Publications by authors named "Xiansheng Li"

Room temperature (RT) synthesized mixed bromine and chlorine CsPbBrCl perovskite quantum dots (Pe-QDs) offer notable advantages for blue quantum dot light-emitting diodes (QLEDs), such as cost-effective processing and narrow luminescence peaks. However, the efficiency of blue QLEDs using these RT-synthesized QDs has been limited by inferior crystallinity and deep defect presence. In this study, we demonstrate a precise approach to constructing high-quality gradient core-shell (CS) structures of CsPbBrCl QD through anion exchange.

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The heat generation of the human body dramatically varies between resting and active status, so dynamic heat dissipation is required to ensure optimal thermal comfort. Herein, we propose a spectrally self-adaptive smart fabric (SSSF) by covering polyester fabric with silver nanowires, which autonomously adjusts its emissivity in response to the body's movement status from dry to wet states. During periods of inactivity, the SSSF maintains radiative heat insulation with a low emissivity state of 0.

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Introduction: Breeding rice with drought tolerance for harsh environments is crucial for agricultural sustainability. Understanding the genetic underpinnings of drought tolerance is vital for developing resilient rice varieties. Genome-wide association studies (GWAS) have emerged as pivotal tools in unravelling the complex genetic architecture of traits like drought tolerance, capitalizing on the natural genetic diversity within rice germplasm collections.

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  • Researchers have developed a new strategy to convert environmental energy into electricity for powering off-grid electronics throughout the day and night, overcoming limitations of traditional solar panels.
  • This approach combines daytime solar energy and nighttime cooling using a special thermoelectric generator (TEG) with a dynamic coating, improving energy efficiency significantly.
  • The system shows impressive results with power generation rates of over 1000 mW/m² during the day and 25 mW/m² at night, marking substantial increases compared to traditional methods and promoting sustainable energy use.
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Cu-based catalysts possess great potential in the electrocatalytic nitrate (NO) reduction reaction for ammonia (NH) synthesis. However, the low atomic economy limits their further application. Here we report a Cu single-atom (SA) incorporated in nitrogen-doped carbon (Cu SA/NC) with high atomic economy, which exhibits superior NH Faradaic efficiency (FE) of 100% along with an impressive NH yield rate of 7480 μg h mg.

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Passive radiative cooling is an energy-free cooling method by exchanging thermal radiation with the cold universe through the transparent atmospheric window. Spectrum tailoring of the radiative cooler is the key to daytime radiative cooling in previously reported works. In addition, radiative coolers with large-scale fabrication and self-cleaning characteristics should be further developed to improve their industrial applicability.

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Perovskite quantum dot light-emitting diodes (Pe-QLEDs) have been shown as promising candidates for next-generation displays and lightings due to their unique feature of wide color gamut and high color saturation. Hole-transporting materials (HTMs) play crucial roles in the device performance and stability of Pe-QLEDs. However, small-molecule HTMs have been less studied in Pe-QLEDs due to their poor solvent resistance and low hole mobility.

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  • The study introduces a novel device using vanadium dioxide (VO) that can adaptively switch between solar thermal energy collection during the day and radiative cooling at night, addressing energy and environmental challenges.
  • The device leverages the unique phase transition properties of VO to achieve a wide range of infrared emissivity, allowing continuous and efficient energy harvesting.
  • Potential applications for this technology include thermal management for spacecraft, infrared camouflage, and adaptive optical devices, highlighting its versatility beyond just energy harvesting.
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Hydrogen spillover from metal nanoparticles to oxides is an essential process in hydrogenation catalysis and other applications such as hydrogen storage. It is important to understand how far this process is reaching over the surface of the oxide. Here, we present a combination of advanced sample fabrication of a model system and in situ X-ray photoelectron spectroscopy to disentangle local and far-reaching effects of hydrogen spillover in a platinum-ceria catalyst.

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Perovskite quantum-dot-based light-emitting diodes (QLEDs) are highly promising for future solid-state lightings and high-definition displays due to their excellent color purity. However, their device performance is easily affected by charge accumulation induced luminescence quenching due to imbalanced charge injection in the devices. Here we report green perovskite QLEDs with simultaneously improved efficiency and operational lifetime through balancing the charge injection with the employment of a bilayered electron transport structure.

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  • A new study revealed that calcium and arsenic together significantly enhance the performance of a CeO-WO catalyst used in reducing nitrogen oxides (NO) with ammonia (NH) at high temperatures.
  • The catalyst achieved up to 89% NO conversion at 350 °C, influencing its structure, surface acidity, and redox properties, as analyzed through various techniques like XRD and XPS.
  • The findings indicated that the interaction between cerium and arsenic improved the catalyst's effectiveness by restoring key acid sites and oxygen defects, with the observed drop in performance linked to reduced surface area and changes in particle structure.
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  • Chlorobenzene (CB) decreases the effectiveness of V-based catalysts in selective catalytic reduction (SCR) at low temperatures, even with low levels of CB adsorbed.
  • The oxidation of CB breaks the C-Cl bond, which leads to increased ammonia (NH) adsorption due to the release of Cl ions that create additional Brønsted acid sites.
  • The presence of Ce and Mn enhances the dechlorination process, resulting in an increased formation of inactive NHCl on the catalyst surface.
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An actinomycete strain, H41-55 from sea sediment was identified as Streptomyces antibiotic on the basis of its morphological, physiological and biochemical characteristics as well as 16S rDNA data. A new secondary metabolite, (2S,3R)-N-[3-(formylamino)-2-hydroxybenzoyl]-l-threonine propyl ester (1), together with five known compounds was isolated from fermentation product by use of silica gel and Sephadex LH-20 column chromatography, and preparative RP-C18 HPLC, and identified by HR-TOF-MS and NMR spectra. The cytotoxicities of these isolates against three cancer cell lines and their antifungal activities on Candida albicans were tested.

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  • - The study focuses on how MoO3-doped CeO2/TiO2 catalysts resist arsenic (As) poisoning compared to undoped CeO2/TiO2 catalysts during the selective catalytic reduction (SCR) of nitrogen oxides (NOx) with ammonia (NH3).
  • - Experimental analyses reveal that arsenic oxide affects the BET surface area and redox properties of the catalysts, leading to a reduced catalytic performance and altering the primary reaction pathways in the SCR process.
  • - The addition of MoO3 helps mitigate arsenic's negative effects by enhancing interactions that allow certain active sites to recover, thus restoring some catalytic activity and enabling better performance despite As exposure.
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A spectrum-tunable ground scenery spectrum radiation source, using LEDs and bromine tungsten lamp as luminescence media, was introduced. System structure and control of the spectrum radiation source was expounded in detail. In order to simulate various ground scenery spectrum distribution with different shapes, a ground scenery spectral database was established in the control system.

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  • Traditional loudspeaker equalization methods struggle to determine the optimal filter order until after completing the entire process, often requiring multiple attempts.
  • A new approach using balanced model truncation simplifies this challenge by allowing designers to easily choose the equalizer order and manage the error between the model and the loudspeaker.
  • The text includes examples and discusses the effectiveness of the proposed method through comparative experiments.
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The effectiveness and safety of acupuncture for the treatment of supraventricular tachycardia were systematically reviewed. The randomized controlled trials (RCTs) regarding acupuncture for supraventricular tachycardia were searched in domestic and overseas databases, and the evaluation tool of bias risk in Cochrane Handbook 5.1.

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The present paper introduced a spectral calibration method to calibrate a large aperture infrared radiation facility. We developed a radiometer which consisted of optical system, infrared detectors(cavity pyroelectric detector and HgCdTe detector 2 - 14 microm), fine mechanical modulator, lock in amplifier, signal processor, etc. At first, we analyzed the method on how to measure the spectral calibration of the large aperture infrared radiometer, and established the spectral calibration facility.

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