Publications by authors named "Wenfa Tan"

Article Synopsis
  • Immobilization of uranium (U (VI)) through uranyl phosphate precipitation shows promise for cleaning up contaminated environments, highlighting the importance of phosphorus in bacteria's role in this process.
  • Research indicated that phosphates significantly improve U (VI) removal, achieving a remarkable 99.84% efficiency while revealing that both U (VI) and U (IV) are present on sample surfaces.
  • Despite the successful immobilization, long-term stability issues arise as bacteria may lead to uranium redissolution over time, particularly in mining areas, emphasizing the need to consider environmental conditions for lasting solutions.
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Phosphate-solubilizing bacteria (PSB) are important but often overlooked regulators of uranium (U) cycling in soil. However, the impact of PSB on uranate fixation coupled with the decomposition of recalcitrant phosphorus (P) in mining land remains poorly understood. Here, we combined gene amplicon sequencing, metagenome and metatranscriptome sequencing analysis and strain isolation to explore the effects of PSB on the stabilization of uranate and P availability in U mining areas.

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Residues generated from the uranium purification process, characterized by a high uranium content, pose a significant challenge for recovery through leaching and present a considerable environmental threat. After using XRD and SEM-mapping characterization analysis combined with the BCR continuous graded extraction test to analyze the content of different states of uranium, it was found that the main reason why the uranium in the residue was difficult to leach because it was encapsulated by SiO crystals. Using NHHF as a leaching agent, a leaching study of uranium in the residue was carried out, and the results showed that the H and F produced by NHHFcould react with SiO, destroying the crystal lattice of SiO and causing the encapsulated uranium to come into contact with the leaching agent, facilitating the leaching of uranium in the residue.

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Enzymatically catalyzed reduction of metals by bacteria has potential application value to uranium-mine wastewater. However, its practical implementation has long been restricted by its intrinsic drawbacks such as low efficiency and long treatment-time. This study aims to explore the effect of electrodes on U (VI) removal efficiency by a purified indigenous bacteria isolated from a uranium mining waste pile in China.

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Article Synopsis
  • The study investigates how indigenous microorganisms, particularly Leifsonia sp., can be used to immobilize uranyl (U(VI)) in the presence of iron (Fe(III)) (hydr)oxides, which may either enhance or hinder uranium removal based on environmental conditions.
  • Results show that Fe(III) (hydr)oxides, especially hematite, significantly retarded the removal of U(VI) from water, and the process led to slow-release of U(VI) bound within precipitates over time.
  • Findings suggest that the transformation of ferrihydrite to goethite and the conversion of U(VI) to U(IV) play key roles in the
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Uranium mining and milling activities for many years resulted in release of uranium into the adjoining soil in varying degrees. Bioremediation approaches (i.e.

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Immobilization of U(VI) by naturally ubiquitous ferrous ions (Fe(II)) has been considered as an efficient and ecofriendly method to retard the migration of aqueous U(VI) at many nuclear sites and surface environments. In this study, we conducted Fe-U coprecipitation experiments to investigate the mechanism and stability of uranium (U) precipitation induced by a small quantity of Fe(II) under oxygen-rich conditions. The experimental results suggest that the sedimentation rates of U(VI) by Fe(II) under neutral oxygen-rich conditions are more than 96%, which are about 36% higher than those without Fe(II) and 16% higher than those under oxygen-free conditions.

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Zero-valent iron (ZVI) has been widely applied to the remediation of uranium (U)-contaminated water. Notably, indigenous bacteria may possess potential positive or unfavorable influence on the mechanism and stability of Fe-U precipitates. However, the focus of the researches in this field has mainly been on physical and/or chemical aspects.

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Soil contains large amounts of humic acid (HA), iron ions and manganese ions, all of which affect U(VI) migration in the soil. HA interacts with iron and manganese ions to form HA salts (called HA-Fe and HA-Mn in this paper); however, the effects of HA-Fe and HA-Mn on the migration of U(VI) is not fully understood. In this study, HA-Fe and HA-Mn were compounded by HA interactions with ferric chloride hexahydrate and manganese chloride tetrahydrate, respectively.

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Uranium (U) contamination of soil has become a major concern with respect to its toxicity, accumulation in the food chain, and persistence in the environment. Anthropogenic activities like mining and processing of U ores has become pressing issues throughout the world. The aim of the work is to understand the chemical fractionation of U in polluted soil and the mechanism involved.

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It has generally been assumed that the immobilization of U(VI) via polyphosphate accumulating microorganisms may present a sink for uranium, but the potential mechanisms of the process and the stability of precipitated uranium under aerobic conditions remain elusive. This study seeks to explore the mechanism, capacity, and stability of uranium precipitation under aerobic conditions by a purified indigenous bacteria isolated from acidic tailings (pH 6.5) in China.

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