Influence of photothermal and plasma-mediated nano-processes on fluence thresholds for ultrafast laser-induced cavitation around gold nanoparticles.

Laser fluence thresholds of ultrafast excitation of vapor bubbles around gold nanoparticles are determined experimentally. An optical scattering technique of limited minimum bubble size resolution is employed and analyzed for that purpose. Measurements were performed for spherical gold nanoparticles of varying sizes (40-200 nm) and for laser pulses of varying pulse width (55 fs to 4.