Multifunctional Metasurface Tuning by Liquid Crystals in Three Dimensions.

Optical metasurfaces present remarkable opportunities for manipulating wave propagation in unconventional ways, surpassing the capabilities of traditional optical devices. In this work, we introduce and demonstrate a multifunctional dynamic tuning of dielectric metasurfaces containing liquid crystals (LCs) through an effective three-dimensional (3D) control of the molecular orientation. We theoretically and experimentally study the spectral tuning of the electric and magnetic resonances of dielectric metasurfaces, which was enabled by rotating an external magnetic field in 3D.

Formation and stability of vortex solitons in nematic liquid crystals.

We study the propagation dynamics of bright optical vortex solitons in nematic liquid crystals with a nonlocal reorientational nonlinear response. We investigate the role of optical birefringence on the stability of these solitons. In agreement with recent experimental observations, we show that the birefringence-induced astigmatism can eventually destabilize these vortex solitons.

Anomalous interaction of spatial solitons in nematic liquid crystals.

We study experimentally the interaction of mutually incoherent bright spatial solitons in dye-doped nematic liquid crystals (LCs). The dye-induced light absorption results in a complex nonlinear optical response of the LC having spatially nonlocal focusing and defocusing contributions. The competition between both nonlinearities leads to the separation-dependent soliton interaction with repulsion of distant and attraction of closely placed solitons.

Nonlinear propagation and quasi self-confinement of light in plasmonic resonant media.

We study nonlinear propagation of light in colloidal suspension of metallic nanoparticles, in the regime of particles surface plasmon resonance. We show that the propagation exhibits features typical for purely defocusing media and the observed spatial confinement is not a real self-trapping, as for solitons, but rather than is caused by the phase modulation of the beam via nonlocal defocusing nonlinearity. We also show that the light-induced refractive index change in the suspension leads to stabilization of structured light beams.

Magnetic routing of light-induced waveguides.

Among photofunctional materials that can be employed to control the propagation of light by modifying their properties, soft dielectrics such as nematic liquid crystals (NLCs) stand out for their large all-optical response. Through reorientation, the molecular distribution of NLCs can be modified by the electric field of light, permitting functional operations and supporting self-localized light beams or spatial optical solitons. To date, the generation and routing of such solitons have been limited by the boundary conditions employed to tailor the properties of NLCs in planar cells or capillaries.

Quasi-phase matching via femtosecond laser-induced domain inversion in lithium niobate waveguides.

We demonstrate an all-optical fabrication method of quasi-phase matching structures in lithium niobate (LiNbO) waveguides using a tightly focused femtosecond near-infrared laser beam (wavelength of 800 nm). In contrast to other all-optical schemes that utilize a periodic lowering of the nonlinear coefficient χ by material modification, here the illumination of femtosecond pulses directly reverses the sign of χ through the process of ferroelectric domain inversion. The resulting quasi-phase matching structures, therefore, lead to more efficient nonlinear interactions.

Nonlinear diffraction in orientation-patterned semiconductors.

This work represents experimental demonstration of nonlinear diffraction in an orientation-patterned semiconducting material. By employing a new transverse geometry of interaction, three types of second-order nonlinear diffraction have been identified according to different configurations of quasi-phase matching conditions. Specifically, nonlinear Čerenkov diffraction is defined by the longitudinal quasi-phase matching condition, nonlinear Raman-Nath diffraction satisfies only the transverse quasi-phase matching condition, and nonlinear Bragg diffraction fulfils the full vectorial quasi-phase matching conditions.

Unveiling the orbital angular momentum and acceleration of electron beams.

New forms of electron beams have been intensively investigated recently, including vortex beams carrying orbital angular momentum, as well as Airy beams propagating along a parabolic trajectory. Their traits may be harnessed for applications in materials science, electron microscopy, and interferometry, and so it is important to measure their properties with ease. Here, we show how one may immediately quantify these beams' parameters without need for additional fabrication or nonstandard microscopic tools.

The role of light-induced nanostructures in femtosecond laser micromachining with vector and scalar pulses.

In this article we compare the results of micromachining of fused silica and silicon with tightly focused scalar (viz., circularly and linearly polarized) and vector (viz., azimuthally and radially polarized) femtosecond laser pulses.

Polarization-dependent ablation of silicon using tightly focused femtosecond laser vortex pulses.

We demonstrate experimentally that, in a tight focusing geometry, circularly polarized femtosecond laser vortex pulses ablate material differently depending on the handedness of light. This effect offers an additional degree of freedom to control the shape and size of laser-machined structures on a subwavelength scale.

Optical manipulation of particle ensembles in air.

We demonstrate that airborne light-absorbing particles can be photophoretically trapped and moved inside an optical lattice formed by multiple-beam interference. This technique allows simultaneous three-dimensional manipulation of multiple micro-objects in gases.

Robust trapping and manipulation of airborne particles with a bottle beam.

We demonstrate that micron-sized light-absorbing particles can be trapped and transported photophoretically in air using an optical bottle formed inside the focal volume of a lens with a controlled amount of spherical aberration. This optical fiber-based single beam trap can be used in numerous applications where true 3D manipulation and delivery of airborne micro-objects is required.

Revealing local field structure of focused ultrashort pulses.

We utilize the interaction of tightly focused ultrashort pulses with transparent media to imprint their local polarization in the focal region. In particular, we demonstrate that this technique allows for a subwavelength resolution diagnostic of complex polarization states including the presence of the longitudinal component of the electric field. Moreover, we demonstrate the first ever material ablation with the longitudinal electric field of femtosecond pulses.

Materials processing with a tightly focused femtosecond laser vortex pulse.

In this Letter we present the first (to our knowledge) demonstration of material modification using tightly focused single femtosecond laser vortex pulses. Double-charge femtosecond vortices were synthesized with a polarization-singularity beam converter based on light propagation in a uniaxial anisotropic medium and then focused using moderate- and high-NA optics (viz., NA=0.

Giant optical manipulation.

We demonstrate a new principle of optical trapping and manipulation increasing more than 1000 times the manipulation distance by harnessing strong thermal forces while suppressing their stochastic nature with optical vortex beams. Our approach expands optical manipulation of particles into a gas media and provides a full control over trapped particles, including the optical transport and pinpoint positioning of ∼100  μm objects over a meter-scale distance with ±10  μm accuracy.

Efficient beam converter for the generation of high-power femtosecond vortices.

We describe an optical beam converter for an efficient transformation of Gaussian femtosecond laser beams to single- or double-charge vortex beams. The device achieves a conversion efficiency of 75% for single- and 50% for double-charge vortex beams and can operate with high-energy broad bandwidth pulses. We also show that the topological charge of a femtosecond vortex beam can be determined by analyzing its intensity distribution in the focal area of a cylindrical lens.

Spatially engineered polarization states and optical vortices in uniaxial crystals.

We describe how the propagation of light through uniaxial crystals can be used as a versatile tool towards the spatial engineering of polarization and phase, thereby providing an all-optical technique for vectorial and scalar singular beam shaping in optics. Besides the prominent role played by the linear birefringence, the influence of circular birefringence (the optical activity) is discussed as well and both the monochromatic and polychromatic singular beam shaping strategies are addressed. Under cylindrically symmetric light-matter interaction, the radially, azimuthally, and spirally polarized eigen-modes for the light field are revealed to be of a fundamental interest to describe the physical mechanisms at work when dealing with scalar and vectorial optical singularities.

Soliton bending and routing induced by interaction with curved surfaces in nematic liquid crystals.

We study experimentally the interaction of spatial optical solitons with curved dielectric surfaces in unbiased nematic liquid crystals. We demonstrate that this interaction depends on the curvature of the surface and the walk-off, and it can be employed for efficient routing and control of the soliton trajectories. We also observe a large-angle total internal reflection of the soliton beam from an interface between liquid crystal and air.

Selective trapping of multiple particles by volume speckle field.

We suggest a new approach for selective trapping of light absorbing particles in gases by multiple optical bottle-beam-like traps created by volume speckle field. We demonstrate stable simultaneous confinement of a few thousand micro-particles in air with a single lowpower laser beam. The size distribution of trapped particles exhibits a narrow peak near the average size of an optical speckle.

Determination of topological charges of polychromatic optical vortices.

We introduce a simple, single beam method for determination of the topological charge of polychromatic optical vortices. It is based on astigmatic transformation of singular optical beams, where the intensity pattern of a vortex beam acquires a form of dark stripes in the focal plane of a cylindrical lens. The number of the dark stripes is equal to the modulus of the vortex topological charge, while the stripe tilt indicates the charge sign.

Dynamics of linear polarization conversion in uniaxial crystals.

We report on the experimental and theoretical investigation of polarization conversion of linearly polarized Gaussian beam propagating in perpendicularly cut homogeneous uniaxial crystals. We derive analytical expressions, in good agreement with experimental data, for power transfer between components at normal incidence accompanied by the generation of a topological quadrupole. We extend the results to the oblique incidence case and confirm experimentally the optimal parameters for generation of a single charge on-axis optical vortex, including spectrally resolved measurements for the white-light beams.

Photophoretic manipulation of absorbing aerosol particles with vortex beams: theory versus experiment.

We develop a theoretical approach for describing the optical trapping and manipulation of carbon nanoclusters in air with a dual-vortex optical trap, as realized recently in experiment [V. Shvedov et al., Opt.

Dynamics of optical spin-orbit coupling in uniaxial crystals.

We study theoretically and verify experimentally the detailed dynamics of spin-to-orbital angular momentum conversion for a circularly polarized Gaussian beam propagating along the optical axis of a uniaxial crystal. We extend the results to the case of white-light beams when each of the spectral components undergoes its own wavelength-dependent angular momentum conversion process.

Optical guiding of absorbing nanoclusters in air.

We suggest a novel approach in all-optical trapping employing a photophoretic force for manipulation of absorbing particles in open air. We demonstrate experimentally the robust three-dimensional guiding, over the distances of a few millimeters, of agglomerates of carbon nanoparticles with the size spanned from 100 nm to 10 microm, as well as their acceleration up to velocities of 1 cm/sec. We achieve stable positioning and guiding of particles as well as simultaneous trapping of a large number of particles in a dual-beam optical trap created by two counter-propagating and co-rotating optical vortex beams.