Perfect excitation and attenuation-free propagation of graphene surface polaritons under optical admittance matching.

Graphene supports both transverse magnetic and electric modes of surface polaritons due to the intraband and interband transition properties of electrical conductivity. Here, we reveal that perfect excitation and attenuation-free propagation of surface polaritons on graphene can be achieved under the condition of optical admittance matching. With both vanished forward and backward far-field radiation, incident photons are fully coupled to surface polaritons.

Enhancing electromagnetic field gradient in tip-enhanced Raman spectroscopy with a perfect radially polarized beam.

Tip-enhanced Raman spectroscopy (TERS) is a promising label-free super-resolving imaging technique, and the electric field gradient of nanofocusing plays a role in TERS performance. In this paper, we theoretically investigated the enhancement and manipulation of the electric field gradient in a bottom-illumination TERS configuration through a tightly focused perfect radially polarized beam (PRPB). Improvement and manipulation in electric field enhancement and field gradient of the gap-plasmon mode between a plasmonic tip and a virtual surface plasmons (SPs) probe are achieved by adjusting the ring radius of the incident PRPB.

Visible-Band Chiroptical Meta-devices with Phase-Change Adjusted Optical Chirality.

Low-cost large-area chirality meta-devices (CMDs) with adjustable optical chirality are of great interest for polarization-sensitive imaging, stereoscopic display, enantioselectivity analysis, and catalysis. Currently, CMDs with adjusted chiroptical responses in the mid-infrared to terahertz band have been demonstrated by exploiting photocarriers of silicon, pressure, and phase-change of GSTs but are still absent in the visible band, which in turn limits the development of chiral nanophotonic devices. Herein, by employing a phase-change material (SbS), we present a protocol for the fabrication of wafer-scale visible-band enantiomeric CMDs with handedness, spectral, and polarization adjustability.

Tip-enhanced four-wave mixing internally illuminated by an ultrafast vector light field.

A tip nanofocusing light field, with high electric-field intensity and nanoscale mode volume, can significantly improve nonlinear light scattering efficiency, thereby greatly promoting the development of strong-field nano-optics. Here, tip-enhanced four-wave mixing (FWM) is theoretically analyzed through two ultrafast radial vector beams internally illuminating an Ag-coated silica tip (ACST). Two femtosecond pulses, with radial electric vectors and pulse width of 100 fs, are adopted as excitation sources to illuminate the ACST.

Robust and low cost in-fiber acousto-optic Mach-Zehnder interferometer and its application in a dual-wavelength laser.

A robust in-fiber tunable acousto-optic Mach-Zehnder interferometer with a taper-shaped sandwich-like fiber structure is proposed and characterized experimentally, based on which tunable dual-wavelength lasers are demonstrated. The fiber structure was prepared by two-step etching methods, which could be used to fabricate either a symmetric structure for a continuous tuning dual-wavelength laser or an asymmetric structure for a switchable one. The proposed structure has advantages of low cost, low driving power, and robustness.

Three-photon-induced free-carrier absorption in Ga-doped ZnO.

Ga-doped ZnO (Ga:ZnO) possesses many advantages due to the unique atomic structure and intriguing physical and chemical properties of Ga, but its optical nonlinear characteristics are rarely studied, so it is difficult to expand its application in the fields of optoelectronics and all-optical components. Here, we examine the optical nonlinearity of Ga:ZnO with the help of a theoretical quantitative model of three-photon-absorption (3PA)-induced free carrier absorption (FCA) and free carrier refraction (FCR). 3PA-induced FCA was examined and distinguished successfully from 3PA through z-scan measurements.

Circular nanocavity substrate-assisted plasmonic tip for its enhancement in nanofocusing and optical trapping.

Plasmonic tip nanofocusing has widely been applied in tip-enhanced Raman spectroscopy, optical trapping, nonlinear optics, and super-resolution imaging due to its capability of high local field enhancement. In this work, a substrate with a circular nanocavity is proposed to enhance the nanofocusing and optical trapping characteristics of the plasmonic tip. Under axial illumination of a tightly focused radial polarized beam, the circular nanohole etched on a metallic substrate can form a nanocavity to induce an interference effect and further enhance the electric field intensity.

Extracting epsilon-near-zero wavelength of ultrathin plasmonic film.

Strong optical nonlinearities of plasmonic thin films exist at their epsilon-near-zero (ENZ) wavelengths, which are essential to be acquired first for the design and fabrication of ENZ photonic devices. However, it has been challenging to obtain the ENZ wavelength precisely when the film thickness is reduced to tens of nanometers or less. By enhancing both electric field intensity and light-matter interaction distance in the film, we propose that the ENZ wavelength and the medium model of ultrathin films can be extracted accurately from the transmittance and reflectance spectra under oblique light excitation.

Metallic nanosphere-assisted coupling ultrafast surface plasmon polaritons background-free tip nanofocusing.

Plasmonic tip nanofocusing has gained much attention owing to its wide application in the field of nanospectroscopy. Here, we present the Au nanosphere (AuNS)-assisted coupling ultrafast surface plasmon polaritons (SPP) background-free tip nanofocusing. The plasmonic tip was prepared by attaching an AuNS on the shaft of an Au conical tip fabricated by electrochemical etching.

Nanofocusing of a metallized double periodic arranged nanocone array for surface-enhanced Raman spectroscopy.

A plasmonic double periodic arranged nanocone array (DPANA) integrated by nanotips and nanogaps exhibit strong capability of light compression, and thus lead to extremely enhanced electric near-field intensity. The DPANA is fabricated by the self-assembled mask integrated with the inductively couple plasma (ICP) etching technology. Finite-difference time-domain (FDTD) simulations suggest that the metallized DPANA can generate a strong hotspot at the sharp tip apex and the nanogap between adjacent sharp tips.

Anisotropy of 2PA, 3PA, and Kerr effect in nonpolar ZnO.

Anisotropic optical nonlinearity plays an important role in polarization-dependent optoelectronic devices. Taking the advantage of in-plane crystallographic axis, the polarization dependence of third- and fifth-order nonlinearity in nonpolar ZnO has been investigated by scan. Here, we established the theory model of anisotropic relation of fifth-order nonlinearity in hexagonal wurtzite crystal.

Novel Method Based on Hollow Laser Trapping-LIBS-Machine Learning for Simultaneous Quantitative Analysis of Multiple Metal Elements in a Single Microsized Particle in Air.

Elemental identification of individual microsized aerosol particles is an important topic in air pollution studies. However, simultaneous and quantitative analysis of multiple constituents in a single aerosol particle with the noncontact in situ manner is still a challenging task. In this work, we explore the laser trapping-LIBS-machine learning to analyze four elements (Zn, Ni, Cu, and Cr) absorbed in a single micro-carbon black particle in air.

Optical trapping of single nano-size particles using a plasmonic nanocavity.

Trapping and manipulating micro-size particles using optical tweezers has contributed to many breakthroughs in biology, materials science, and colloidal physics. However, it remains challenging to extend this technique to a few nanometers particles owing to the diffraction limit and the considerable Brownian motion of trapped nanoparticles. In this work, a nanometric optical tweezer is proposed by using a plasmonic nanocavity composed of the closely spaced silver coated fiber tip and gold film.

Lab on D-shaped fiber excited via azimuthally polarized vector beam for surface-enhanced Raman spectroscopy.

We present a method for Raman examination using a silver-nanoparticles (Ag-NPs) coated D-shaped fiber (DSF) internally excited via an in-fiber azimuthally polarized beam (APB) generated by an acoustically induced fiber grating. Simulation results show that an electric-field intensity enhancement factor can be effectively improved under APB excitation compared with the linear polarization beam (LPB) excitation, because the strong gap-mode is uniformly generated between two adjacent Ag NPs on the surface of the DSF planar side. Experimental results show that the Raman signal intensity of the methylene blue (MB) detected by DSF in the case of APB excitation is ∼4.

Plasmonic color filter based on a hetero-metal-insulator-metal grating.

Plasmonic color filters are expected to be candidates for application to complementary metal-oxide-semiconductor (CMOS) image sensor arrays with reduced pixel size, owing to the subwavelength mode volume of plasmons. Designs of metallic gratings based on the guided-mode resonance effect suffer from the sideband transmission issue due to high-order diffraction. Here, we propose a plasmonic color filter structure based on a hetero-metal-insulator-metal grating.

Plasmon-enhanced nonlinear nanofocusing of gold nanoprisms driven via an ultrafast azimuthal vector beam.

We present the plasmon-enhanced nonlinear nanofocusing of a gold (Au) nanoprism array substrate (ANAS) driven via an ultrafast azimuthal vector beam (AVB). Theoretical calculations show that the electric-field intensity of the ANAS vertically excited via the femtosecond AVB is higher than that of LPB excitation. In this experiment, the second-order surface nonlinear optical response of the ANAS is adopted to examine the nonlinear plasmonic nanofocusing of the ANAS, and it was observed that the second harmonic (SH) intensity of the ANAS excited via the femtosecond AVB is ∼3.

Surface-Enhanced Raman Spectroscopy Based on a Silver-Film Semi-Coated Nanosphere Array.

In this paper, we present a convenient and economical method to fabricate a silver (Ag)-film semi-coated polystyrene (PS) nanosphere array substrate for surface-enhanced Raman spectroscopy (SERS). The SERS substrate was fabricated using the modified self-assembled method combined with the vacuum thermal evaporation method. By changing the thickness of the Ag film, the surface morphology of the Ag film coated on the PS nanospheres can be adjusted to obtain the optimized localized surface plasmonic resonance (LSPR) effect.

Feasibility of quasicritical coupling based on LP modes and its application as a filter with tunable bandwidth and stable insertion loss.

The feasibility of the quasicritical coupling based on the high order scalar modes in tapered fiber was presented and discussed in detail theoretically. As its applications, the bandwidth evolution of the coupling process both in the Through port and the Drop port were also included in the calculations and demonstrated in the experiment. As a result, tunable bandwidth filters with stable insertion loss were realized by changing the gap between the few-mode tapered fiber and microcavity working under a state of quasicritical coupling.

All-fiber frequency shifter consisting of a fiber Bragg grating modulated via an acoustic flexural wave for optical heterodyne measurement.

We present an all-fiber frequency shifter (AFFS) consisting of a fiber Bragg grating (FBG) modulated via an acoustic flexural wave for optical heterodyne measurement. The AFFS can efficiently generate the frequency-shifted signal due to the resonance peak with a high-reflection efficiency and being completely separated from the reflection spectrum of the original FBG, simultaneously. The experimental result shows that the minimal measurable vibration amplitude and the resolution of the all-fiber optical heterodyne measurement setup constructed with the AFFS are 0.

Strong Coupling between Dark Plasmon and Anapole Modes.

Plasmonic nanocavities enable extreme light-matter interaction by pushing light down to the nanoscale. The dipolar feature of bright modes allows coupling with the external excitation from free space but results in a radiating background, whereas nonradiating dark plasmon modes can hardly be excited. Here, we report for the first time on strong coupling between dark plasmon and anapole modes in a hybrid metal-dielectric nanostructure.

All-fiber narrow-linewidth ring laser with continuous and large tuning range based on microsphere resonator and fiber Bragg grating.

We demonstrate an all-fiber single-longitudinal-mode (SLM) narrow-linewidth ring laser stabilized by a microsphere resonator and fiber Bragg gratings (FBGs) with a large continuous wavelength tuning range from 1540 nm to 1570 nm. In the experiment, stable lasing with a linewidth smaller than 5 kHz was obtained. The laser wavelength was linearly and continuously tuned in the range of 0.

Near-infrared photodetection with plasmon-induced hot electrons using silicon nanopillar array structure.

A plasmon-induced hot-electron photodetector based on silicon nanopillar array is developed. The nanostructure is fabricated by reactive ion etching with a monolayer of self-assembled polystyrene nanosphere in hexagonal close-packed lattice as the mask. Light absorption and hot-electron generation are mainly enhanced by the surface plasmon polaritons formed at the surface of the gold film on the nanopillar sidewalls.

Tip-Enhanced Raman Spectroscopy with High-Order Fiber Vector Beam Excitation.

We investigated tip-enhanced Raman spectra excited by high-order fiber vector beams. Theoretical analysis shows that the high-order fiber vector beams have stronger longitudinal electric field components than linearly polarized light under tight focusing conditions. By introducing the high-order fiber vector beams and the linearly polarized beam from a fiber vector beam generator based on an electrically-controlled acoustically-induced fiber grating into a top-illumination tip-enhanced Raman spectroscopy (TERS) setup, the tip-enhanced Raman signal produced by the high-order fiber vector beams was 1.

Broadband polarization-insensitive saturable absorption of FeO nanoparticles.

The synthesis and functionalization of transition-metal oxides are one of the most active research areas in advanced materials. As a typical transition-metal oxide, iron oxide has been widely used in lithium-ion batteries, gas sensors, and for water treatment. Herein, we synthesized FeO nanoparticles by a co-precipitation method that is inexpensive and non-toxic.