Ultraviolet photodetectors (UV PDs) based on microcrystals (MCs) have attracted extensive attention due to their outstanding detection performance. Nevertheless, precise manipulation of the MCs still remains challenging, which may hinder the mass processing and performance improvement of the UV PDs. In this work, a single high-quality CsCuI MC that had a special X-shaped morphology was demonstrated to be successfully manipulated to prepare high-performance UV PDs by virtue of optical focusing, probe micromanipulation, and direct-write photolithography techniques.
View Article and Find Full Text PDFACS Appl Mater Interfaces
May 2024
Recently, the FeOCl-type two-dimensional materials have attracted significant attention owing to their versatile applications in fields such as thermoelectricity and photocatalysis. This study aims to systematically investigate the thermoelectric properties of ScSX (X = Cl, Br, and I) monolayers by a combination of the first-principles calculations and the machine-learning interatomic potential approach. These monolayers are indirect semiconductors with band gaps of 3.
View Article and Find Full Text PDFFirmness, soluble solid content (SSC) and titratable acidity (TA) are characteristic substances for evaluating the quality of cherry tomatoes. In this paper, a hyper spectral imaging (HSI) system using visible/near-infrared (Vis-NIR) and near-infrared (NIR) was proposed to detect the key qualities of cherry tomatoes. The effects of individual spectral information and fused spectral information in the detection of different qualities were compared for firmness, SSC and TA of cherry tomatoes.
View Article and Find Full Text PDFCesium copper halide perovskite is one of the promising materials for solar-blind light detection. However, most of the cesium copper halide perovskite-based photodetectors (PDs) are focused on ultraviolet A detection and realized on the rigid substrate in the single device configuration. Here, a flexible solar-blind PDs array (10 × 10 pixels) based on the CsCu I film patterns for ultraweak light sensing and light distribution imaging is reported.
View Article and Find Full Text PDFAs versatile energy harvesters, triboelectric nanogenerators (TENGs) have attracted considerable attention in developing portable and self-powered energy suppliers. The question of how to improve the output power of TENGs using cost-effective means is still under vigorous investigation. In this paper, high-output TENGs were successfully produced by using a simple and low-cost lotus-leaf-bionic (LLB) method.
View Article and Find Full Text PDFACS Appl Mater Interfaces
September 2022
Halide perovskites featuring remarkable optoelectronic properties hold great potential for threshold switching devices (TSDs) that are of primary importance to next-generation memristors and neuromorphic computers. However, such devices are still in their infancy due to the unsolved challenges of high threshold voltage, poor stability, and lead-containing features. Herein, a unipolar TSD based on an all-inorganic halide perovskite of CsCuI is demonstrated, exhibiting the fascinating attributes of a low threshold voltage of 0.
View Article and Find Full Text PDFImage analysis is a useful technique to evaluate the efficacy of a treatment for weed control. In this study, we address two practical challenges in the image analysis. First, it is challenging to accurately quantify the efficacy of a treatment when an entire experimental unit is not affected by the treatment.
View Article and Find Full Text PDFVoltage control of room-temperature ferromagnetism has remained a big challenge which will greatly influence the multifunctional memory devices. In this paper, porous TiO thin films were deposited by dc-reactive magnetron sputtering onto ordered porous anodic alumina (PAA) substrates. Voltage-driving room-temperature resistance and magnetization switching without external magnetic field are simultaneously found in an Ag/TiO/PAA/Al (Ag/TP/Al) device.
View Article and Find Full Text PDFChem Commun (Camb)
April 2019
Low-dimensional, lead-free, and cuprous-based halide compounds of Cs3Cu2Br5 micro-rods and CsCuBr2 micro-crosses (MCs) were synthesized via a simple solution method. The CsCuBr2 MCs were quite stable in air. Distinct green electroluminescence at 527 nm originating from CsCuBr2 MCs was observed at a low driving voltage of less than 3 V.
View Article and Find Full Text PDFA strategy to realize ZnO-based near-white-light electroluminescence (EL) was proposed by utilizing and regulating the intrinsic defect-related emissions of solution-processed ZnO nanocrystals (NCs). Prototype near-white light-emitting diodes (LEDs) based upon this strategy were demonstrated by using n-ZnO NCs/n-Si isotype heterojunctions. The emission color of the n-ZnO NCs/n-Si isotype heterojunction LEDs was tuned toward near white by using an Al-doped ZnO (AZO) spectral "scissor" which can tailor the green light more severely, rather than the blue or red light.
View Article and Find Full Text PDFZnO/GaN-based light-emitting diodes (LEDs) with improved asymmetric double heterostructure of Ta₂O₅/ZnO/HfO₂ have been fabricated. Electroluminescence (EL) performance has been enhanced by the HfO₂ electron blocking layer and further improved by continuing inserting the Ta₂O₅ hole blocking layer. The origins of the emission have been identified, which indicated that the Ta₂O₅/ZnO/HfO₂ asymmetric structure could more effectively confine carriers in the active i-ZnO layer and meanwhile suppresses of radiation from GaN.
View Article and Find Full Text PDFLight-emitting diodes (LEDs) based on n-ZnO@i-MgO core-shell (CS) nanowires (NWs) are herein demonstrated and characterized. MgO insulating layers were rationally introduced as shells to modify/passivate the surface defects of ZnO NWs. A high-quality ZnO/MgO interface was attained and the optically pumped near-band-edge emission of the bare ZnO NWs was greatly enhanced after cladding i-MgO shells.
View Article and Find Full Text PDFIn this paper, layered ZnO nanowall networks were directly grown on Al substrates using a hydrothermal method without predepositing seed layers. The individual ZnO nanowalls with a thickness of several nanometers and a size of several hundred nanometers were (002) surface dominated, in which the preferential growth direction of ZnO was suppressed. White electroluminescence devices were fabricated based on Au/polymethylmethacrylate/ZnO-nanowall (metal-insulator-semiconductor) structures.
View Article and Find Full Text PDFHigh-quality Mn:ZnO (MZO) film had been prepared on N-GaN coated sapphire substrates followed by postdeposition thermal annealing treatment at 700 °C. For the annealed MZO/GaN heterojunction, a 15 nm cubic structural ZnGa(2)O(4) layer was observed at the MZO/GaN interface through transmission electron microscope analysis. Through electroluminescence (EL) measurement, the formation of the nanointerface results in an EL transition from ultraviolet- to red-dominant mode for n-Mn:ZnO/N-GaN heterojunction light-emitting diodes (LEDs).
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