Effect of Femtosecond Ultraviolet and Infrared Laser Wavelength on Plasma Characteristics of Metals, Ceramics and Glass Samples Using Femtosecond Laser-Induced Breakdown Spectroscopy.

In this work, we present studies on the effect of laser wavelengths on the laser-induced plasma characterization using a femtosecond (fs) ytterbium-doped potassium-gadolinium tungstate (Yb:KGW) laser. Plasma plumes of copper, steel, ceramics, and glass samples were induced using a multiple shot of 200 fs laser pulses with 1030 nm and 343 nm wavelengths at fixed laser fluence () and analyzed using the laser-induced breakdown spectroscopy (LIBS) technique. Time-resolved fs-LIBS measurements were performed on the same set of samples and under the same experimental conditions.

Direct time-resolved plasma characterization with broadband terahertz light pulses.

We report here the results of comprehensive plasma characterization and diagnostics by analyzing time-resolved absorption spectra of short ultrabroadband (0.1-50 THz) pulses propagated through the test plasma. Spectral analysis of plasma-induced absorption of such THz pulses provides very direct, in situ, high dynamical range, potentially single-shot access to the plasma density, plasma decay time, electron temperature, and ballistic dynamics of the plasma expansion.

Intensity modulated terahertz vortex wave generation in air plasma by two-color femtosecond laser pulses.

We investigate the generation of broadband terahertz (THz) pulses with phase singularity from air plasmas created by fundamental and second harmonic laser pulses. We show that when the second harmonic beam carries a vortex charge, the THz beam acquires a vortex structure as well. A generic feature of this THz vortex is that the intensity is modulated along the azimuthal angle, which can be attributed to the spatially varying relative phase difference between the two pump harmonics.

Femtosecond Laser Micromachining of Soda-Lime Glass in Ambient Air and under Various Aqueous Solutions.

We have studied femtosecond ablation of soda-lime glass sample under thin water film, under KOH and NaCl aqueous solutions films and their influence and benefits compared with ablation in the air atmosphere. These have been studied in case of the groove ablation using the infrared (IR) femtosecond laser. KOH aqueous solution film above the glass sample improved the ablation efficiency and led to the formation of the grooves with a higher aspect ratio when multi-scan glass cutting conditions were applied.

Probing electronic coherences by combined two- and one-photon excitation in atomic vapors.

Wave mixing in a three-level quantum system induced by two-photon resonant pump and one-photon resonant coupling at lower transition has been studied theoretically and experimentally. Resonantly enhanced difference-frequency generation efficiency was observed clearly dependent on the time delay and its sign between the femtosecond pump and probe. The role of the atomic coherences on the amplification without inversion during different sequences of interaction in a closed three-level system has been also stressed.

Conical third-harmonic generation in normally dispersive media.

It is shown, both theoretically and experimentally, that in normally dispersive media under tight-focusing conditions third harmonic is generated by six-wave mixing rather than via common third-order frequency tripling. Though far-field pattern of third-harmonic signal was an axially symmetric ring for a wide range of the material wave vector mismatch and laser beam focusing conditions, in some cases the generation of more complex beams has been found possible. Results of simulations of the proposed model qualitatively correspond well with experimental data for the calculated values of third- and fifth-order nonlinear susceptibilities of sodium.