Publications by authors named "Xianning Li"

The addition of exogenous quorum sensing signaling molecules significantly enhanced the degradation efficiency of antibiotics, such as chloramphenicol in bio-electrochemical systems (BESs). However, the effects and mechanisms by which AHLs addition in BES facilitated the removal of sulfamethoxazole (SMX) remained inadequately explored. This study systematically compared the electrochemical performance and SMX removal efficiency in BES under two conditions: with and without the addition of N-acyl-homoserine lactones (AHLs) signaling molecules.

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Organic pollutants can alter the physicochemical properties and microbial communities of water bodies. In water contaminated with organic pollutants, the unique extracellular electron transfer mechanisms that promote sulfamethoxazole (SMX) degradation in tri-electrode microbial electrochemical systems (TE-MES) may be impacted. To simulate biodegradable organic matter contamination, glucose (GLU) was added.

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The quinoid component of humic acids (HAs) had been studied as exogenous electron mediators (EMs), but the redox-mediating abilities of other functional groups remained unclear. This study evaluated the effects of various HAs functional groups on cellular respiration and extracellular electron transfer. The three EMs increased the current density compared to the control.

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Article Synopsis
  • - The study explores the modification of microbial electrodes in a microbial electrochemical system (MES) using PEDOT and reduced graphene oxide (rGO) to enhance the degradation of antibiotics in water.
  • - Density functional theory identifies vulnerable bonds in the SMX antibiotic molecule, and the modified electrodes showed improved electron utilization and increased degradation efficiency of SMX by up to 45.47% compared to unmodified ones.
  • - The modifications also positively impacted microbial communities, boosting sulfate-reducing and denitrifying bacteria while reducing nitrifying bacteria and antibiotic resistance genes, suggesting a promising approach for antibiotics degradation and overall environmental cleanup.
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To enhance the removal efficiencies of polycyclic aromatic hydrocarbons (PAHs) in sediments and to elucidate the mechanisms by which microbial electrochemical action aids in the degradation of PAHs, humic acid was used as an electron mediator in the microbial electrochemical system in this study. The results revealed that the addition of humic acids led to increases in the removal efficiencies of naphthalene, phenanthrene, and pyrene by 45.91%, 97.

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Anaerobic Membrane Bioreactors (AnMBR) offer numerous advantages in wastewater treatment, yet they are prone to membrane fouling after extended operation, impeding their long-term efficiency and stability. In this study, a coupled system was developed using modified conductive membranes as the filtration membrane for the AnMBR and as the anodic conductive membrane in the microbial electrochemical system, with a total volume of approximately 2.57 L.

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FeO plays a complex role in soil electron transfer. A microbial fuel cell (MFC) was constructed to drive the directional transfer of electrons in soil, and the results revealed that FeO acts first as a capacitor, intercepting and reserving the electrons produced by electrochemically active bacteria (EAB) in the soil, which leads to a decrease in hexachlorobenzene (HCB) removal efficiency with increasing proportions of FeO dosing (R = 0.85).

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Excessive discharge of phosphorus can produce eutrophication in aquatic environments, damaging public health, the living environment, and the economy. The conventional mechanical-biological phosphorus removal methods are not suitable for small rural domestic sewage due to the features of small scale, scattered distribution, intermittent emission, and large fluctuation. This work evaluated electrocoagulation (EC) with industrial steel as electrodes on small rural domestic sewage.

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To remove membrane fouling, a bio-electrochemical system that can generate a micro-electric field and micro-current was constructed. After 11 days of operation, the trans-membrane pressure difference of membrane modules in the open- and closed-circuit groups increased by 35.8 kPa and 6.

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Soil microbial fuel cells (MFCs) have been increasingly studied in recent years and have attracted significant attention as an environmentally sustainable bioelectrochemical technology. However, the poor conductivity of the soil matrix and the neglect of the cathodic function have limited its application. In this study, quartz sand and activated carbon were subjected to investigation on their influence on atrazine degradation.

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In the water environment such as lakes, there is a phenomenon that the sediment and overlying water are polluted at the same time. In this study, A microbial electrochemical system with an embedded active electrode was developed for simultaneous removal of polycyclic aromatic hydrocarbons in sediment and antibiotics in overlying water by in-situ utilization of electrons. In the closed-circuit group, the pyrene concentration in sediment decreased from 9.

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To alleviate membrane fouling, a membrane of the membrane bioreactor was directly used as the anode of the bio-electrochemical system. On the 14th day, the control group had blocked, while the experimental group with a current of 0.44 mA, the increase in ΔTMP was only 2.

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Exploring the removal rules of MFC on composite heavy metal pollution is very important for the future development and field application of MFC. We constructed a three-chamber soil MFC and the results showed that with the gradual deterioration of soil heavy metal contamination from single heavy metal to metals in different oxidation states (e.g.

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A coupled system consisting of a double-anode microbial fuel cell (MFC) unit and a biofilm electrode reactor (BER) has been applied to degrade the azo dye reactive brilliant red X-3B. In this system, the MFC effluent was used as the input of the BER. The MFC preliminarily degraded X-3B while generating electricity, and the BER obtained electrons from the MFC through the external circuit to continue degrading pollutants without the need for an external power supply.

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This study constructed sediment microbial fuel cells (SMFCs) for polycyclic aromatic hydrocarbons (PAHs) removal in contaminated aquaculture sediment. Starch, a waste deposited in aquaculture sediment, was employed as the co-substrate for electricity generation and PAHs removal, and the effect of starch-derived organic acids on SMFC performance was assessed. The results indicated that sufficient starch promoted PAHs removal (69.

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Sediment microbial fuel cells (SMFCs) have been used for treating pollutants in sediment or overlying water. This study investigated the feasibility of constructing SMFCs under aquaculture conditions by employing indigenous carbohydrates as substrates to enhance the removal efficiency of polycyclic aromatic hydrocarbons (PAHs) in sediment, as well as the correlation between PAHs removal and electricity generation in SMFCs. The results showed that adding glucose could allow SMFCs to generate more electrical power and increase the removal efficiency of PAHs (by 57.

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Microbial fuel cells (MFCs) with different electrode configurations were constructed to study the mechanism of influence of multiple current paths on their electrical performance and the removal of heavy metals in soil. Three types of MFCs were constructed, namely, double anode-single cathode (DASC), single anode-dual cathode (SADC), and single anode-single cathode (SASC). The total electricity generation of the three kinds of MFC was similar: 143.

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In this study, two double-anode microbial fuel cells (MFCs) were connected in series for degradation of the azo dye reactive brilliant red X-3B. After the series connection, the electricity generation of one of the MFCs decreased, and the other was not affected too much. Due to the special structure in the double-anode MFC reduced the imbalanced performance between the MFC units, the occurrence of voltage reversal was limited.

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Microbial fuel cell (MFC) technology is widely used to remediate heavy metal pollution of soil, and the applicability of soils with different physical and chemical properties under micro-electric field has not been studied. In this study, copper was effectively removed in four typical soil-filled MFCs. The removal efficiencies of copper from closed-circuit MFCs filled with paddy, red, black and alluvial soils were 2.

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In this study, we constructed a three-chamber microbial fuel cell (TC-MFC) that avoided the adverse effects of H diffusion on anode microorganisms in the acidic catholyte and the precipitation of heavy metals in the soil near the cathode side (S4), while also achieving migration of copper from the soil and reduction of Cu in the catholyte. The removal efficiency of acid-soluble Cu from the soil near the anode region reached 42.5% after 63 days of operation at an external resistance of 100 Ω and electrode spacing of 10 cm, and Cu in the catholyte was completely removed within 21 days.

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As an environmentally sustainable bioelectrochemical technology, the microbial fuel cell (MFC) has attracted great attention. In this study, a three-chamber MFC (TC-MFC) was enhanced with different auxiliary reagents to remove heavy metals from soil. The results showed that the removal efficiency of heavy metals from soil increased with increasing auxiliary reagent concentration.

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Microbial fuel cells (MFCs) can remove and recover metals in wastewater; however, there are relatively few studies of metal removal from soil by MFCs. In this study, we developed a three-chamber soil MFC consisting of an anode, contaminated soil, and cathode chamber to remove heavy metals from soil. The performance of the soil MFC was investigated by assessing the relationships among current, voltage, and Cu migration, and reduction.

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In this study, a continuous-flow microbial fuel cell (MFC) system was constructed to treat azo dye wastewater for 400 days. The electrical properties of the MFC after 400-day operation and the removal efficiencies of the MFC after long- and short-term operation were analyzed with respect to co-substrate concentrations. The power output of the MFC system decreased from 586 to 330 mV with increasing operating time, and the removal efficiencies of the MFC remained stable after long-term operation in comparison to those after short-term operation, even when the co-substrate concentration was reduced.

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The demand for removal of refractory organic pollutants limits the application of microbial fuel cells. In this study, the synergistic effects of bioelectrochemical and photocatalysis methods were captured by constructing a biophoto anode from a combination of WO/TiO and carbon felt. This biophoto electrode was able to decrease the aniline concentration from 63.

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This study aims to demonstrate that an up-flow microbial fuel cell-coupled constructed wetland (UCW-MFC) can effectively treat synthetic wastewater that contains a high concentration of pharmaceutical and personal care products (PPCPs, 10 mg L level), such as ibuprofen (IBP) and bisphenol A (BPA). A significant decline in chemical oxygen demand (COD) and ammonia nitrogen (NH-N) removal was observed when BPA was added, which indicated that BPA was more toxic to bacteria. The closed circuit operation of UCW-MFC performed better than the open circuit mode for COD and NH-N removal.

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