Publications by authors named "Wolfgang Paa"

Laser safety is starting to play an increasingly important role, especially when the laser is used as a tool. Passive laser safety systems quickly reach their limits and, in some cases, provide inadequate protection. To counteract this, various active systems have been developed.

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The effect of roughness and thickness of alumina layers, mimicking the passivation layer commonly used in dye-sensitized photoelectrodes, on the molecular adsorption of P1 dye, 4-(bi(4-(2,2-dicyano-vinyl)-thiophene-2-yl]-phenyl]-aminobenzoic acid) has been studied using surface-sensitive vibrational sum frequency generation(VSFG) spectroscopy. The VSFG spectra reveal the formation of poorly ordered dye layers on relatively rough surfaces where XPS measures a higher dye loading. Furthermore, these poorly ordered dye molecules are responsible for the generation of trapped electronic states as probed by successive photoluminescence (PL) measurements.

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To investigate the fundamentals of liquid oxygen droplet combustion in hydrogen under microgravity conditions, a drop tower apparatus has been developed. In a cryogenic combustion chamber cooled with liquid nitrogen, single oxygen droplets with a diameter of 1 mm are suspended at the tip of a thin suspender. Ignition is accomplished after microgravity conditions are reached by a near-infrared laser, which generates a plasma spark positioned in the immediate vicinity of the oxygen droplet.

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We describe a specially designed diode pumped solid state laser system based on the disk laser architecture for combustion diagnostics under microgravity (μg) conditions at the drop tower in Bremen. The two-stage oscillator-amplifier-system provides an excellent beam profile (TEM00) at narrowband operation (Δλ < 1 pm) and is tunable from 1018 nm to 1052 nm. The laser repetition rate of up to 4 kHz at pulse durations of 10 ns enables the tracking of processes on a millisecond time scale.

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A new concept enhances the capability of photo-thermal absorption measurements with transversal probe beam guiding by overcoming drawbacks such as a lack of sensitivity for materials with low photo-thermal response and/or round substrate geometry. The sandwich concept using the laser-induced deflection technique is introduced and tested for the investigation of highly reflecting (HR) coatings. The idea behind the sandwich concept is based on the decoupling of the optical materials for the pump and probe beams.

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We demonstrate an excitation transfer along a fluorescently labeled dsDNA nanowire over a length of several micrometers. Launching of the excitation is done by exciting a localized surface plasmon mode of a 40 nm silver nanoparticle by 800 nm femtosecond laser pulses via two-photon absorption. The plasmonic mode is subsequently coupled or transformed to excitation in the nanowire in contact with the particle and propagated along it, inducing bleaching of the dyes on its way.

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We investigate the characteristics of a thin disk laser system based on the master oscillator-power amplifier design. The amplifier emits parasitic laser oscillation (PL) when the wavelength of the tunable narrow-bandwidth seed pulse is detuned more than 4 nm from the gain maximum at 1030 nm. For suppression of this unwanted PL, a birefringent filter (Lyot filter) was inserted into the amplifier cavity in order to generate wavelength selective losses, especially at the gain maximum of the Yb:YAG crystal.

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We investigate a cavity ring down setup that offers the possibility to measure the spectrally resolved reflectivities of high reflectivity mirrors. The setup consists of a resonator (ring down cavity) and an intensified CCD camera system combined with a spectrograph for spectral resolution. A commercial supercontinuum laser (350-1750 nm) is applied as a compact excitation source.

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