Strong Coupling Dynamics of a Quantum Emitter near a Topological Insulator Nanoparticle.

We study the spontaneous emission dynamics of a quantum emitter near a topological insulator Bi2Se3 spherical nanoparticle. Using the electromagnetic Green's tensor method, we find exceptional Purcell factors of the quantum emitter up to 1010 at distances between the emitter and the nanoparticle as large as half the nanoparticle's radius in the terahertz regime. We study the spontaneous emission evolution of a quantum emitter for various transition frequencies in the terahertz and various vacuum decay rates.

Pump-Probe Optical Response and Four-Wave Mixing in a Zinc-Phthalocyanine-Metal Nanoparticle Hybrid System.

We investigate theoretically the optical response of a zinc-phthalocyanine molecular quantum system near a gold spherical nanoparticle with a radius of 80 nm. The quantum system is irradiated by a strong pump and a weak probe coherent electromagnetic field. Using the density matrix methodology, we obtain analytical expressions for the absorption, dispersion, and the four-wave-mixing coefficients.

Topological insulator nanoparticles for strong light-matter interaction in the terahertz regime.

We study the spontaneous emission (SPEM) for a quantum emitter (QUEM) near a topological insulator BiSe nanosphere. We calculate numerically the QUEM Purcell factor near nanospheres of radii between 40 nm and 100 nm, with and without taking into account the topologically protected delocalized states at the surface of the nanosphere. We find exceptionally large Purcell factors up to 10 at distances between the QUEM and the nanosphere as large as half its radius in the terahertz regime.

Nonlinear Optical Rectification in an Inversion-Symmetry-Broken Molecule near a Metallic Nanoparticle.

We study the nonlinear optical rectification of an inversion-symmetry-broken quantum system interacting with an optical field near a metallic nanoparticle, exemplified in a polar zinc-phthalocyanine molecule in proximity to a gold nanosphere. The corresponding nonlinear optical rectification coefficient under external strong field excitation is derived using the steady-state solution of the density matrix equations. We use electronic structure calculations for determining the necessary spectroscopic data of the molecule under study, as well as classical electromagnetic calculations for obtaining the influence of the metallic nanoparticle to the molecular spontaneous decay rates and to the external electric field applied to the molecule.

Correction: Computing the T-matrix of a scattering object with multiple plane wave illuminations.

[This corrects the article DOI: 10.3762/bjnano.8.

Computing the T-matrix of a scattering object with multiple plane wave illuminations.

Given an arbitrarily complicated object, it is often difficult to say immediately how it interacts with a specific illumination. Optically small objects, e.g.

Gold nanoparticles, radiations and the immune system: Current insights into the physical mechanisms and the biological interactions of this new alliance towards cancer therapy.

Considering both cancer's serious impact on public health and the side effects of cancer treatments, strategies towards targeted cancer therapy have lately gained considerable interest. Employment of gold nanoparticles (GNPs), in combination with ionizing and non-ionizing radiations, has been shown to improve the effect of radiation treatment significantly. GNPs, as high-Z particles, possess the ability to absorb ionizing radiation and enhance the deposited dose within the targeted tumors.

Unidirectional Wave Propagation in Low-Symmetric Colloidal Photonic-Crystal Heterostructures.

We show theoretically that photonic crystals consisting of colloidal spheres exhibit unidirectional wave propagation and one-way frequency band gaps without breaking time-reversal symmetry via, e.g., the application of an external magnetic field or the use of nonlinear materials.

Spatiotemporal control of temperature in nanostructures heated by coherent laser fields.

We demonstrate theoretically that it is possible to exercise coherent control of the temperature in nanostructures by laser fields. In particular we show that by use of nanosecond laser pulses it is possible to induce a temperature distribution on a collection of nanoparticles which can last for up to thousands of nanoseconds before assuming the temperature of the environment. Although the form of the temperature distribution depends on the spatiotemporal control of the optical near field induced by the laser field, it is far from being proportional to the local radiation field at a particular point due to the cooling mechanisms which take place among the nanoparticles.

Plasmon-induced enhancement of quantum interference near metallic nanostructures.

We show that the quantum interference between two spontaneous emission channels can be greatly enhanced when a three-level V-type atom is placed near plasmonic nanostructures such as metallic slabs, nanospheres, or periodic arrays of metal-coated spheres. The spontaneous emission rate is calculated by a rigorous first-principles electromagnetic Green's tensor technique. The enhancement of quantum interference is attributed to the strong dependence of the spontaneous emission rate on the orientation of an atomic dipole relative to the surface of the nanostructure at the excitation frequencies of surface plasmons.

First-principles study of Casimir repulsion in metamaterials.

We examine theoretically the Casimir effect between a metallic plate and several types of magnetic metamaterials in pursuit of Casimir repulsion, by employing a rigorous multiple-scattering theory for the Casimir effect. We first examine metamaterials in the form of two-dimensional lattices of inherently nonmagnetic spheres such as spheres made from materials possessing phonon-polariton and exciton-polariton resonances. Although such systems are magnetically active in infrared and optical regimes, the force between finite slabs of these materials and metallic slabs is plainly attractive since the effective electric permittivity is larger than the magnetic permeability for the studied spectrum.

All-optical nanotraps for atoms atop flat metamaterial lenses: a theoretical study.

We propose a novel setup for optically trapping neutral atoms based upon the focusing properties of metamaterials. The optical trap is created at the focal point of an inverted-opal crystal when the latter is illuminated by a localized light source. The trap is located away from the surface of the inverted-opal lens, rendering the Casimir-Polder attraction exerted by the lens on the atom negligible.

Circular dichroism in planar nonchiral plasmonic metamaterials.

It is shown theoretically that a nonchiral, two-dimensional array of metallic spheres exhibits optical activity as manifested in calculations of circular dichroism. The metallic spheres occupy the sites of a rectangular lattice, and for off-normal incidence they show a strong circular-dichroism effect around the surface-plasmon frequencies. The optical activity is a result of the rectangular symmetry of the lattice, which gives rise to different polarization modes of the crystal along the two orthogonal primitive lattice vectors.

Optical switching of electric charge transfer pathways in porphyrin: a light-controlled nanoscale current router.

We introduce a novel molecular junction based on a thiol-functionalized porphyrin derivative with two almost energetically degenerate equilibrium configurations. We show that each equilibrium structure defines a pathway of maximal electric charge transfer through the molecular junction and that these two conduction pathways are spatially orthogonal. We further demonstrate computationally how to switch between the two equilibrium structures of the compound by coherent light.

Fluctuational electrodynamics in the presence of finite thermal sources.

We present exact calculations of the spatial correlation of the blackbody radiation in the presence of spheres whose dimensions are smaller or comparable to the radiation wavelength. By going beyond the standard scalar coherence theory, we show that the spatial correlation function of a spherical thermal source is not universal but depends on the material properties of the source and exhibits near-field-induced features. Near-field effects are also manifested in the case of a linear chain of dielectric spheres where the correlation function probes the inhomogeneity of the chain.

First-principles theory of van der Waals forces between macroscopic bodies.

We present a first-principles method for the determination of the van der Waals interactions for a collection of finite-sized macroscopic bodies. The method is based on fluctuational electrodynamics and a rigorous multiple-scattering method for the electromagnetic field. As such, the method takes fully into account retardation, many-body, multipolar, and near-fields effects.

Negative refractive index metamaterials from inherently non-magnetic materials for deep infrared to terahertz frequency ranges.

We present a new set of artificial structures which can exhibit a negative refractive index band in excess of 6% in a broad frequency range from the deep infrared to the terahertz region. The structures are composites of two different kinds of non-overlapping spheres, one made from inherently non-magnetic polaritonic and the other from a Drude-like material. The polaritonic spheres are responsible for the existence of negative effective magnetic permeability whilst the Drude-like spheres are responsible for negative effective electric permittivity.