab initio deep learned refractive optics.

Deep optical optimization has recently emerged as a new paradigm for designing computational imaging systems using only the output image as the objective. However, it has been limited to either simple optical systems consisting of a single element such as a diffractive optical element or metalens, or the fine-tuning of compound lenses from good initial designs. Here we present a DeepLens design method based on curriculum learning, which is able to learn optical designs of compound lenses ab initio from randomly initialized surfaces without human intervention, therefore overcoming the need for a good initial design.

Aberration-Aware Depth-From-Focus.

Computer vision methods for depth estimation usually use simple camera models with idealized optics. For modern machine learning approaches, this creates an issue when attempting to train deep networks with simulated data, especially for focus-sensitive tasks like Depth-from-Focus. In this work, we investigate the domain gap caused by off-axis aberrations that will affect the decision of the best-focused frame in a focal stack.

Highly Chemoselective Ni-Catalyzed Protecting-Group-Free 2,2'-Biphenol Synthesis and Mechanistic Insights.

The utilization of readily available starting materials to produce useful molecules is often challenged by selectivity issues. In this study, a Ni-catalyzed protecting-group-free C-C coupling protocol is described for the efficient synthesis of 2,2'-biphenol derivatives. Its remarkable chemoselectivity control ability, wide substrate scope, and excellent functional group tolerance highlight this newly developed strategy.

Coherent Manipulation with Resonant Excitation and Single Emitter Creation of Nitrogen Vacancy Centers in 4H Silicon Carbide.

Silicon carbide (SiC) has become a key player in the realization of scalable quantum technologies due to its ability to host optically addressable spin qubits and wafer-size samples. Here, we have demonstrated optically detected magnetic resonance (ODMR) with resonant excitation and clearly identified the ground state energy levels of the NV centers in 4H-SiC. Coherent manipulation of NV centers in SiC has been achieved with Rabi and Ramsey oscillations.

HfS/MoTe vdW heterostructure: bandstructure and strain engineering based on first-principles calculation.

In this study, a multilayered van der Waals (vdW) heterostructure, HfS/MoTe, was modeled and simulated using density functional theory (DFT). It was found that the multilayers (up to 7 layers) are typical indirect bandgap semiconductors with an indirect band gap varying from 0.35 eV to 0.