On-chip light sources are an essential component of scalable photonic integrated circuits (PICs), and coupling between light sources and waveguides has attracted a great deal of attention. Photonic waveguides based on bound states in the continuum (BICs) allow optical confinement in a low-refractive-index waveguide on a high-refractive-index substrate and thus can be employed for constructing PICs. In this work, we experimentally demonstrated that the photoluminescence (PL) from a monolayer of tungsten sulfide (WS) could be coupled into a BIC waveguide on a lithium-niobate-on-insulator (LNOI) substrate.
View Article and Find Full Text PDFInterlayer electronic coupling in two-dimensional materials enables tunable and emergent properties by stacking engineering. However, it also results in significant evolution of electronic structures and attenuation of excitonic effects in two-dimensional semiconductors as exemplified by quickly degrading excitonic photoluminescence and optical nonlinearities in transition metal dichalcogenides when monolayers are stacked into van der Waals structures. Here we report a van der Waals crystal, niobium oxide dichloride (NbOCl), featuring vanishing interlayer electronic coupling and monolayer-like excitonic behaviour in the bulk form, along with a scalable second-harmonic generation intensity of up to three orders higher than that in monolayer WS.
View Article and Find Full Text PDFSingle photon emitters (SPEs) are critical components of photon-based quantum technology. Recently, the interaction between surface plasmons and emitters has attracted increasing attention because of its potential to improve the quality of single-photon sources through stronger light-matter interactions. In this work, we use a hybrid plasmonic probe composed of a fiber taper and silver nanowire to controllably modulate the radiation properties of SPEs with differently oriented polarization.
View Article and Find Full Text PDFAs an important degree of freedom (d.o.f.
View Article and Find Full Text PDFBoosting second-order optical nonlinear frequency conversion over subwavelength thickness has long been pursued through optical resonance in micro- and nanophotonics. However, the availability of thin film materials with high second-order nonlinearity is limited to III-V semiconductors, which have low transparency in the visible. Here, we experimentally demonstrated strongly enhanced second harmonic generation in one-dimensional heterostructure cavities on thin film lithium niobate.
View Article and Find Full Text PDFSilver nanowires (AgNWs), as one of the most important plasmonic waveguides, can support several different plasmonic modes. These surface plasmon polariton (SPP) modes have different electric field distributions, effective mode areas, propagation lengths and losses and thus can be used for different applications, from efficiently collecting single photons to carrying quantum entanglement. Therefore, the excitation and analysis of these different SPP modes are of pivotal importance for the development of subwavelength optical devices.
View Article and Find Full Text PDFDesigning high-efficiency catalyst is at the heart of a transition to future renewable energy systems. Great achievements have been made to optimize thermodynamics to reduce energetic barriers of the catalytic reactions. However, little attention has been paid to design catalysts to improve kinetics to enrich the local concentration of reactant molecules surrounding electrocatalysts.
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