China has experienced rapid population growth and increasing human N and P discharge from point sources. This paper presents a new spatial and temporal model-based, province-scale inventory of N and P in wastewater using detailed information on the location and functioning of 4436 WWTPs covering China for the period 1970-2015. China's nutrient discharge to surface water increased 22-fold from 177 to 3908 Gg N yr and 29-fold from 20 to 577 Gg P yr in urban areas between 1970 and 2015.
View Article and Find Full Text PDFNitrous oxide (NO) is a long-lived greenhouse gas and currently contributes ∼10% to global greenhouse warming. Studies have suggested that inland waters are a large and growing global NO source, but whether, how, where, when, and why inland-water NO emissions changed in the Anthropocene remains unclear. Here, we quantify global NO formation, transport, and emission along the aquatic continuum and their changes using a spatially explicit, mechanistic, coupled biogeochemistry-hydrology model.
View Article and Find Full Text PDFRivers play an important role in the global carbon (C) cycle. However, it remains unknown how long-term river C fluxes change because of climate, land-use, and other environmental changes. Here, we investigated the spatiotemporal variations in global freshwater C cycling in the 20th century using the mechanistic IMAGE-Dynamic Global Nutrient Model extended with the Dynamic In-Stream Chemistry Carbon module (DISC-CARBON) that couples river basin hydrology, environmental conditions, and C delivery with C flows from headwaters to mouths.
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